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Direct C(sp3)–H Acylation by Mechanistically Controlled Ni/Ir Photoredox Catalysis

https://doi.org/10.1021/acs.accounts.3c00252

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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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Direct Acylation of C(sp 3 )−H Bonds Enabled by Nickel and Photoredox Catalysis

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Nickel‐Catalyzed Activation of Acyl C−O Bonds of Methyl Esters

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Mild, Redox‐Neutral Formylation of Aryl Chlorides through the Photocatalytic Generation of Chlorine Radicals

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Ketones from Nickel‐Catalyzed Decarboxylative, Non‐Symmetric Cross‐Electrophile Coupling of Carboxylic Acid Esters

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Synergistic Activation of Amides and Hydrocarbons for Direct C(sp3)–H Acylation Enabled by Metallaphotoredox Catalysis

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Visible‐Light‐Induced Homolysis of Earth‐Abundant Metal‐Substrate Complexes: A Complementary Activation Strategy in Photoredox Catalysis

inferredcites →https://doi.org/10.1002/anie.202108987openalex-snapshot

Rapid and Direct Photocatalytic C(sp3)−H Acylation and Arylation in Flow

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Theoretical Mechanistic Study of C( sp 3 )−C( sp 2 ) Cross‐Coupling by Photoredox‐Mediated Iridium(III)/Nickel(II)/Quinuclidine Triple Catalysis

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Exploring Regioselective Bond Cleavage and Cross‐Coupling Reactions using a Low‐Valent Nickel Complex

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Twisted Amides: From Obscurity to Broadly Useful Transition‐Metal‐Catalyzed Reactions by N−C Amide Bond Activation

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The Nickel Age in Synthetic Dual Photocatalysis: A Bright Trip Toward Materials Science

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N‐Acyl‐Glutarimides: Privileged Scaffolds in Amide N–C Bond Cross‐Coupling

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Recent Progress in Fragmentation of Katritzky Salts Enabling Formation of C–C, C–B, and C–S Bonds

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Reaction of acyl chlorides with organometallic reagents: A banquet table of metals for ketone synthesis

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Organomanganese (II) reagents XIX. Acylation of organomanganese chlorides by carboxylic acid chlorides in THF: A clear improvement in the field of the preparation of ketones from organomanganese compounds

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Electrosynthesis of ketones from organic halides and anhydrides

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N-methoxy-n-methylamides as effective acylating agents

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Synthetic and Mechanistic Implications of Chlorine Photoelimination in Nickel/Photoredox C(sp 3 )–H Cross-Coupling

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The Development and Application of Two-Chamber Reactors and Carbon Monoxide Precursors for Safe Carbonylation Reactions

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Metallaphotoredox: The Merger of Photoredox and Transition Metal Catalysis

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Dual Catalysis Strategies in Photochemical Synthesis

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Halogen Photoelimination from Monomeric Nickel(III) Complexes Enabled by the Secondary Coordination Sphere

inferredcites →https://doi.org/10.1021/acs.orglett.0c00885openalex-snapshot

Nickel-Catalyzed Conversion of Amides to Carboxylic Acids

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Iron-Catalyzed Acylation of Polyfunctionalized Aryl- and Benzylzinc Halides with Acid Chlorides

inferredcites →https://doi.org/10.1021/acs.orglett.7b00989openalex-snapshot

Synergistic Visible-Light Photoredox/Nickel-Catalyzed Synthesis of Aliphatic Ketones via N–C Cleavage of Imides

inferredcites →https://doi.org/10.1021/acs.orglett.7b01552openalex-snapshot

Photocatalytic α-Acylation of Ethers

inferredcites →https://doi.org/10.1021/acs.orglett.8b00160openalex-snapshot

Synthetic Approach to Benzocyclobutenones Using Visible Light and a Phosphonate Auxiliary

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Divergent Acyl and Decarbonylative Liebeskind–Srogl Cross-Coupling of Thioesters by Cu-Cofactor and Pd–NHC (NHC = N-Heterocyclic Carbene) Catalysis

inferredcites →https://doi.org/10.1021/acscatal.6b00793openalex-snapshot

Nickel-Catalyzed Alkylation of Amide Derivatives

inferredcites →https://doi.org/10.1021/acscatal.9b00375openalex-snapshot

How Does Iridium(III) Photocatalyst Regulate Nickel(II) Catalyst in Metallaphotoredox-Catalyzed C–S Cross-Coupling? Theoretical and Experimental Insights

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Recent Advances in Pyridinium Salts as Radical Reservoirs in Organic Synthesis

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Chemistry of Acyl Radicals

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Oxygen-Induced Ligand Dehydrogenation of a Planar Bis-μ-Chloronickel(I) Dimer Featuring an NHC Ligand

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Trap-Free Halogen Photoelimination from Mononuclear Ni(III) Complexes

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Group-Transfer Reactions of Ni(II)−Ni(II) Bridging Imido Complexes. Catalytic Formation of Carbodiimides and Isocyanates via Nitrene Transfer from Organoazides

inferredcites →https://doi.org/10.1038/nature14615openalex-snapshot

Conversion of amides to esters by the nickel-catalysed activation of amide C–N bonds

inferredcites →https://doi.org/10.1038/nchem.2388openalex-snapshot

Nickel-catalysed Suzuki–Miyaura coupling of amides

inferredcites →https://doi.org/10.1038/s41467-021-23887-2openalex-snapshot

Asymmetric benzylic C(sp3)−H acylation via dual nickel and photoredox catalysis

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Mild ketone formation via Ni-catalyzed reductive coupling of unactivated alkyl halides with acid anhydrides

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Photoredox mediated nickel catalyzed C(sp 3 )–H thiocarbonylation of ethers

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Decarbonylative cross-coupling of amides

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Photoinduced deaminative strategies: Katritzky salts as alkyl radical precursors

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Synthesis of unsymmetrical ketones by applying visible-light benzophenone/nickel dual catalysis for direct benzylic acylation

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Recent advances in the synthesis of α-amino ketones

inferredcites →https://doi.org/10.1039/d0sc00712aopenalex-snapshot

Recent advances in photoredox and nickel dual-catalyzed cascade reactions: pushing the boundaries of complexity

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Palladium catalyzed carbonylative generation of potent, pyridine-based acylating electrophiles for the functionalization of arenes to ketones

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Merging Transition-Metal Catalysis with Photoredox Catalysis: An Environmentally Friendly Strategy for C–H Functionalization

inferredcites →https://doi.org/10.1055/s-0037-1610329openalex-snapshot

Acyl Radical Chemistry via Visible-Light Photoredox Catalysis

inferredcites →https://doi.org/10.3390/catal9010053openalex-snapshot

Recent Advances in Acyl Suzuki Cross-Coupling

inferredcites →https://doi.org/10.3762/bjoc.17.143openalex-snapshot

Photoredox catalysis in nickel-catalyzed C–H functionalization

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

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Photoredox‐Catalyzed Minisci‐Type Acylation of Heterocyclic C−H Bonds with Amino Acid‐Tethered Dihydropyridines

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Cooperative NHC and Photoredox Catalyzed Radical Aminoacylation of Alkenes to Tetrahydropyridazines

inferred← citeshttps://doi.org/10.1002/ejoc.202500937openalex-snapshot

Cyclization of Carbonyl Electrophiles via Dual HAT/Photoredox‐Catalyzed Reductive Radical‐Polar Crossover

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Recent advances in palladium-catalysed organic synthesis using water as solvent

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Earth-abundant Ni(II)-based molecular photoredox catalysts: Emerging platform for sustainable cross coupling reactions

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Ir-catalyzed photoredox cascade radical annulation reactions toward phosphinimides bearing quaternary carbon center at room temperature

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Visible light-induced synergistic photoredox/palladium catalysis for decarboxylative benzoylation of aryl pyridines: Efficient access to pyridine-substituted aryl ketones at ambient temperature

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Nickel-Catalyzed Functionalization Reactions Involving C–H Bond Activation via an Amidate-Promoted Strategy and Its Extension to the Activation of C–F, C–O, C–S, and C–CN Bonds

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Strategies and Mechanisms of First-Row Transition Metal-Regulated Radical C–H Functionalization

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The Subtle Mechanism of Nickel-Photocatalyzed C(sp3)–H Cross-Coupling

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Synthesis of Aryl Phosphines via Pd/C-Catalyzed Decarbonylation of Acylphosphines

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The Merger of Halogen Atom Transfer (XAT) and Energy Transfer Catalysis (EnT) for the Modular 1,2-Iminylalkylation of Diazenes

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Visible-Light-Promoted [4π + 2σ] Annulation of Dienes and Alkylamines via Dual Inert C(sp3)–H Bond Activation

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Decatungstate-Photocatalyzed Transformations of 2-Bromo-3,3,3-trifluoropropene for Selective Synthesis of Z / E -β-CF 3 -Enones

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Visible-Light-Induced ortho-Quinone Methides Formation in Situ Using ortho-Alkylarenols as Precursors for Tandem [4 + 2] Cycloaddition Reaction

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Triplet Energy Transfer as a Handle to Tune 1,2-Dialkyldiazene Fragmentation in Radical C(sp 3 )–C(sp 2 ) Cross-Coupling

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Photoexcited Cyanohydrin Anions Enable Redox-Neutral Acylarylation of Olefins

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Radical Allylation of Aldehydes with Allenes by Photoredox Cobalt and Chromium Dual Catalysis

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