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Radical Decyanations of Unactivated Carbon‐CN Bonds: Recent Achievements and Mechanistic Studies

https://doi.org/10.1002/adsc.202300281

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Nonequilibrium Radical Reductions

inferredcites →https://doi.org/10.1021/jacs.0c04456openalex-snapshot

Generation of Alkyl Radical through Direct Excitation of Boracene-Based Alkylborate

inferredcites →https://doi.org/10.1021/jacs.0c07600openalex-snapshot

Metal-Free, Redox-Neutral, Site-Selective Access to Heteroarylamine via Direct Radical–Radical Cross-Coupling Powered by Visible Light Photocatalysis

inferredcites →https://doi.org/10.1021/jacs.0c11968openalex-snapshot

Polysulfide Anions as Visible Light Photoredox Catalysts for Aryl Cross-Couplings

inferredcites →https://doi.org/10.1021/jacs.2c01458openalex-snapshot

Catalytic Asymmetric Reductive Azaarylation of Olefins via Enantioselective Radical Coupling

inferredcites →https://doi.org/10.1021/jacs.2c08278openalex-snapshot

Intercepting Hydrogen Evolution with Hydrogen-Atom Transfer: Electron-Initiated Hydrofunctionalization of Alkenes

inferredcites →https://doi.org/10.1021/jacs.5b04677openalex-snapshot

Radical Reactions of N-Heterocyclic Carbene Boranes with Organic Nitriles: Cyanation of NHC-Boranes and Reductive Decyanation of Malononitriles

inferredcites →https://doi.org/10.1021/jacs.5b12249openalex-snapshot

Cobalt-Catalyzed Benzylic Borylation: Enabling Polyborylation and Functionalization of Remote, Unactivated C(sp3)–H Bonds

inferredcites →https://doi.org/10.1021/jacs.6b09690openalex-snapshot

Contra-thermodynamic Hydrogen Atom Abstraction in the Selective C–H Functionalization of Trialkylamine N -CH3 Groups

inferredcites →https://doi.org/10.1021/jacs.6b11813openalex-snapshot

Pyridine-Catalyzed Radical Borylation of Aryl Halides

inferredcites →https://doi.org/10.1021/jacs.7b00823openalex-snapshot

Metal-Free Synthesis of C-4 Substituted Pyridine Derivatives Using Pyridine-boryl Radicals via a Radical Addition/Coupling Mechanism: A Combined Computational and Experimental Study

inferredcites →https://doi.org/10.1021/jacs.7b05165openalex-snapshot

Oxidative [1,2]-Brook Rearrangements Exploiting Single-Electron Transfer: Photoredox-Catalyzed Alkylations and Arylations

inferredcites →https://doi.org/10.1021/jacs.7b09394openalex-snapshot

Transition-Metal-Free Radical C(sp3)–C(sp2) and C(sp3)–C(sp3) Coupling Enabled by 2-Azaallyls as Super-Electron-Donors and Coupling-Partners

inferredcites →https://doi.org/10.1021/jacs.8b07539openalex-snapshot

TiO2 Nanoparticles Functionalized with Non-innocent Ligands Allow Oxidative Photocyanation of Amines with Visible/Near-Infrared Photons

inferredcites →https://doi.org/10.1021/jacs.8b08933openalex-snapshot

A Toolbox Approach To Construct Broadly Applicable Metal-Free Catalysts for Photoredox Chemistry: Deliberate Tuning of Redox Potentials and Importance of Halogens in Donor–Acceptor Cyanoarenes

inferredcites →https://doi.org/10.1021/jacs.8b10238openalex-snapshot

Radical Hydroarylation of Functionalized Olefins and Mechanistic Investigation of Photocatalytic Pyridyl Radical Reactions

inferredcites →https://doi.org/10.1021/jacs.8b13652openalex-snapshot

Rhodium-Catalyzed Aldehyde Arylation via Formate-Mediated Transfer Hydrogenation: Beyond Metallic Reductants in Grignard/Nozaki–Hiyami–Kishi-Type Addition

inferredcites →https://doi.org/10.1021/jacs.8b13709openalex-snapshot

Nickel-Catalyzed Addition of Aryl Bromides to Aldehydes To Form Hindered Secondary Alcohols

inferredcites →https://doi.org/10.1021/jacs.9b03973openalex-snapshot

Catalytic Ring Expansions of Cyclic Alcohols Enabled by Proton-Coupled Electron Transfer

inferredcites →https://doi.org/10.1021/jacs.9b07564openalex-snapshot

1,2-Boron Shifts of β-Boryl Radicals Generated from Bis-boronic Esters Using Photoredox Catalysis

inferredcites →https://doi.org/10.1021/jacs.9b10870openalex-snapshot

Electrochemical Synthesis of Hindered Primary and Secondary Amines via Proton-Coupled Electron Transfer

inferredcites →https://doi.org/10.1021/jacs.9b10871openalex-snapshot

Synthesis of Sterically Hindered Primary Amines by Concurrent Tandem Photoredox Catalysis

inferredcites →https://doi.org/10.1021/jacs.9b12490openalex-snapshot

Remote Nickel-Catalyzed Cross-Coupling Arylation via Proton-Coupled Electron Transfer-Enabled C–C Bond Cleavage

inferredcites →https://doi.org/10.1021/jacs.9b13165openalex-snapshot

Highly Diastereoselective Functionalization of Piperidines by Photoredox-Catalyzed α-Amino C–H Arylation and Epimerization

inferredcites →https://doi.org/10.1021/jm060854fopenalex-snapshot

4,5-Dihydroxypyrimidine Carboxamides and N-Alkyl-5-hydroxypyrimidinone Carboxamides Are Potent, Selective HIV Integrase Inhibitors with Good Pharmacokinetic Profiles in Preclinical Species

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Analysis of the Structural Diversity, Substitution Patterns, and Frequency of Nitrogen Heterocycles among U.S. FDA Approved Pharmaceuticals

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Photochemistry induced allylic hydrogen from 1-X-1,2-dialkylethylenes: experimental data and theoretical calculations

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Notes-Alkylation Reactions in Dimethyl Sulfoxide

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Electroreductive Dimerization of Coumarin and Coumarin Analogues at Carbon Cathodes

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Avoiding Olefin Isomerization During Decyanation of Alkylcyano α,ω-Dienes: A Deuterium Labeling and Structural Study of Mechanism

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Magnetic Field Effects on Chemical Reactions of Biradical Radical Ion Pairs in Homogeneous Fluid Solvents

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Reducing Power of Photogenerated α-Hydroxy Radicals. Proton-Coupled Electron Transfer

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Iron-Catalyzed Allylic Arylation of Olefins via C(sp 3 )–H Activation under Mild Conditions

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Electron Transfer Reduction of Nitriles Using SmI 2 –Et 3 N–H 2 O: Synthetic Utility and Mechanism

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Highly efficient organic light-emitting diodes from delayed fluorescence

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The direct arylation of allylic sp3 C–H bonds via organic and photoredox catalysis

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Iterative reactions of transient boronic acids enable sequential C–C bond formation

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Transition-metal-free chemo- and regioselective vinylation of azaallyls

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Photoredox-catalyzed branch-selective pyridylation of alkenes for the expedient synthesis of Triprolidine

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Palladium-catalyzed asymmetric allylic 4-pyridinylation via electroreductive substitution reaction

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Accessing chiral sulfones bearing quaternary carbon stereocenters via photoinduced radical sulfur dioxide insertion and Truce–Smiles rearrangement

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Organic synthesis provides opportunities to transform drug discovery

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Direct α-alkylation of primary aliphatic amines enabled by CO2 and electrostatics

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From alkylarenes to anilines via site-directed carbon–carbon amination

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A family of luminescent coordination compounds: iridium(iii) polyimine complexes

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Practical iron-catalyzed dehalogenation of aryl halides

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Nickel-catalyzed decyanation of inert carbon–cyano bonds

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A new radical decarboxylation reaction for the conversion of carboxylic acids into hydrocarbons

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Active participation of amine-derived radicals in photoredox catalysis as exemplified by a reductive cyclization

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Photoinduced direct 4-pyridination of C(sp3)–H Bonds

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Asymmetric catalysis activated by visible light

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Olefinic C–H functionalization through radical alkenylation

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Reductive decyanation of malononitriles and cyanoacetates using photoactivated neutral organic super-electron-donors

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Catalytic enantioselective organic transformations via visible light photocatalysis

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Boron chemistry in a new light

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Decarboxylative reactions with and without light – a comparison

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Arylation of benzyl amines with aromatic nitriles

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What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

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Progression on Oxidative Decyanation Approaches from Secondary Nitriles to Ketones and α‐Aminonitriles to Amides

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Metal Free Functionalization of Saturated Heterocycles with Vinylarenes and Pyridine Enabled by Photocatalytic Hydrogen Atom Transfer

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Photocatalytic Reductive Azaarenylation of Cyclopropanes via Consecutive Photo‐induced Electron Transfer: A Facile Route to α‐Quaternary Azaarenes †

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Hazards and mitigation measures of applying biochar in water, soil, plants, animals and atmospheric for environmental safety

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Exploring the reactivity of hydroxyl and sulfate radicals in enhancing water decontamination processes

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Ir-catalyzed photoredox cascade radical annulation reactions toward phosphinimides bearing quaternary carbon center at room temperature

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[Cu]/NFSI-Mediated Cascade Diels–Alder Radical Annulations Using Norbornene as H-Acceptor under Redox-Neutral Conditions

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Paired Electrolysis-Enabled Arylation of Quinoxalin-2(1H)-ones

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Modular Room Temperature Synthesis of Sulfoximidoyl Amidines Enabled by Pd-Catalyzed Cascade Aza-Claisen Rearrangement Strategy

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Photocatalytic Consecutive Photoinduced Electron Transfer-Enabled C(sp3)–H Pyridylation of Dihydroquinoxalin-2-ones

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Photocatalytic Redox-Neutral C(sp3)–C(sp3) Cleaving Transalkylation of Heteroarenes

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Copper-Catalyzed Regio- and Stereo-Defined Protocols to Access β-Aminated Carbonyl Derivatives

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Photoredox 1,2-Alkylarylation of Alkenes with 1-(Allyloxy)-2-iodobenzenes and Cyano(hetero)aromatics Involving XAT-Enabled Annulation

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Visible-Light-Induced Acylative Pyridylation of Styrenes

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Decyanative Heteroarylations of Glycine Derivatives

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Dual Inert C–H Bond Site-Selective Activations Enabled by Pd/Norbornene-Mediated Cascade Cyclization toward Medium-Sized Polyheterocyclic Methylene Sulfoximines

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Photocatalytic Pyridyl-carbamoylation of Alkenes for Accessing β-Pyridyl Amides

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Relay Photocatalyzed Reductive Cleavage of C sp 2 –I To Establish Radical Cyclization/Coupling between O-Tethered Iodoarenes with Cyanoarenes

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Electrochemical Decyanative Carboxylation of Cyanoaromatics with CO2 Leading to Aryl Carboxylic Acids

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Electroreductive α-Aminoalkylation of Sulfonylazoles with Amines and Aldehydes

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Photocatalytic Three-Component Glycosylation of Styrenes with Glycosyl Acids and Pyridines via Decarboxylation

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Harnessing the potential of acyl triazoles in bifunctional cobalt-catalyzed radical cross-coupling reactions

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Switchable electrochemical pathways for the selective C(sp3)-Ge bond formation

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Photocatalytic redox-neutral α-C(sp 3 )–H pyridination of glycine derivatives and N -arylamines with cyanopyridines

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Organophotocatalytic pyridination of N -arylglycines with 4-cyanopyridines by decarboxylative and decyanative radical–radical coupling

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Photoinduced three-component alkylpyridination of alkenes via spiro-dihydroquinazolinone fragmentation

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Harnessing the reactivity of captodative radicals: photocatalytic α-pyridination of glycyl derivatives through reversible radical coupling

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Rapid access to difluoroalkyl phosphinimide heterocycles and their preliminary biological activities toward the cathepsin D active site

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Photocatalytic three-component 1,2-boroarylation and carbopyridylation of alkene

inferred← citeshttps://doi.org/10.1039/d5qo01578bopenalex-snapshot

Benzophenone-catalyzed alkenylative pyridylation of vinylarenes with alkenylboronic esters

inferred← citeshttps://doi.org/10.1039/d6gc00661bopenalex-snapshot

Non-decarboxylative functionalization of free carboxylic acids: strategies for C–O bond formation via photo- and electrochemical approaches

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1,2-Diketones as in situ persistent radical precursors: symmetric and unsymmetric diacylation of alkenes under visible light

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Recent progress on annulation reactions of aromatic nitriles

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