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Bioinspired design of elastomeric vitrimers with sacrificial metal-ligand interactions leading to supramechanical robustness and retentive malleability

https://doi.org/10.1016/j.matdes.2020.108756
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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

inferredcites →https://doi.org/10.1002/adma.201901561openalex-snapshot
Multiscale Toughening Mechanisms in Biological Materials and Bioinspired Designs
inferredcites →https://doi.org/10.1002/anie.201504127openalex-snapshot
Catalytic Silylations of Alcohols: Turning Simple Protecting‐Group Strategies into Powerful Enantioselective Synthetic Methods
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Dynamic Covalent Bonds in Polymeric Materials
inferredcites →https://doi.org/10.1002/mame.200400034openalex-snapshot
The Reinforcement of Elastomeric Networks by Fillers
inferredcites →https://doi.org/10.1002/pola.28577openalex-snapshot
Recyclable polybutadiene elastomer based on dynamic imine bond
inferredcites →https://doi.org/10.1007/s10118-018-2131-xopenalex-snapshot
Effects of Binding Energy of Bioinspired Sacrificial Bond on Mechanical Performance of cis-1,4-Polyisoprene with Dual-crosslink
inferredcites →https://doi.org/10.1016/j.cej.2019.123820openalex-snapshot
Vitrimers: Associative dynamic covalent adaptive networks in thermoset polymers
inferredcites →https://doi.org/10.1016/j.compositesb.2008.01.002openalex-snapshot
Effects of particle size, particle/matrix interface adhesion and particle loading on mechanical properties of particulate–polymer composites
inferredcites →https://doi.org/10.1016/j.compscitech.2018.10.017openalex-snapshot
Reprocessable and robust crosslinked elastomers via interfacial C N transalkylation of pyridinium
inferredcites →https://doi.org/10.1016/j.eurpolymj.2016.03.016openalex-snapshot
From landfilling to vitrimer chemistry in rubber life cycle
inferredcites →https://doi.org/10.1016/j.pmatsci.2009.05.001openalex-snapshot
Merger of structure and material in nacre and bone – Perspectives on de novo biomimetic materials
inferredcites →https://doi.org/10.1016/j.pmatsci.2012.03.001openalex-snapshot
Biological materials: Functional adaptations and bioinspired designs
inferredcites →https://doi.org/10.1016/j.polymer.2010.10.023openalex-snapshot
Epoxidized natural rubber/dicarboxylic acid self-vulcanized blends
inferredcites →https://doi.org/10.1016/j.polymer.2018.06.042openalex-snapshot
Tailoring vinylogous urethane chemistry for the cross-linked polybutadiene: Wide freedom design, multiple recycling methods, good shape memory behavior
inferredcites →https://doi.org/10.1016/j.tet.2013.01.017openalex-snapshot
Selective deprotection of silyl ethers
inferredcites →https://doi.org/10.1016/s0032-3861(96)00710-0openalex-snapshot
Partial conversion of epoxide groups to diols in epoxidized natural rubber
inferredcites →https://doi.org/10.1016/s0079-6700(00)00020-4openalex-snapshot
Reclamation and recycling of waste rubber
inferredcites →https://doi.org/10.1016/s1386-1425(02)00013-6openalex-snapshot
Vibrational assignment of aluminum(III) Tris–acetylacetone
inferredcites →https://doi.org/10.1021/acs.iecr.8b05309openalex-snapshot
Multifunctional Vitrimer-Like Polydimethylsiloxane (PDMS): Recyclable, Self-Healable, and Water-Driven Malleable Covalent Networks Based on Dynamic Imine Bond
inferredcites →https://doi.org/10.1021/acs.macromol.6b00826openalex-snapshot
Silica–Epoxy Vitrimer Nanocomposites
inferredcites →https://doi.org/10.1021/acs.macromol.7b01261openalex-snapshot
Malleable, Mechanically Strong, and Adaptive Elastomers Enabled by Interfacial Exchangeable Bonds
inferredcites →https://doi.org/10.1021/acs.macromol.9b00419openalex-snapshot
Mechanically Robust, Self-Healable, and Reprocessable Elastomers Enabled by Dynamic Dual Cross-Links
inferredcites →https://doi.org/10.1021/acs.macromol.9b00503openalex-snapshot
Using Dynamic Bonds to Enhance the Mechanical Performance: From Microscopic Molecular Interactions to Macroscopic Properties
inferredcites →https://doi.org/10.1021/acsami.8b09863openalex-snapshot
Covalently Cross-Linked Elastomers with Self-Healing and Malleable Abilities Enabled by Boronic Ester Bonds
inferredcites →https://doi.org/10.1021/acsmacrolett.8b00166openalex-snapshot
Vitrimeric Silicone Elastomers Enabled by Dynamic Meldrum’s Acid-Derived Cross-Links
inferredcites →https://doi.org/10.1021/acsmacrolett.9b00012openalex-snapshot
Integrating Sacrificial Bonds into Dynamic Covalent Networks toward Mechanically Robust and Malleable Elastomers
inferredcites →https://doi.org/10.1021/acssuschemeng.9b01875openalex-snapshot
Mechanically Robust and Recyclable EPDM Rubber Composites by a Green Cross-Linking Strategy
inferredcites →https://doi.org/10.1021/ja01466a014openalex-snapshot
Infrared Spectra of Metal Chelate Compounds. II. Infrared Spectra of Acetylacetonates of Trivalent Metals1
inferredcites →https://doi.org/10.1021/ja303356zopenalex-snapshot
Making Insoluble Polymer Networks Malleable via Olefin Metathesis
inferredcites →https://doi.org/10.1021/jacs.5b01601openalex-snapshot
Enhancing Mechanical Performance of a Covalent Self-Healing Material by Sacrificial Noncovalent Bonds
inferredcites →https://doi.org/10.1021/jacs.7b08826openalex-snapshot
Silyl Ether as a Robust and Thermally Stable Dynamic Covalent Motif for Malleable Polymer Design
inferredcites →https://doi.org/10.1021/jacs.9b07922openalex-snapshot
Adaptable Crosslinks in Polymeric Materials: Resolving the Intersection of Thermoplastics and Thermosets
inferredcites →https://doi.org/10.1021/ma2001614openalex-snapshot
Structure and Dynamics of Zinc-Neutralized Sulfonated Polystyrene Ionomers
inferredcites →https://doi.org/10.1021/ma500240vopenalex-snapshot
Evidence for an in Situ Developed Polymer Phase in Ionic Elastomers
inferredcites →https://doi.org/10.1038/s41467-019-11144-6openalex-snapshot
Detecting topology freezing transition temperature of vitrimers by AIE luminogens
inferredcites →https://doi.org/10.1038/s41598-017-11485-6openalex-snapshot
Recyclable Polydimethylsiloxane Network Crosslinked by Dynamic Transesterification Reaction
inferredcites →https://doi.org/10.1039/c1sc00260kopenalex-snapshot
A mechanistic study of Lewis acid-catalyzed covalent organic framework formation
inferredcites →https://doi.org/10.1039/c3cs60046gopenalex-snapshot
Covalent adaptable networks: smart, reconfigurable and responsive network systems
inferredcites →https://doi.org/10.1039/c4sc00543kopenalex-snapshot
Carbon nanotube–vitrimer composite for facile and efficient photo-welding of epoxy
inferredcites →https://doi.org/10.1039/c5gc00754bopenalex-snapshot
Crack healing and reclaiming of vulcanized rubber by triggering the rearrangement of inherent sulfur crosslinked networks
inferredcites →https://doi.org/10.1039/c5py00459dopenalex-snapshot
Chemically crosslinked yet reprocessable epoxidized natural rubber via thermo-activated disulfide rearrangements
inferredcites →https://doi.org/10.1039/c7cs00276aopenalex-snapshot
Progress in bio-inspired sacrificial bonds in artificial polymeric materials
inferredcites →https://doi.org/10.1039/c8gc02932fopenalex-snapshot
A real recycling loop of sulfur-cured rubber through transalkylation exchange of C–S bonds
inferredcites →https://doi.org/10.1039/c8ta09866bopenalex-snapshot
Malleable organic/inorganic thermosetting hybrids enabled by exchangeable silyl ether interfaces
inferredcites →https://doi.org/10.1039/c9py01260eopenalex-snapshot
Dynamic covalent chemistry in polymer networks: a mechanistic perspective
inferredcites →https://doi.org/10.1039/c9ta10909aopenalex-snapshot
Biomimetic design of elastomeric vitrimers with unparalleled mechanical properties, improved creep resistance and retained malleability by metal–ligand coordination
inferredcites →https://doi.org/10.1063/1.1747424openalex-snapshot
Statistical Mechanics of Swelling of Network Structures
inferredcites →https://doi.org/10.1126/science.1212648openalex-snapshot
Silica-Like Malleable Materials from Permanent Organic Networks
inferredcites →https://doi.org/10.5254/rct.12.87973openalex-snapshot
RUBBER RECYCLING: CHEMISTRY, PROCESSING, AND APPLICATIONS

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

inferred← citeshttps://doi.org/10.2139/ssrn.4500232openalex-extracted
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inferred← citeshttps://doi.org/10.1002/adfm.202108431openalex-snapshot
Complementary Dynamic Chemistries for Multifunctional Polymeric Materials
inferred← citeshttps://doi.org/10.1002/adma.202512968openalex-snapshot
Sustainable Liquid Metal Composites for Soft Electronics and E‐Waste Reduction
inferred← citeshttps://doi.org/10.1002/app.51182openalex-snapshot
Based on transalkylation reaction the rearrangeable conventional sulfur network facile design for vulcanized diolefin elastomers
inferred← citeshttps://doi.org/10.1002/chem.202202058openalex-snapshot
Coordination Adaptable Networks: Zirconium(IV) Carboxylates
inferred← citeshttps://doi.org/10.1002/macp.202400461openalex-snapshot
Research Progresses in Methods for Improving the Properties of Dynamic Covalent Polymer Networks
inferred← citeshttps://doi.org/10.1002/mame.202200067openalex-snapshot
Bioinspired Rubber Composites with Mechanical Robustness, Recyclability, and Shape Memory Properties
inferred← citeshttps://doi.org/10.1002/marc.202100432openalex-snapshot
Catalyst‐Free Vitrimer Cross‐Linked by Biomass‐Derived Compounds with Mechanical Robustness, Reprocessability, and Multishape Memory Effects
inferred← citeshttps://doi.org/10.1002/marc.202500076openalex-snapshot
Thioketones as a Simple Route Toward Thioester‐Based Materials
inferred← citeshttps://doi.org/10.1002/pen.26230openalex-snapshot
Fabricated coordinate and ionic bonds in chemically cross‐linked ethylene acrylic elastomer for high‐performing elastomers
inferred← citeshttps://doi.org/10.1002/pen.70667openalex-snapshot
Recyclable Epoxidized EPDM ‐ XNBR Elastomer Vitrimer and Optimization of Processing Strategy
inferred← citeshttps://doi.org/10.1002/pls2.10113openalex-snapshot
Covalent adaptable network offers “sustainable” closed‐loop circularity in epoxy vitrimers
inferred← citeshttps://doi.org/10.1002/pls2.10114openalex-snapshot
A designer Schiff based motif offered dual dynamic exchangeable bonds, faster curing and closed‐loop circularity in epoxy vitrimers
inferred← citeshttps://doi.org/10.1002/pol.20230431openalex-snapshot
A robust and efficiently reprocessable poly(dimethylsiloxane) elastomers enhanced by self‐catalysis Z n( II )‐ligand bonds and silyl ethers
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inferred← citeshttps://doi.org/10.1007/978-981-16-4667-6_4openalex-snapshot
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inferred← citeshttps://doi.org/10.1007/s00289-023-05116-6openalex-snapshot
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inferred← citeshttps://doi.org/10.1007/s10118-022-2674-8openalex-snapshot
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inferred← citeshttps://doi.org/10.1007/s10924-023-03048-wopenalex-snapshot
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inferred← citeshttps://doi.org/10.1007/s40843-021-1963-2openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.ccr.2025.217490openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.cej.2022.139130openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.cej.2025.161857openalex-snapshot
Reprocessable bio-based rubber with hierarchical hydrogen bonding: A sustainable solution for high strength, superior extensibility, and recyclability
inferred← citeshttps://doi.org/10.1016/j.cej.2026.181868openalex-snapshot
A tung oil-based dual-function modifier for high-performance epoxy vitrimers: Synergistic toughening via sacrificial bonds and in-situ catalysis for upcycling
inferred← citeshttps://doi.org/10.1016/j.compositesa.2024.108007openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.compscitech.2023.110382openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.compscitech.2025.111132openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.compstruct.2021.115071openalex-snapshot
Modified MXene-doped conductive organosilicon elastomer with high-stretchable, toughness, and self-healable for strain sensors
inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2022.111341openalex-snapshot
Room temperature Self-healable and extremely stretchable elastomer with improved mechanical Properties: Exploring a simplistic Metal-Ligand interaction
inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2023.111844openalex-snapshot
Dynamic chemistry: The next generation platform for various elastomers and their mechanical properties with self-healing performance
inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2023.112101openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.ijbiomac.2023.124681openalex-snapshot
Biobased epoxidized natural rubber/sodium carboxymethyl cellulose composites with enhanced strength and healing ability
inferred← citeshttps://doi.org/10.1016/j.indcrop.2021.113978openalex-snapshot
Catalyst-free self-healing fully bio-based vitrimers derived from tung oil: Strong mechanical properties, shape memory, and recyclability
inferred← citeshttps://doi.org/10.1016/j.matdes.2023.112057openalex-snapshot
A self-healing and energy-dissipating impact-hardening polymer based on a variety of reversible dynamic bonds
inferred← citeshttps://doi.org/10.1016/j.polymer.2020.123309openalex-snapshot
Unusual low temperature relaxation behavior of crosslinked acrylonitrile-butadiene co-polymer
inferred← citeshttps://doi.org/10.1016/j.polymer.2021.124114openalex-snapshot
Toughening polyisoprene rubber with sacrificial bonds: The interplay between molecular mobility, energy dissipation and strain-induced crystallization
inferred← citeshttps://doi.org/10.1016/j.polymer.2021.124373openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.polymer.2022.124626openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.polymer.2022.124710openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.polymer.2024.126775openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.polymer.2025.128570openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.polymer.2026.130042openalex-snapshot
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inferred← citeshttps://doi.org/10.1016/j.polymer.2026.130789openalex-snapshot
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inferred← citeshttps://doi.org/10.1021/acs.biomac.6c00126openalex-snapshot
Deformation-Induced Morphology Evolution of Protein-Lipid Aggregates and Its Relationship with Mechanical Properties of Vulcanized Natural Rubber
inferred← citeshttps://doi.org/10.1021/acs.iecr.2c00601openalex-snapshot
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inferred← citeshttps://doi.org/10.1021/acsapm.1c00667openalex-snapshot
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inferred← citeshttps://doi.org/10.1021/acsapm.2c00659openalex-snapshot
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inferred← citeshttps://doi.org/10.1021/acsomega.4c04264openalex-snapshot
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inferred← citeshttps://doi.org/10.1021/acssuschemeng.1c00033openalex-snapshot
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inferred← citeshttps://doi.org/10.1039/9781837675470-00107openalex-snapshot
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inferred← citeshttps://doi.org/10.1039/d2py00489eopenalex-snapshot
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inferred← citeshttps://doi.org/10.1039/d2py00991aopenalex-snapshot
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inferred← citeshttps://doi.org/10.1039/d3gc02799fopenalex-snapshot
Preparation of lignin-based vinylogous urethane vitrimer materials and their potential use as on-demand removable adhesives
inferred← citeshttps://doi.org/10.1039/d4ta06405dopenalex-snapshot
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inferred← citeshttps://doi.org/10.1080/15583724.2024.2405904openalex-snapshot
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inferred← citeshttps://doi.org/10.1122/8.0000473openalex-snapshot
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inferred← citeshttps://doi.org/10.2139/ssrn.5179080openalex-snapshot
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inferred← citeshttps://doi.org/10.2139/ssrn.5358736openalex-snapshot
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DYNAMIC REVERSIBLE NETWORKS AND DEVELOPMENT OF SELF-HEALING RUBBERS: A CRITICAL REVIEW
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