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Elucidating the Solvation Structure and Dynamics of Lithium Polysulfides Resulting from Competitive Salt and Solvent Interactions

https://doi.org/10.1021/acs.chemmater.7b00068
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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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On the Way Toward Understanding Solution Chemistry of Lithium Polysulfides for High Energy Li–S Redox Flow Batteries
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Characterization of Polysulfide Radicals Present in an Ether‐Based Electrolyte of a Lithium–Sulfur Battery During Initial Discharge Using In Situ X‐Ray Absorption Spectroscopy Experiments and First‐Principles Calculations
inferredcites →https://doi.org/10.1002/aenm.201600160openalex-snapshot
Restricting the Solubility of Polysulfides in Li‐S Batteries Via Electrolyte Salt Selection
inferredcites →https://doi.org/10.1016/j.jpowsour.2012.12.102openalex-snapshot
Liquid electrolyte lithium/sulfur battery: Fundamental chemistry, problems, and solutions
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A review of electrolytes for lithium–sulphur batteries
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Nanocomposite polymer electrolyte for rechargeable magnesium batteries
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A quantum-chemical study on the discharge reaction mechanism of lithium-sulfur batteries
inferredcites →https://doi.org/10.1021/acs.jpcc.5b12538openalex-snapshot
Long-Chain Polysulfide Retention at the Cathode of Li–S Batteries
inferredcites →https://doi.org/10.1021/acsenergylett.6b00194openalex-snapshot
Sparingly Solvating Electrolytes for High Energy Density Lithium–Sulfur Batteries
inferredcites →https://doi.org/10.1021/ar300179vopenalex-snapshot
Challenges and Prospects of Lithium–Sulfur Batteries
inferredcites →https://doi.org/10.1021/jp5015466openalex-snapshot
Toward a Molecular Understanding of Energetics in Li–S Batteries Using Nonaqueous Electrolytes: A High-Level Quantum Chemical Study
inferredcites →https://doi.org/10.1021/jp510644kopenalex-snapshot
Effect of Organic Solvents on Li + Ion Solvation and Transport in Ionic Liquid Electrolytes: A Molecular Dynamics Simulation Study
inferredcites →https://doi.org/10.1021/jz500260sopenalex-snapshot
X-ray Absorption Spectra of Dissolved Polysulfides in Lithium–Sulfur Batteries from First-Principles
inferredcites →https://doi.org/10.1038/nmat3191openalex-snapshot
Li–O2 and Li–S batteries with high energy storage
inferredcites →https://doi.org/10.1039/c2cc36986aopenalex-snapshot
Polysulfide dissolution control: the common ion effect
inferredcites →https://doi.org/10.1039/c4cp00889hopenalex-snapshot
Molecular structure and stability of dissolved lithium polysulfide species
inferredcites →https://doi.org/10.1039/c4cp05316hopenalex-snapshot
X-ray spectroscopy as a probe for lithium polysulfide radicals
inferredcites →https://doi.org/10.1039/c5cp02781kopenalex-snapshot
Evidence for the existence of Li 2 S 2 clusters in lithium–sulfur batteries: ab initio Raman spectroscopy simulation
inferredcites →https://doi.org/10.1063/1.4894481openalex-snapshot
Diffusional motion of redox centers in carbonate electrolytes
inferredcites →https://doi.org/10.1149/2.045308jesopenalex-snapshot
In-Situ Raman Investigation of Polysulfide Formation in Li-S Cells

What points at this work

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inferred← citeshttps://doi.org/10.1021/acsami.4c21057openalex-snapshot
Defect-Induced Li-Ion Trapping and Hopping in a Grain Boundary-Engineered Li1.3Al0.3Ti1.7(PO4)3 Solid-State Electrolyte
inferred← citeshttps://doi.org/10.1021/acsami.4c22330openalex-snapshot
Slurry Additive Approach Enables a Mechanically Robust Binder for Silicon–Carbon Anodes in Lithium-Ion Batteries
inferred← citeshttps://doi.org/10.1021/acsami.5c25456openalex-snapshot
Catalyzing the Polysulfide Redox Chemistry in Lithium–Sulfur Batteries: Mechanisms Bridging First-Principles Theory and Experimental Characterization
inferred← citeshttps://doi.org/10.1021/acsapm.3c00379openalex-snapshot
Solvation Structure of Conjugated Organosulfur Polymers for Lithium–Sulfur Battery Cathodes
inferred← citeshttps://doi.org/10.1021/acscentsci.9b00406openalex-snapshot
Ion Transport and the True Transference Number in Nonaqueous Polyelectrolyte Solutions for Lithium Ion Batteries
inferred← citeshttps://doi.org/10.1021/acsenergylett.0c00148openalex-snapshot
Electrolyte Engineering Enables High Stability and Capacity Alloying Anodes for Sodium and Potassium Ion Batteries
inferred← citeshttps://doi.org/10.1021/acsenergylett.0c02461openalex-snapshot
Evoking High-Donor-Number-Assisted and Organosulfur-Mediated Conversion in Lithium–Sulfur Batteries
inferred← citeshttps://doi.org/10.1021/acsenergylett.5c00974openalex-snapshot
Practical Lithium–Sulfur Batteries Enabled by a Six-Membered Cyclic Urea Solvent
inferred← citeshttps://doi.org/10.1021/acsenergylett.6c00391openalex-snapshot
Role of the Electrolyte Concentration in Polysulfide Shuttle and Electrochemical Performance of Lithium–Sulfur Batteries
inferred← citeshttps://doi.org/10.1021/acsmacrolett.4c00824openalex-snapshot
Salt Effects on Ionic Conductivity Mechanisms in Ethylene Carbonate Electrolytes: Interplay of Viscosity and Ion–Ion Relaxations
inferred← citeshttps://doi.org/10.1021/acsnano.1c05875openalex-snapshot
All-Liquid-Phase Reaction Mechanism Enabling Cryogenic Li–S Batteries
inferred← citeshttps://doi.org/10.1021/acsnano.2c06362openalex-snapshot
A High-Performance Quasi-Solid-State Aqueous Zinc–Dual Halogen Battery
inferred← citeshttps://doi.org/10.1021/acsomega.6c01811openalex-snapshot
Accelerating Electrolyte Discovery Using Generative Models and Molecular Dynamics Simulations
inferred← citeshttps://doi.org/10.1021/acssuschemeng.6c04616openalex-snapshot
Unlocking the Capacity of Li−S Batteries via a Solvation-Mediated Trade-Off between Anode Stability and Cathode Kinetics
inferred← citeshttps://doi.org/10.1021/jacs.0c10587openalex-snapshot
Correlating Li-Ion Solvation Structures and Electrode Potential Temperature Coefficients
inferred← citeshttps://doi.org/10.1021/jacs.8b02057openalex-snapshot
Interfacial Mechanism in Lithium–Sulfur Batteries: How Salts Mediate the Structure Evolution and Dynamics
inferred← citeshttps://doi.org/10.1021/jacs.9b11056openalex-snapshot
A New Class of Ionically Conducting Fluorinated Ether Electrolytes with High Electrochemical Stability
inferred← citeshttps://doi.org/10.1038/s41467-018-07975-4openalex-snapshot
Achieving three-dimensional lithium sulfide growth in lithium-sulfur batteries using high-donor-number anions
inferred← citeshttps://doi.org/10.1038/s41467-021-27861-wopenalex-snapshot
Multifactorial engineering of biomimetic membranes for batteries with multiple high-performance parameters
inferred← citeshttps://doi.org/10.1038/s41467-023-37995-8openalex-snapshot
Exploiting nonaqueous self-stratified electrolyte systems toward large-scale energy storage
inferred← citeshttps://doi.org/10.1038/s41560-017-0005-zopenalex-snapshot
Non-encapsulation approach for high-performance Li–S batteries through controlled nucleation and growth
inferred← citeshttps://doi.org/10.1038/s41560-019-0351-0openalex-snapshot
Intercalation-conversion hybrid cathodes enabling Li–S full-cell architectures with jointly superior gravimetric and volumetric energy densities
inferred← citeshttps://doi.org/10.1038/s41565-019-0624-6openalex-snapshot
Electrochemical generation of liquid and solid sulfur on two-dimensional layered materials with distinct areal capacities
inferred← citeshttps://doi.org/10.1038/s41586-023-06918-4openalex-snapshot
Establishing reaction networks in the 16-electron sulfur reduction reaction
inferred← citeshttps://doi.org/10.1038/s43588-022-00200-9openalex-snapshot
An automated framework for high-throughput predictions of NMR chemical shifts within liquid solutions
inferred← citeshttps://doi.org/10.1038/s44359-026-00147-4openalex-snapshot
Semi-liquid lithium−sulfur batteries for large-scale energy storage
inferred← citeshttps://doi.org/10.1039/c9ta11079hopenalex-snapshot
Ultrathin bismuth nanosheets as an efficient polysulfide catalyst for high performance lithium–sulfur batteries
inferred← citeshttps://doi.org/10.1039/c9ta14003dopenalex-snapshot
An in situ encapsulation approach for polysulfide retention in lithium–sulfur batteries
inferred← citeshttps://doi.org/10.1039/d1me00185jopenalex-snapshot
Lithium polysulfide conformer analysis in ether-based solvents for Li–S batteries
inferred← citeshttps://doi.org/10.1039/d1sc04265copenalex-snapshot
The solvation structure, transport properties and reduction behavior of carbonate-based electrolytes of lithium-ion batteries
inferred← citeshttps://doi.org/10.1039/d1ta02779dopenalex-snapshot
Unifying the clustering kinetics of lithium polysulfides with the nucleation behavior of Li 2 S in lithium–sulfur batteries
inferred← citeshttps://doi.org/10.1039/d2cp02301fopenalex-snapshot
Distinct effects of zwitterionic molecules on ionic solvation in (ethylene oxide) 10 : a molecular dynamics simulation study
inferred← citeshttps://doi.org/10.1039/d2ta07832eopenalex-snapshot
Inspired by the Cu-driven conversion reaction: how anionic properties dictate the electrochemical performance of vanadium sulfide
inferred← citeshttps://doi.org/10.1039/d2ta08404jopenalex-snapshot
A comparative analysis of the influence of hydrofluoroethers as diluents on solvation structure and electrochemical performance in non-flammable electrolytes
inferred← citeshttps://doi.org/10.1039/d3ee04183bopenalex-snapshot
Interface engineering toward stable lithium–sulfur batteries
inferred← citeshttps://doi.org/10.1039/d4cp03352copenalex-snapshot
Diffusion and thermodynamic properties of lithium polysulfides in different solvents: a molecular dynamics approach
inferred← citeshttps://doi.org/10.1039/d4cs00318gopenalex-snapshot
Polysulfide chemistry in metal–sulfur batteries
inferred← citeshttps://doi.org/10.1039/d4ee05789aopenalex-snapshot
Small modification, striking improvement: super-fast charging over a wide temperature range by simply replacing n -propyl acetate with isopropyl acetate
inferred← citeshttps://doi.org/10.1039/d5ta05082kopenalex-snapshot
The mechanism of Li + transport in an ether-based electrolyte
inferred← citeshttps://doi.org/10.1039/d5ta08753hopenalex-snapshot
The mechanism of Li-ion transport in carbonate-based electrolytes
inferred← citeshttps://doi.org/10.1039/d6cp02008aopenalex-snapshot
Fluorinated EC analogues as co-solvents in EMC-based electrolytes for Li-ion batteries: a computational study
inferred← citeshttps://doi.org/10.1063/5.0059246openalex-snapshot
Liquid state properties of SEI components in dimethoxyethane
inferred← citeshttps://doi.org/10.1063/5.0102937openalex-snapshot
The effects of polarization on the rotational diffusion of ions in organic ionic plastic crystals
inferred← citeshttps://doi.org/10.1073/pnas.2316564121openalex-snapshot
The electrochemistry of stable sulfur isotopes versus lithium
inferred← citeshttps://doi.org/10.1080/17415993.2022.2126318openalex-snapshot
Redox induced electron transfer in lithium polysulfide – A DFT study
inferred← citeshttps://doi.org/10.1088/2515-7655/ac4ac3openalex-snapshot
Perspectives on manufacturing simulations of Li-S battery cathodes
inferred← citeshttps://doi.org/10.1140/epje/s10189-023-00365-9openalex-snapshot
Anomalous diffusion of lithium-anion clusters in ionic liquids
inferred← citeshttps://doi.org/10.1149/2.0161902jesopenalex-snapshot
Electrolyte Concentration Effect on Sulfur Utilization of Li-S Batteries
inferred← citeshttps://doi.org/10.21203/rs.3.rs-4364688/v1openalex-snapshot
Knowledge-driven design of fluorinated ether electrolytes via a multi-model approach
inferred← citeshttps://doi.org/10.26434/chemrxiv-2024-fvgdqopenalex-snapshot
Mixed1-ethyl-3-methylimidazoliumbis(trifluoromethylsulfonyl)imide/lithium bis(fluoromethylsulfonyl)imide based ionic liquid and carbonate co-solvents for Li-ion battery applications– analysis of transport properties using MD simulation
inferred← citeshttps://doi.org/10.3866/pku.whxb202303061openalex-snapshot
Sulfur Cathode Electrocatalysis in Lithium-Sulfur Batteries: A Comprehensive Understanding
inferred← citeshttps://doi.org/10.54227/mlab.20220031openalex-snapshot
Ab-Initio Simulations Accelerate the Development of High-Performance Lithium-Sulfur Batteries
inferred← citeshttps://doi.org/10.7302/2749openalex-snapshot
Bioinspired Nanocomposites for Structural Energy Storage
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