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Intergranular Cracking as a Major Cause of Long-Term Capacity Fading of Layered Cathodes

https://doi.org/10.1021/acs.nanolett.7b00379
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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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Performance of LiNiCoO2 materials for advanced lithium-ion batteries
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inferred← citeshttps://doi.org/10.1016/j.cej.2022.134745openalex-snapshot
Bifunctional nitrile-borate based electrolyte additive enables excellent electrochemical stability of lithium metal batteries with single-crystal Ni-rich cathode at 4.7 V
inferred← citeshttps://doi.org/10.1016/j.cej.2022.135276openalex-snapshot
Hydrophobic surface coating against chemical environmental instability for Ni-rich layered oxide cathode materials
inferred← citeshttps://doi.org/10.1016/j.cej.2022.136825openalex-snapshot
In situ co-doping strategy for achieving long-term cycle stability of single-crystal Ni-rich cathodes at high voltage
inferred← citeshttps://doi.org/10.1016/j.cej.2023.148223openalex-snapshot
Engineering lithium nickel cobalt manganese oxides cathodes: A computational and experimental approach to bridging gaps
inferred← citeshttps://doi.org/10.1016/j.cej.2024.148905openalex-snapshot
Selenium treatment towards enhanced cyclic stability for single-crystal Ni-rich cathode at ultra-high voltage of 4.7 V
inferred← citeshttps://doi.org/10.1016/j.cej.2024.149575openalex-snapshot
Surface-enriched Co engineering promoting electronic conductivity for single-crystalline Ni-based layered oxide cathodes
inferred← citeshttps://doi.org/10.1016/j.cej.2024.150667openalex-snapshot
Efficient trapping of lithium-ions by branched amine for stable lithium metal anodes
inferred← citeshttps://doi.org/10.1016/j.cej.2024.152078openalex-snapshot
Revealing the origin of enhanced structural stability for nickel-rich LiNi0.83Co0.11Mn0.06O2 cathodes in situ modified with multifunctional polysiloxane
inferred← citeshttps://doi.org/10.1016/j.cej.2024.153603openalex-snapshot
Enhancing interfacial compatibility and ionic transportation kinetics in lithium-rich manganese oxide via magnetron sputtering conformal coating with amorphous LiPON
inferred← citeshttps://doi.org/10.1016/j.cej.2024.158260openalex-snapshot
Impact of low temperature exposure on lithium-ion batteries: A multi-scale study of performance degradation, predictive signals and underlying mechanisms
inferred← citeshttps://doi.org/10.1016/j.cej.2025.159376openalex-snapshot
Water-based Pickering emulsion for concurrent washing and CNT coating of high-nickel layered lithium-ion cathodes
inferred← citeshttps://doi.org/10.1016/j.cej.2025.163974openalex-snapshot
Progress and challenges of zinc ion capacitors: From basic principles to performance optimization strategies
inferred← citeshttps://doi.org/10.1016/j.cej.2025.171202openalex-snapshot
Rejuvenating humidity-aged ultra-high nickel cathodes by targeted sodium doping
inferred← citeshttps://doi.org/10.1016/j.ceramint.2019.06.261openalex-snapshot
Surface modification of Li rich Li1.2Mn0.54Ni0.13Co0.13O2 cathode particles
inferred← citeshttps://doi.org/10.1016/j.ceramint.2021.01.055openalex-snapshot
Effects of Al doping on the electrochemical performances of LiNi0.83Co0.12Mn0.05O2 prepared by coprecipitation
inferred← citeshttps://doi.org/10.1016/j.chempr.2023.09.007openalex-snapshot
Accelerating Li-based battery design by computationally engineering materials
inferred← citeshttps://doi.org/10.1016/j.cjche.2021.04.001openalex-snapshot
Tungsten and phosphate polyanion co-doping of Ni-ultrahigh cathodes greatly enhancing crystal structure and interface stability
inferred← citeshttps://doi.org/10.1016/j.commatsci.2023.112186openalex-snapshot
Data-driven multiscale simulation of solid-state batteries via machine learning
inferred← citeshttps://doi.org/10.1016/j.crsus.2025.100552openalex-snapshot
Upgrading polycrystalline battery cathodes to single-crystal NMC622 via morphology-controlled recycling
inferred← citeshttps://doi.org/10.1016/j.electacta.2017.12.176openalex-snapshot
Cathode materials with cross-stack structures for suppressing intergranular cracking and high-performance lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.electacta.2019.134587openalex-snapshot
Tailoring structure of Ni-rich layered cathode enable robust calendar life and ultrahigh rate capability for lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.electacta.2020.137358openalex-snapshot
The effects of ambient storage conditions on the structural and electrochemical properties of NMC-811 cathodes for Li-ion batteries
inferred← citeshttps://doi.org/10.1016/j.electacta.2021.138124openalex-snapshot
One-step bulk and surface co-modification of LiNi0.8Co0.15Al0.05O2 cathode material towards excellent long-term cyclability
inferred← citeshttps://doi.org/10.1016/j.electacta.2021.139417openalex-snapshot
Understanding the combined effect of Ca doping and phosphate coating on Ni-rich LiNi0.91Co0.06Mn0.03O2 cathode material for Li-ion batteries
inferred← citeshttps://doi.org/10.1016/j.electacta.2024.143790openalex-snapshot
Consequences of plane-strain and plane-stress assumptions in fully coupled chemo-mechanical Li-ion battery models
inferred← citeshttps://doi.org/10.1016/j.electacta.2024.145223openalex-snapshot
Chemo-mechanical instabilities in lithium cobalt oxide at higher state-of-charge in Li-Ion batteries
inferred← citeshttps://doi.org/10.1016/j.electacta.2025.147189openalex-snapshot
Quantification and modeling framework of mechanical-electrochemical degradation in Ni-Rich layered cathode
inferred← citeshttps://doi.org/10.1016/j.electacta.2026.149351openalex-snapshot
Synergistic enhancement of structural stability and electrochemical performance in Ni-rich LiNi0.8Mn0.1Co0.1O2 cathode materials via Na+/Al3+ co-doping
inferred← citeshttps://doi.org/10.1016/j.electacta.2026.149639openalex-snapshot
Dual-layer-porous-structured Ni-rich cathodes with high long cycling stability for lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.eml.2026.102452openalex-snapshot
Effects of electrolyte infiltration on the cracking of active materials in lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.energy.2025.135553openalex-snapshot
Extreme fast charging algorithm for lithium-ion batteries with precision lithium plating regulation for degradation reduction
inferred← citeshttps://doi.org/10.1016/j.engfracmech.2024.110370openalex-snapshot
Microstructure impact on chemo-mechanical fracture of polycrystalline lithium-ion battery cathode materials
inferred← citeshttps://doi.org/10.1016/j.engfracmech.2024.110647openalex-snapshot
Assessment of inter- and intra-granular fracture behaviors of polycrystalline LiNixCoyMn1-x-yO2 particles during a charging process
inferred← citeshttps://doi.org/10.1016/j.engfracmech.2025.111389openalex-snapshot
Impact of grain boundaries on the fracture behavior of polycrystalline electrode materials: a chemo-mechanical phase field model
inferred← citeshttps://doi.org/10.1016/j.engfracmech.2026.112036openalex-snapshot
Electrolyte infiltration effects on the cracking of polycrystalline NCM cathodes
inferred← citeshttps://doi.org/10.1016/j.engfracmech.2026.112390openalex-snapshot
Chemo-mechanical degradation of secondary particles in lithium-ion battery electrodes based on statistical and homogenization methods
inferred← citeshttps://doi.org/10.1016/j.engfracmech.2026.112481openalex-snapshot
3D electrochemo-mechanical modeling of electrolyte infiltration–fracture evolution in polycrystalline NCM particles
inferred← citeshttps://doi.org/10.1016/j.ensm.2020.01.027openalex-snapshot
Single-crystal nickel-rich layered-oxide battery cathode materials: synthesis, electrochemistry, and intra-granular fracture
inferred← citeshttps://doi.org/10.1016/j.ensm.2020.12.018openalex-snapshot
Interface cation migration kinetics induced oxygen release heterogeneity in layered lithium cathodes
inferred← citeshttps://doi.org/10.1016/j.ensm.2020.12.026openalex-snapshot
Microstructure boosting the cycling stability of LiNi0.6Co0.2Mn0.2O2 cathode through Zr-based dual modification
inferred← citeshttps://doi.org/10.1016/j.ensm.2021.07.001openalex-snapshot
Extended cycle life implications of fast charging for lithium-ion battery cathode
inferred← citeshttps://doi.org/10.1016/j.ensm.2022.06.004openalex-snapshot
π-type orbital hybridization and reactive oxygen quenching induced by Se-doping for Li-rich Mn-based oxide cathode
inferred← citeshttps://doi.org/10.1016/j.ensm.2022.08.010openalex-snapshot
Effect of particle size on thermodynamics and lithium ion transport in electrodes made of Ti2Nb2O9 microparticles or nanoparticles
inferred← citeshttps://doi.org/10.1016/j.ensm.2022.08.011openalex-snapshot
Nanotomographic observation and statistical analysis of overcharging induced cracks in LiCoO2 single crystalline particles
inferred← citeshttps://doi.org/10.1016/j.ensm.2022.11.019openalex-snapshot
Revealing the surface-to-bulk degradation mechanism of nickel-rich cathode in sulfide all-solid-state batteries
inferred← citeshttps://doi.org/10.1016/j.ensm.2023.02.003openalex-snapshot
A comprehensive review of foreign-ion doping and recent achievements for nickel-rich cathode materials
inferred← citeshttps://doi.org/10.1016/j.ensm.2023.102828openalex-snapshot
Microscopic investigation of crack and strain of LiCoO2 cathode cycled under high voltage
inferred← citeshttps://doi.org/10.1016/j.ensm.2023.102969openalex-snapshot
Ni-rich layered cathodes for lithium-ion batteries: From challenges to the future
inferred← citeshttps://doi.org/10.1016/j.ensm.2023.103049openalex-snapshot
Chemo-mechanical failure of solid composite cathodes accelerated by high-strain anodes in all-solid-state batteries
inferred← citeshttps://doi.org/10.1016/j.ensm.2024.103350openalex-snapshot
Improved interfacial contact and electrochemical performance of highly Ni-rich LiNixCoyMn1-x-yO2 (x>90%) cathode in all-solid-state lithium battery
inferred← citeshttps://doi.org/10.1016/j.ensm.2024.103440openalex-snapshot
Ni-rich cathode evolution: exploring electrochemical dynamics and strategic modifications to combat degradation
inferred← citeshttps://doi.org/10.1016/j.ensm.2024.103632openalex-snapshot
Unraveling the oxygen evolution in layered LiNiO2 with the role of Li/Ni disordering
inferred← citeshttps://doi.org/10.1016/j.ensm.2025.104014openalex-snapshot
Suppressing side reactions in spinel ZnMn2O4 for high-performance aqueous zinc-ion batteries
inferred← citeshttps://doi.org/10.1016/j.ensm.2026.104874openalex-snapshot
Decoding silicon-driven degradation: An adaptive fusion framework for robust battery electrode-level diagnostics
inferred← citeshttps://doi.org/10.1016/j.esci.2022.08.003openalex-snapshot
Precipitate-stabilized surface enabling high-performance Na0.67Ni0.33-xMn0.67ZnxO2 for sodium-ion battery
inferred← citeshttps://doi.org/10.1016/j.est.2022.106420openalex-snapshot
A microcrack propagation-based life prediction model for lithium-ion batteries with Ni-rich cathode materials
inferred← citeshttps://doi.org/10.1016/j.est.2024.110821openalex-snapshot
Dual-modified surface encapsulation strategy for elevating rate performance and cycling stability of Ni-rich NCM811 cathode
inferred← citeshttps://doi.org/10.1016/j.est.2024.114823openalex-snapshot
Enhanced performance of lithium-ion battery cathodes using a composite conductive network of CNTs, GQDs, and GNRs embedded in Li₁.₂Mn₀.₅₄Ni₀.₁₃Co₀.₁₃O₂ (LMNCO)
inferred← citeshttps://doi.org/10.1016/j.est.2025.117148openalex-snapshot
A dual-coating strategy based on primary and secondary particle structures of Li-rich Mn-based materials
inferred← citeshttps://doi.org/10.1016/j.est.2025.117813openalex-snapshot
Extracting health indicators from a single cycle of data based on the aging mechanism to accurately predict the knee point and remaining useful life of spent lithium-ion battery
inferred← citeshttps://doi.org/10.1016/j.est.2025.120247openalex-snapshot
In situ stress monitoring unravels particle-scale microstructural evolution in aging LiFePO4/graphite batteries
inferred← citeshttps://doi.org/10.1016/j.etran.2026.100637openalex-snapshot
A scalable multi-source aging coupling framework for high-fidelity electrochemical and thermal modeling of lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.ijmecsci.2019.02.042openalex-snapshot
Simulation of crack behavior of secondary particles in Li-ion battery electrodes during lithiation/de-lithiation cycles
inferred← citeshttps://doi.org/10.1016/j.ijmecsci.2025.111124openalex-snapshot
Unraveling the mechanism of non-monotonic C-rate-dependent electrode particle fracture
inferred← citeshttps://doi.org/10.1016/j.ijplas.2019.11.015openalex-snapshot
Coupled chemo-mechanical modeling of fracture in polycrystalline cathode for lithium-ion battery
inferred← citeshttps://doi.org/10.1016/j.ijsolstr.2021.111098openalex-snapshot
Strain gradient enhanced chemo-mechanical modeling of fracture in cathode materials for lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.jallcom.2019.02.285openalex-snapshot
Flux growth and enhanced electrochemical properties of LiNi0.5Co0.2Mn0.3O2 cathode material by excess lithium carbonate for lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.jallcom.2019.153048openalex-snapshot
A review on doping/coating of nickel-rich cathode materials for lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.jallcom.2020.156773openalex-snapshot
Probing the morphology dependence, size preference and electron/ion conductance of manganese-based lithium transition-metal phosphate as cathode materials for high-performance lithium-ion battery
inferred← citeshttps://doi.org/10.1016/j.jallcom.2020.158325openalex-snapshot
Pretreated precursor to realize dual modification that improves the high voltage electrochemical performance of LiNi0.8Co0.1Mn0.1O2 cathode materials
inferred← citeshttps://doi.org/10.1016/j.jallcom.2021.158806openalex-snapshot
Tuning (003) interplanar space by boric acid co-sintering to enhance Li+ storage and transfer in Li(Ni0.8Co0.1Mn0.1)O2 cathode
inferred← citeshttps://doi.org/10.1016/j.jallcom.2022.164024openalex-snapshot
Heterostructured LCAO/LMNCO cathode material for high capacity lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.jallcom.2022.167637openalex-snapshot
Realizing excellent cycling stability of LiNi0.80Co0.15Al0.05O2 cathode at high cutoff voltage by Al(PO3)3 modification
inferred← citeshttps://doi.org/10.1016/j.jallcom.2023.170362openalex-snapshot
Molten salt synthesis of high quality 2D δ‑MnO2 nanosheets for advanced aqueous Zn/MnO2 batteries
inferred← citeshttps://doi.org/10.1016/j.jallcom.2023.173097openalex-snapshot
Elevating cycle stability of Ni-rich NCM811 cathode via single-crystallization integrating dual-modification strategy for lithium-ion batteries
inferred← citeshttps://doi.org/10.1016/j.jallcom.2025.179198openalex-snapshot
Aluminum/titanium bimetallic doping for boosting the high-voltage Li-storage performance of Co-free high nickel cathode
inferred← citeshttps://doi.org/10.1016/j.jcis.2021.03.038openalex-snapshot
Synergetic effect of high Ni ratio and low oxygen defect interface zone of single crystals on the capacity retention of lithium rich layered oxides
inferred← citeshttps://doi.org/10.1016/j.jcis.2022.04.075openalex-snapshot
Nanoscale interface engineering of inorganic Solid-State electrolytes for High-Performance alkali metal batteries
inferred← citeshttps://doi.org/10.1016/j.jcis.2023.09.058openalex-snapshot
A new high-valence cation pillar within the Li layer of compositionally optimized Ni-rich LiNi0.9Co0.1O2 with improved structural stability for Li-ion battery
inferred← citeshttps://doi.org/10.1016/j.jcis.2024.02.150openalex-snapshot
Boosting sodium-ion battery performance by anion doping in NASICON Na4MnCr(PO4)3 cathode
inferred← citeshttps://doi.org/10.1016/j.jechem.2018.06.007openalex-snapshot
In situ X-ray diffraction and thermal analysis of LiNi0.8Co0.15Al0.05O2 synthesized via co-precipitation method
inferred← citeshttps://doi.org/10.1016/j.jechem.2019.05.013openalex-snapshot
Understanding of performance degradation of LiNi0.80Co0.10Mn0.10O2 cathode material operating at high potentials
inferred← citeshttps://doi.org/10.1016/j.jechem.2019.09.011openalex-snapshot
Operando X-ray diffraction analysis of the degradation mechanisms of a spinel LiMn2O4 cathode in different voltage windows
inferred← citeshttps://doi.org/10.1016/j.jechem.2021.07.021openalex-snapshot
Monitoring the morphology evolution of LiNi0.8Mn0.1Co0.1O2 during high-temperature solid state synthesis via in situ SEM
inferred← citeshttps://doi.org/10.1016/j.jechem.2021.08.017openalex-snapshot
Inhomogeneous lithium-storage reaction triggering the inefficiency of all-solid-state batteries
inferred← citeshttps://doi.org/10.1016/j.jechem.2022.11.016openalex-snapshot
Unraveling the degradation mechanism of LiNi0.8Co0.1Mn0.1O2 at the high cut-off voltage for lithium ion batteries
inferred← citeshttps://doi.org/10.1016/j.jechem.2024.01.014openalex-snapshot
Residual alkali-evoked cross-linked polymer layer for anti-air-sensitivity LiNi0.89Co0.06Mn0.05O2 cathode
inferred← citeshttps://doi.org/10.1016/j.jechem.2024.06.012openalex-snapshot
Surface-to-bulk engineering with high-valence W6+ enabling stabilized single-crystal LiNi0.9Co0.05Mn0.05O2 cathode
inferred← citeshttps://doi.org/10.1016/j.jechem.2024.10.022openalex-snapshot
High-areal-capacity and long-life sulfide-based all-solid-state lithium battery achieved by regulating surface-to-bulk oxygen activity
inferred← citeshttps://doi.org/10.1016/j.jechem.2025.01.039openalex-snapshot
Synergistically dissipating the local strain and restraining lattice oxygen escape by fine-tuning of microstructure enabling Ni-rich cathodes with superior cyclabilities
inferred← citeshttps://doi.org/10.1016/j.jechem.2026.02.015openalex-snapshot
Potassium storage in 2D layered TMD anode: Unraveling structure-performance correlations via rational microstructure design
inferred← citeshttps://doi.org/10.1016/j.jelechem.2023.117991openalex-snapshot
Analysis of lithium diffusion and overpotential in lithium nickle cobalt aluminum oxide based lithium ion cells
inferred← citeshttps://doi.org/10.1016/j.jeurceramsoc.2018.05.007openalex-snapshot
Energetic design of grain boundary networks for toughening of nanocrystalline oxides
inferred← citeshttps://doi.org/10.1016/j.jiec.2026.10.011openalex-snapshot
Interfacial instability governs performance in nanomaterial-based batteries
inferred← citeshttps://doi.org/10.1016/j.jmps.2018.12.005openalex-snapshot
A consistently coupled multiscale mechanical–electrochemical battery model with particle interaction and its validation
inferred← citeshttps://doi.org/10.1016/j.jmps.2021.104612openalex-snapshot
A consistent framework for chemo-mechanical cohesive fracture and its application in solid-state batteries
inferred← citeshttps://doi.org/10.1016/j.jmps.2022.104839openalex-snapshot
Chemo-mechanical modeling of inter- and intra-granular fracture in heterogeneous cathode with polycrystalline particles for lithium-ion battery
inferred← citeshttps://doi.org/10.1016/j.jmps.2024.106013openalex-snapshot
A length-scale insensitive cohesive phase-field interface model: Application to concurrent bulk and interface fracture simulation in Lithium-ion battery materials
inferred← citeshttps://doi.org/10.1016/j.jmst.2020.02.080openalex-snapshot
Atomic-scale tuned interface of nickel-rich cathode for enhanced electrochemical performance in lithium-ion batteries
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