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Strong Tough Polyampholyte Hydrogels via the Synergistic Effect of Ionic and Metal–Ligand Bonds

https://doi.org/10.1002/adfm.202103917

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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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inferred← citeshttps://doi.org/10.1016/j.cej.2024.155206openalex-snapshot

Hydrogels mimicking the viscoelasticity of extracellular matrix for regenerative medicine: Design, application, and molecular mechanism

inferred← citeshttps://doi.org/10.1016/j.cej.2024.156800openalex-snapshot

Ultra-stretchable, robust, self-healable conductive hydrogels enabled by the synergistic effects of hydrogen bonds and ionic coordination bonds toward high-performance e-skins

inferred← citeshttps://doi.org/10.1016/j.cej.2024.158401openalex-snapshot

Large-scalable, flexible and durable MXene/gelatin composite film for electromagnetic shielding and self-powered sensing

inferred← citeshttps://doi.org/10.1016/j.cej.2025.160329openalex-snapshot

Multifunctional flexible MXene/TA@CNC electronic hydrogel patch with robust adhesion and self-healing properties for wearable electronics

inferred← citeshttps://doi.org/10.1016/j.cej.2025.160657openalex-snapshot

Skin-like soft yet robust hydrogels with rapid mechanical and electronic responses

inferred← citeshttps://doi.org/10.1016/j.cej.2025.160728openalex-snapshot

Strong and tough hydrogels fabricated through molecular and structural engineering and their biomedical applications

inferred← citeshttps://doi.org/10.1016/j.cej.2025.168286openalex-snapshot

“Subject-object” multi-scale regulated aluminum coordination hydrogel self-powered sensors for percussion instruments application

inferred← citeshttps://doi.org/10.1016/j.cej.2026.180102openalex-snapshot

Stretchable, rapid adhesion and high-efficient self-healing ionogels for wearable sensing and long-term electrophysiological signal monitoring

inferred← citeshttps://doi.org/10.1016/j.cis.2025.103610openalex-snapshot

Advanced conductive eutectogel material for flexible sensor applications

inferred← citeshttps://doi.org/10.1016/j.colsurfa.2025.136145openalex-snapshot

Enhanced anti-corrosion performance of sodium carboxymethyl cellulose coating on 5052 aluminium alloy via rapid gelation by metal ions

inferred← citeshttps://doi.org/10.1016/j.compositesb.2022.109895openalex-snapshot

Recent advances in 3D printing of tough hydrogels: A review

inferred← citeshttps://doi.org/10.1016/j.compscitech.2024.110732openalex-snapshot

Enhanced mechanical strength and stretchable ionic conductive hydrogel with double-network structure for wearable strain sensing and energy harvesting

inferred← citeshttps://doi.org/10.1016/j.envres.2025.123347openalex-snapshot

Functional hydrogels—enabling the gateway for sustainable water treatment and harvesting technologies

inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2022.111277openalex-snapshot

Adhesion mechanism and application progress of hydrogels

inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2022.111327openalex-snapshot

Long/Short chain Crosslinkers-optimized and PEDOT:PSS-enhanced covalent double network hydrogels rapidly prepared under green LED irradiation as flexible strain sensor

inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2022.111628openalex-snapshot

Strong and tough collagen/cellulose nanofibril composite films via the synergistic effect of hydrogen and metal–ligand bonds

inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2024.112895openalex-snapshot

Recent progress in fabrications, properties and applications of multifunctional conductive hydrogels

inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2025.114195openalex-snapshot

Performance of main-chain polyimidazolium ionic liquid-based elastomer

inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2026.114547openalex-snapshot

Dynamic covalent network toughened PBAT/MMT thermoplastic nanocomposite through melt grafting and reversible boronic ester crosslinking

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2023.125978openalex-snapshot

Tough polyvinyl alcohol-gelatin biological macromolecules ionic hydrogel temperature, humidity, stress and strain, sensors

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2024.129378openalex-snapshot

Rapid fabricated in-situ polymerized lignin hydrogel sensor with highly adjustable mechanical properties

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2024.130511openalex-snapshot

Strong and tough poly(vinyl alcohol)/xanthan gum-based ionic conducting hydrogel enabled through the synergistic effect of ion cross-linking and salting out

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2024.132994openalex-snapshot

Extreme condition-tolerant stretchable flexible supercapacitor and triboelectric nanogenerator based on carrageenan-enhanced gel for energy storage, energy collection and self-powered sensing

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2024.136128openalex-snapshot

Highly sensitive and structure stable polyvinyl alcohol hydrogel sensor with tailored free water fraction and multiple networks by reinforcement of conductive nanocellulose

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2025.146671openalex-snapshot

Conductive, flexible, and adhesive lignin-polyacrylic acid hydrogel crosslinked with aluminum ions for supercapacitors

inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2026.150839openalex-snapshot

Cellulose nanofibers-stabilized molybdenum disulfide nanosheets enhanced tough hydrogel for highly efficient marine antifouling

inferred← citeshttps://doi.org/10.1016/j.jcis.2023.09.193openalex-snapshot

Durable hydrogel-based lubricated composite coating with remarkable underwater performances

inferred← citeshttps://doi.org/10.1016/j.jclepro.2022.135705openalex-snapshot

Strong, water-repellent, and recyclable gelatin-based bioplastic film as sustainable express packaging film

inferred← citeshttps://doi.org/10.1016/j.jiec.2022.07.048openalex-snapshot

Robust, fatigue resistant, self-healing and antifreeze ionic conductive supramolecular hydrogels for wearable flexible sensors

inferred← citeshttps://doi.org/10.1016/j.jmps.2025.106243openalex-snapshot

Toughening mechanism of macroscale heterogeneous soft materials: a systematic study from the perspective of energy release rate

inferred← citeshttps://doi.org/10.1016/j.matdes.2026.116739openalex-snapshot

Design strategy, properties and application of high-strength and tough hydrogel: A review

inferred← citeshttps://doi.org/10.1016/j.matlet.2022.132582openalex-snapshot

Strengthening and stiffening in swollen polyampholyte hydrogels

inferred← citeshttps://doi.org/10.1016/j.molliq.2023.121411openalex-snapshot

Network structure and viscoelastic behavior of high-strength crystal microphase crosslinking hydrogels analyzed from combined model

inferred← citeshttps://doi.org/10.1016/j.mseb.2025.118175openalex-snapshot

Stretchable, tough, self-healing, antifreezing, and multifunctional nanocellulose-based hydrogel for wearable monitoring of human motion

inferred← citeshttps://doi.org/10.1016/j.mtchem.2025.102683openalex-snapshot

Highly flexible, self-healing, adhesive, conductive and temperature-resistant eutectogels via a one-step co-crosslinking method for real-time wearable sensors

inferred← citeshttps://doi.org/10.1016/j.mtcomm.2024.110993openalex-snapshot

Straightforwardly-prepared waterborne polyurethane microspheres with superior matting properties by calcium ion-coordinated coagulation

inferred← citeshttps://doi.org/10.1016/j.mtcomm.2025.112720openalex-snapshot

Multifunctional conductive hydrogels with layered polydopamine-coated polyaniline for high-sensitivity small-deformation flexible sensing

inferred← citeshttps://doi.org/10.1016/j.newton.2025.100287openalex-snapshot

Time-temperature-moisture superposition principle of hydrophilic polymer amorphous cellulose

inferred← citeshttps://doi.org/10.1016/j.polymer.2022.124621openalex-snapshot

Tough and rapidly stimuli-responsive luminescent hydrogels for multi-dimensional information encryption and storage

inferred← citeshttps://doi.org/10.1016/j.polymer.2023.126238openalex-snapshot

Extreme condition-resistant flexible triboelectric nanogenerator and sensor based on swollen-yet-enhanced and self-healing deep eutectic gel

inferred← citeshttps://doi.org/10.1016/j.polymer.2024.127465openalex-snapshot

Tough and conductive PVA-based double-network ionic hydrogels for flexible sensors

inferred← citeshttps://doi.org/10.1016/j.polymer.2025.128049openalex-snapshot

DLP printing PEG-based gels with high elasticity and anti-dryness for customized flexible sensors

inferred← citeshttps://doi.org/10.1016/j.polymer.2025.128743openalex-snapshot

High-strength, conductive dual-network nanocomposite hydrogel for multi-substrate adhesion and enhanced wearable sensor performance

inferred← citeshttps://doi.org/10.1016/j.polymer.2025.129145openalex-snapshot

Evaluating the effect of strong binding affinity ions on mechanical properties, electrical conductivity, and weldability of conductive alginate-based hydrogels

inferred← citeshttps://doi.org/10.1016/j.polymertesting.2022.107720openalex-snapshot

Tough, flexible, and durable all-polyampholyte hydrogel supercapacitor

inferred← citeshttps://doi.org/10.1016/j.polymertesting.2023.108089openalex-snapshot

Anti-swelling P(DAC-co-NaSS-co-VDT) polyampholyte hydrogel with solvent displacement and salinity enhanced wet strength and adhesion

inferred← citeshttps://doi.org/10.1016/j.polymertesting.2025.108844openalex-snapshot

Construction of silane-modified polyampholyte hydrogel coatings for multi-scale antibiofouling

inferred← citeshttps://doi.org/10.1016/j.progpolymsci.2022.101622openalex-snapshot

Role of divalent metal ions in the function and application of hydrogels

inferred← citeshttps://doi.org/10.1016/j.revmat.2025.100018openalex-snapshot

Emerging frontiers of conductive supramolecular hydrogels in biomedical applications

inferred← citeshttps://doi.org/10.1016/j.seppur.2024.127492openalex-snapshot

Leaching of palladium from spent Pd/Al2O3 catalysts by coupled ultrasound-microwave technique

inferred← citeshttps://doi.org/10.1016/j.tramat.2025.100041openalex-snapshot

Highly stretchable strain sensors using conductive MoS2 composited PVA-PAA-Li+ hydrogels for information interaction

inferred← citeshttps://doi.org/10.1016/j.wasman.2022.04.023openalex-snapshot

Gelatin from leather waste to tough biodegradable packaging film: One valuable recycling solution for waste gelatin from leather industry

inferred← citeshttps://doi.org/10.1016/j.watcyc.2022.09.001openalex-snapshot

A combined electrodialysis and coal dust suppression system for acid mine drainage treatment and high mechanical hydrogel dust suppressant generation

inferred← citeshttps://doi.org/10.1021/acs.cgd.4c01096openalex-snapshot

Salt Whisker Growth through Macromolecular Crowding Matrix Regulation

inferred← citeshttps://doi.org/10.1021/acs.chemmater.2c02791openalex-snapshot

Regulating Protein Secondary Structures Enables Versatile Hydrogels with Tunable Mechanical Properties

inferred← citeshttps://doi.org/10.1021/acs.chemmater.3c00572openalex-snapshot

Customization of Supramolecular Hydrogels through One-Step Photopolymerization and Its Mechanism

inferred← citeshttps://doi.org/10.1021/acs.chemmater.3c01092openalex-snapshot

Micelle–Micelle Cross-Linked Highly Stretchable Conductive Hydrogels for Potential Applications of Strain and Electronic Skin Sensors

inferred← citeshttps://doi.org/10.1021/acs.chemrev.2c00618openalex-snapshot

Cellulose-Based Ionic Conductor: An Emerging Material toward Sustainable Devices

inferred← citeshttps://doi.org/10.1021/acs.iecr.4c02987openalex-snapshot

An Economic Naked-Eye Visualization Detection of Heavy Metal Ions Using a Shape Memory Hydrogel

inferred← citeshttps://doi.org/10.1021/acs.iecr.6c01840openalex-snapshot

Multiple Networked Cellulose Nanofiber/Sodium Alginate/Polyacrylamide Hydrogels Toughened by Interfacial Ionic Bond Engineering for Pressure Sensors

inferred← citeshttps://doi.org/10.1021/acs.macromol.2c01386openalex-snapshot

Effect of Hydrophobic Side Group on Structural Heterogeneities and Mechanical Performance of Gelatin-Based Hydrogen-Bonded Hydrogel

inferred← citeshttps://doi.org/10.1021/acs.macromol.3c02335openalex-snapshot

Structure–Property Relationships of Granular Hybrid Hydrogels Formed through Polyelectrolyte Complexation

inferred← citeshttps://doi.org/10.1021/acs.macromol.4c02688openalex-snapshot

Ferric Salt-Mediated Tough Zwitterionic Hydrogel

inferred← citeshttps://doi.org/10.1021/acs.macromol.5c00756openalex-snapshot

Tough Hybrid Hydrogels with Exceptional Swollen-State Mechanical Robustness via Nanocrystalline Domain Engineering

inferred← citeshttps://doi.org/10.1021/acs.macromol.5c01293openalex-snapshot

Recyclable Strong Tough Ionogels via the Synergy of Solvent-Induced Cross-Linking and Chain Entanglement

inferred← citeshttps://doi.org/10.1021/acs.macromol.5c01426openalex-snapshot

Enhancing the Mechanical Properties of Hydrogels Based on Photo-Polymerizable π-Conjugated Polymers

inferred← citeshttps://doi.org/10.1021/acs.macromol.5c02758openalex-snapshot

Bioinspired Ion-Mediated Repair Strategy for Irreversibly Covalently Cross-Linked Double-Network Hydrogels

inferred← citeshttps://doi.org/10.1021/acs.macromol.6c01161openalex-snapshot

Dangling-Chain Topology Enables Synergistic Dissipation in Hierarchical Aggregate Elastomers

inferred← citeshttps://doi.org/10.1021/acs.nanolett.6c01768openalex-snapshot

Boltzmann Statistics of Viscoelasticity in High-Strength and -Toughness Hydrogels

inferred← citeshttps://doi.org/10.1021/acsaelm.4c00985openalex-snapshot

Self-Healing Natural Rubber Based on the Double Cross-Linked Networks for Fabrication of the Flexible Electronic Sensor

inferred← citeshttps://doi.org/10.1021/acsami.2c04614openalex-snapshot

Biomimetic Microstructured Antifatigue Fracture Hydrogel Sensor for Human Motion Detection with Enhanced Sensing Sensitivity

inferred← citeshttps://doi.org/10.1021/acsami.2c04791openalex-snapshot

Highly Resilient Dual-Crosslinked Hydrogel Adhesives Based on a Dopamine-Modified Crosslinker

inferred← citeshttps://doi.org/10.1021/acsami.2c07963openalex-snapshot

Strong–Weak Response Network-Enabled Ionic Conductive Hydrogels with High Stretchability, Self-Healability, and Self-Adhesion for Ionic Sensors

inferred← citeshttps://doi.org/10.1021/acsami.2c15138openalex-snapshot

Significant Roles of Ions in Enhancing and Functionalizing Anisotropic Hydrogels

inferred← citeshttps://doi.org/10.1021/acsami.3c18077openalex-snapshot

Masking Strategy Constructed Metal Coordination Hydrogels with Improved Mechanical Properties for Flexible Electronic Sensors

inferred← citeshttps://doi.org/10.1021/acsami.4c18098openalex-snapshot

One-Step Digital Light Processing 3D Printing of Robust, Conductive, Shape-Memory Hydrogel for Customizing High-Performance Soft Devices

inferred← citeshttps://doi.org/10.1021/acsami.6c09270openalex-snapshot

Fabrication of Liquid Metal Composite Ionic Liquid Hydrogels for Antifouling Application

inferred← citeshttps://doi.org/10.1021/acsapm.2c01993openalex-snapshot

Ultra-adhesive Poly(acrylic acid)-Based Hydrogel as a Flexible Sensor for Capturing Human-Motion Signal

inferred← citeshttps://doi.org/10.1021/acsapm.3c00818openalex-snapshot

Tough Ion-Conductive Hydrogel with Anti-Dehydration as a Stretchable Strain Sensor for Gesture Recognition

inferred← citeshttps://doi.org/10.1021/acsapm.3c01497openalex-snapshot

Ionically Conductive and Self-Healing Polyampholyte Hydrogels for Wearable Resistive Strain Sensors and Capacitive Pressure Sensors

inferred← citeshttps://doi.org/10.1021/acsapm.4c02651openalex-snapshot

Tough Porous Hydrogels for Ultrasensitive Naked-Eye and Fluorescence Dual-Mode Detection of Iron(III)

inferred← citeshttps://doi.org/10.1021/acsapm.4c03356openalex-snapshot

Antibacterial, Nontoxic, Antifreezing, and Self-Adhesive Conductive Eutectogel for Strain Sensor

inferred← citeshttps://doi.org/10.1021/acsapm.5c00649openalex-snapshot

Efficient Control of Swelling and Strength of Polyacrylamide/Polyacrylic Acid/Chitosan Hydrogels for NaF Release

inferred← citeshttps://doi.org/10.1021/acsapm.5c01935openalex-snapshot

Zr4+ Coordination and LiCl Synergistically Enhanced High-Strength Antifreezing Conductive Hydrogels for Wearable Sensing Application

inferred← citeshttps://doi.org/10.1021/acsapm.5c03982openalex-snapshot

Tough, Transparent, and Multifunctional Zwitterionic Eutectogels Enabled by Metal-Salt Deep Eutectic Solvents

inferred← citeshttps://doi.org/10.1021/acsbiomaterials.6c00916openalex-snapshot

Natural Bone Regeneration-Inspired Poly(Lipoic Acid)-Based Organic–Inorganic Bone Adhesive for Osteoporotic Bone Defect Repair

inferred← citeshttps://doi.org/10.1021/acsnano.5c04885openalex-snapshot

Iontronics: Neuromorphic Sensing and Energy Harvesting

inferred← citeshttps://doi.org/10.1021/acsnano.5c19580openalex-snapshot

Programming Homogeneous Hydrogels Using Directional Ion Transport toward Rapid 3D Reconfiguration

inferred← citeshttps://doi.org/10.1021/acsomega.3c04966openalex-snapshot

Ultrahigh-Ionic-Conductivity, Antifreezing Poly(amidoxime)-Grafted Polyzwitterion Hydrogel for Facile Integrated into High-Performance Stretchable Flexible Supercapacitor

inferred← citeshttps://doi.org/10.1021/acssensors.6c02467openalex-snapshot

Deep-Eutectic-Solvent-Enabled Polyampholyte/MXene Eutectogels for Environmentally Tolerant Wearable Respiratory Monitoring

inferred← citeshttps://doi.org/10.1021/cbe.4c00129openalex-snapshot

Design and Fabrication of Viscoelastic Hydrogels as Extracellular Matrix Mimicry for Cell Engineering

inferred← citeshttps://doi.org/10.1038/s41378-023-00591-3openalex-snapshot

Stretchable and durable HD-sEMG electrodes for accurate recognition of swallowing activities on complex epidermal surfaces

inferred← citeshttps://doi.org/10.1038/s41467-024-47597-7openalex-snapshot

3D printable strong and tough composite organo-hydrogels inspired by natural hierarchical composite design principles

inferred← citeshttps://doi.org/10.1038/s41467-026-70223-7openalex-snapshot

Oligomeric-solvent engineering of hierarchical hydrogen-bonding networks for multifunctional glass interlayers

inferred← citeshttps://doi.org/10.1039/d1ta08465hopenalex-snapshot

A flexible solid-state supercapacitor with extreme low-temperature tolerance based on an ion conducting ice gel electrolyte

inferred← citeshttps://doi.org/10.1039/d1tb02114aopenalex-snapshot

Synergic influences of network topologies and associative interactions on the microstructures and bulk performances of hydrogels

inferred← citeshttps://doi.org/10.1039/d2mh01299eopenalex-snapshot

Tough hydrogel with high water content and ordered fibrous structures as an artificial human ligament

inferred← citeshttps://doi.org/10.1039/d2mh01451copenalex-snapshot

Hydrogels with ultra-highly additive adjustable toughness under quasi-isochoric conditions

inferred← citeshttps://doi.org/10.1039/d2ra00954dopenalex-snapshot

Highly stretchable, self-healing and conductive silk fibroin-based double network gels via a sonication-induced and self-emulsifying green procedure

inferred← citeshttps://doi.org/10.1039/d2ta05530aopenalex-snapshot

Supramolecular polyelectrolyte hydrogel based on conjoined double-networks for multifunctional applications

inferred← citeshttps://doi.org/10.1039/d2ta07410aopenalex-snapshot

Construction of zwitterionic osmolyte-based hydrogel electrolytes towards stable zinc anode for durable aqueous zinc ion storage and integrated electronics

inferred← citeshttps://doi.org/10.1039/d2ta07834aopenalex-snapshot

Modulation of double-network hydrogels via seeding calcium carbonate microparticles for the engineering of ultrasensitive wearable sensors

inferred← citeshttps://doi.org/10.1039/d2tb02511fopenalex-snapshot

Electrospun fibrous membrane reinforced hydrogels with preferable mechanical and tribological performance as cartilage substitutes

inferred← citeshttps://doi.org/10.1039/d3ra07391bopenalex-snapshot

Revolutionizing biomedicine: advancements, applications, and prospects of nanocomposite macromolecular carbohydrate-based hydrogel biomaterials: a review

inferred← citeshttps://doi.org/10.1039/d3ra07554kopenalex-snapshot

Preparation and dye adsorption properties of activated carbon/clay/sodium alginate composite hydrogel membranes

inferred← citeshttps://doi.org/10.1039/d4mh01862aopenalex-snapshot

Puncture-resistant hydrogels with high mechanical performance achieved by the supersaturated salt

inferred← citeshttps://doi.org/10.1039/d4sc05295aopenalex-snapshot

Recent advances in hydrogel-based flexible strain sensors for harsh environment applications

inferred← citeshttps://doi.org/10.1039/d4sm01430hopenalex-snapshot

Network design for soft materials: addressing elasticity and fracture resistance challenges

inferred← citeshttps://doi.org/10.1039/d4ta02029dopenalex-snapshot

A lignocellulosic biomass-derived polyurethane elastomer with high toughness and excellent crack tolerance

inferred← citeshttps://doi.org/10.1039/d4ta03778bopenalex-snapshot

Anti-swelling and photoresponsive MXene-based polyampholyte hydrogel sensors for underwater positioning and urban waterlogging pre-warning

inferred← citeshttps://doi.org/10.1039/d4tc00998copenalex-snapshot

Biomimetic photonic crystal double-network hydrogel for visual and electrical dual signal bluetooth-enabled wearable sensor

inferred← citeshttps://doi.org/10.1039/d4tc04843aopenalex-snapshot

A transparent ionogel with mechanical robustness enabled by synergistic noncovalent interactions

inferred← citeshttps://doi.org/10.1039/d5mh00588dopenalex-snapshot

Toughening hydrogels with small molecules: tiny matter, big impact

inferred← citeshttps://doi.org/10.1039/d5sm00407aopenalex-snapshot

Interplay of the structures and viscoelastic properties of polyampholyte gels with the interlude of neutral blocks

inferred← citeshttps://doi.org/10.1039/d6mh01579dopenalex-snapshot

Spider-silk-inspired dynamic hard–soft ionogels enabled by solvation-contrast-guided phase separation

showing the first 200 of 222

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