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Dehydration as a Universal Mechanism for Ion Selectivity in Graphene and Other Atomically Thin Pores

https://doi.org/10.1021/acs.nanolett.7b01399

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What this work says

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Applying Transition-State Theory to Explore Transport and Selectivity in Salt-Rejecting Membranes: A Critical Review

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Roles of Anion–Cation Coupling Transport and Dehydration-Induced Ion–Membrane Interaction in Precise Separation of Ions by Nanofiltration Membranes

inferred← citeshttps://doi.org/10.1021/acs.est.4c07510openalex-snapshot

The Hidden Role of the Dielectric Effect in Nanofiltration: A Novel Perspective to Unravel New Ion Separation Mechanisms

inferred← citeshttps://doi.org/10.1021/acs.est.5c04303openalex-snapshot

Role of Ion Dehydration in Ion–Ion Selectivity of Dense Membranes

inferred← citeshttps://doi.org/10.1021/acs.iecr.2c03252openalex-snapshot

Electric Field-Driven Ultraefficient Li+/Mg2+ Separation through Graphyne Membrane

inferred← citeshttps://doi.org/10.1021/acs.jpca.7b10554openalex-snapshot

Strategy for Modeling the Infrared Spectra of Ion-Containing Water Drops

inferred← citeshttps://doi.org/10.1021/acs.jpca.9b05140openalex-snapshot

Free Energies of Hydration for Metal Ions from Heats of Vaporization

inferred← citeshttps://doi.org/10.1021/acs.jpcb.1c03255openalex-snapshot

Field-Dependent Dehydration and Optimal Ionic Escape Paths for C2N Membranes

inferred← citeshttps://doi.org/10.1021/acs.jpcb.1c05255openalex-snapshot

Rectification Correlation between Water and Ions through Asymmetric Graphene Channels

inferred← citeshttps://doi.org/10.1021/acs.jpcb.8b01117openalex-snapshot

Selective Permeation through One-Atom-Thick Nanoporous Carbon Membranes: Theory Reveals Excellent Design Strategies!

inferred← citeshttps://doi.org/10.1021/acs.jpcb.9b09587openalex-snapshot

Reverse Translocation of Nucleotides through a Carbon Nanotube

inferred← citeshttps://doi.org/10.1021/acs.jpcc.0c03641openalex-snapshot

Pressure-Dependent Ion Rejection in Nanopores

inferred← citeshttps://doi.org/10.1021/acs.jpcc.0c04158openalex-snapshot

Coupled Transport of Water and Ions through Graphene Nanochannels

inferred← citeshttps://doi.org/10.1021/acs.jpcc.0c09130openalex-snapshot

Synergic Effects of the Nanopore Size and Surface Charge on the Ion Selectivity of Graphene Membranes

inferred← citeshttps://doi.org/10.1021/acs.jpcc.1c06410openalex-snapshot

Salt-Water System under Diamond Confinement

inferred← citeshttps://doi.org/10.1021/acs.jpcc.2c06016openalex-snapshot

Theoretical Pathway toward Improved Reverse Osmosis Membrane Selectivity for Neutral Solutes: Inspiration from Gas Separations

inferred← citeshttps://doi.org/10.1021/acs.jpcc.4c01734openalex-snapshot

2D Dielectric Enhancement of Ion Coulomb Drag Amplification in Nanofluidics

inferred← citeshttps://doi.org/10.1021/acs.jpcc.8b09742openalex-snapshot

Charge Asymmetry Effect in Ion Transport through Angstrom-Scale Channels

inferred← citeshttps://doi.org/10.1021/acs.jpcc.8b10191openalex-snapshot

Electrically Tunable Ion Selectivity of Charged Nanopores

inferred← citeshttps://doi.org/10.1021/acs.jpcc.9b02178openalex-snapshot

Critical Knowledge Gaps in Mass Transport through Single-Digit Nanopores: A Review and Perspective

inferred← citeshttps://doi.org/10.1021/acs.jpcc.9b11750openalex-snapshot

Ion Permeability and Selectivity in Composite Nanochannels: Engineering through the End Effects

inferred← citeshttps://doi.org/10.1021/acs.jpclett.2c00156openalex-snapshot

Cation-Gated Ion Transport at Nanometer Scale for Tunable Power Generation

inferred← citeshttps://doi.org/10.1021/acs.jpclett.5c03986openalex-snapshot

Electrical Double Layer as a Voltage Divider: Suppressing Counterion Transport in Atomically Thin Nanopores

inferred← citeshttps://doi.org/10.1021/acs.jpclett.6c01538openalex-snapshot

Ion-Pairing-Mediated Selective Transport of Rare Earth Elements through Functionalized Graphene Nanopores

inferred← citeshttps://doi.org/10.1021/acs.langmuir.1c03473openalex-snapshot

Promoting Electroosmotic Water Flow through a Carbon Nanotube by Weakening the Competition between Cations and Anions in a Lateral Electric Field

inferred← citeshttps://doi.org/10.1021/acs.langmuir.2c01780openalex-snapshot

Enhanced Ion Rejection in Carbon Nanotubes by a Lateral Electric Field

inferred← citeshttps://doi.org/10.1021/acs.langmuir.3c00631openalex-snapshot

Selective Ion Transport in Two-Dimensional Ti3C2Tx Nanochannel Decorated by Crown Ether

inferred← citeshttps://doi.org/10.1021/acs.langmuir.7b01249openalex-snapshot

Mg2+-Channel-Inspired Nanopores for Mg2+/Li+ Separation: The Effect of Coordination on the Ionic Hydration Microstructures

inferred← citeshttps://doi.org/10.1021/acs.nanolett.4c00890openalex-snapshot

The Interplay of Solvation and Polarization Effects on Ion Pairing in Nanoconfined Electrolytes

inferred← citeshttps://doi.org/10.1021/acs.nanolett.4c06218openalex-snapshot

Scaling Behavior and Conductance Mechanisms of Ion Transport in Atomically Thin Graphene Nano/Subnanopores

inferred← citeshttps://doi.org/10.1021/acs.nanolett.5c00315openalex-snapshot

Resistance-Restorable Nanofluidic Memristor and Neuromorphic Chip

inferred← citeshttps://doi.org/10.1021/acs.nanolett.7b02846openalex-snapshot

Enantioselective Molecular Transport in Multilayer Graphene Nanopores

inferred← citeshttps://doi.org/10.1021/acsami.0c03932openalex-snapshot

Dehydration-Determined Ion Selectivity of Graphene Subnanopores

inferred← citeshttps://doi.org/10.1021/acsami.0c16468openalex-snapshot

Snap-through in Graphene Nanochannels: With Application to Fluidic Control

inferred← citeshttps://doi.org/10.1021/acsami.0c22689openalex-snapshot

Ionic Transport and Sieving Properties of Sub-nanoporous Polymer Membranes with Tunable Channel Size

inferred← citeshttps://doi.org/10.1021/acsami.3c10113openalex-snapshot

Tailoring Monovalent Ion Sieving in Graphene-Oxide Membranes with High Flux by Rationally Intercalating Crown Ethers

inferred← citeshttps://doi.org/10.1021/acsami.5c15216openalex-snapshot

Molecular Dynamics for Nanoconfined Ion and Water Transport: Mechanisms and Applications in Functional Nanofluidic Devices

inferred← citeshttps://doi.org/10.1021/acsami.6c11813openalex-snapshot

Electric-Field Effects on Selective Transport through Graphene Nanopores

inferred← citeshttps://doi.org/10.1021/acsami.8b09232openalex-snapshot

Renormalization of Ionic Solvation Shells in Nanochannels

inferred← citeshttps://doi.org/10.1021/acsami.9b13484openalex-snapshot

Aqueous Cathodic Exfoliation Strategy toward Solution-Processable and Phase-Preserved MoS2 Nanosheets for Energy Storage and Catalytic Applications

inferred← citeshttps://doi.org/10.1021/acsami.9b18234openalex-snapshot

Ion Rejection in Covalent Organic Frameworks: Revealing the Overlooked Effect of In-Pore Transport

inferred← citeshttps://doi.org/10.1021/acsanm.6c01675openalex-snapshot

Molecular Dynamics Simulation of Nanostructured Grazynes for Water Desalination

inferred← citeshttps://doi.org/10.1021/acsanm.8b02270openalex-snapshot

Single-Layer Graphene Sandwiched between Proton-Exchange Membranes for Selective Proton Transmission

inferred← citeshttps://doi.org/10.1021/acscatal.0c04343openalex-snapshot

Ultrathin Silicon Oxide Overlayers Enable Selective Oxygen Evolution from Acidic and Unbuffered pH-Neutral Seawater

inferred← citeshttps://doi.org/10.1021/acsestengg.6c00239openalex-snapshot

Regulating Ionic Composition to Tune Monovalent–Divalent Ion Selectivity in Nanofiltration Membranes

inferred← citeshttps://doi.org/10.1021/acsnano.0c04716openalex-snapshot

Stochastic Ionic Transport in Single Atomic Zero-Dimensional Pores

inferred← citeshttps://doi.org/10.1021/acsnano.0c05649openalex-snapshot

Precisely Tunable Ion Sieving with an Al13–Ti3C2T x Lamellar Membrane by Controlling Interlayer Spacing

inferred← citeshttps://doi.org/10.1021/acsnano.2c07641openalex-snapshot

Engineering Polymeric Nanofluidic Membranes for Efficient Ionic Transport: Biomimetic Design, Material Construction, and Advanced Functionalities

inferred← citeshttps://doi.org/10.1021/acsnano.3c11068openalex-snapshot

Tuning Pore Size in Graphene in the Angstrom Regime for Highly Selective Ion–Ion Separation

inferred← citeshttps://doi.org/10.1021/acsnano.4c00540openalex-snapshot

Ion–Ion Selectivity of Synthetic Membranes with Confined Nanostructures

inferred← citeshttps://doi.org/10.1021/acsnano.4c12051openalex-snapshot

Two-Dimensional Material-Based Nanofluidic Devices and Their Applications

inferred← citeshttps://doi.org/10.1021/acsnano.5c03775openalex-snapshot

Electrostatically Gated Trilayer Graphene Nanopore as an Ultrathin Rectifying Ion Filter

inferred← citeshttps://doi.org/10.1021/acsnano.5c13306openalex-snapshot

Elucidating the Mechanisms of Ion Permeation through Sub-Nanometer Graphene Pores: Uncovering Free Energy Barriers via High-Throughput Molecular Simulations

inferred← citeshttps://doi.org/10.1021/acsnano.6c04846openalex-snapshot

Anion Transport and Selectivity in Ordered Nanoporous Polymers with 1 nm Scale Charged Pores

inferred← citeshttps://doi.org/10.1021/acsnano.6c04963openalex-snapshot

Beyond the Continuum Theory: Conductance Scaling and Correlated Imaging in Atom-Scale Artificial Ion Channels

inferred← citeshttps://doi.org/10.1021/acsnano.9b06505openalex-snapshot

Ionic Conductance through Graphene: Assessing Its Applicability as a Proton Selective Membrane

inferred← citeshttps://doi.org/10.1021/jacs.1c05765openalex-snapshot

In Situ Characterization of Dehydration during Ion Transport in Polymeric Nanochannels

inferred← citeshttps://doi.org/10.1021/jacs.2c00318openalex-snapshot

Highly Ion-Permselective Porous Organic Cage Membranes with Hierarchical Channels

inferred← citeshttps://doi.org/10.1021/jacs.6c07978openalex-snapshot

Water-Mediated Ion Selectivity in 2D MXene Channels

inferred← citeshttps://doi.org/10.1021/jacs.8b08488openalex-snapshot

Drastically Reduced Ion Mobility in a Nanopore Due to Enhanced Pairing and Collisions between Dehydrated Ions

inferred← citeshttps://doi.org/10.1038/nnano.2017.21openalex-snapshot

Tunable sieving of ions using graphene oxide membranes

inferred← citeshttps://doi.org/10.1038/s41467-019-13648-7openalex-snapshot

Design principles of ion selective nanostructured membranes for the extraction of lithium ions

inferred← citeshttps://doi.org/10.1038/s41467-021-25938-0openalex-snapshot

Two-dimensional monolayer salt nanostructures can spontaneously aggregate rather than dissolve in dilute aqueous solutions

inferred← citeshttps://doi.org/10.1038/s41467-024-51877-7openalex-snapshot

Nanofluidic sensing inspired by the anomalous water dynamics in electrical angstrom-scale channels

inferred← citeshttps://doi.org/10.1038/s41467-024-52109-8openalex-snapshot

In situ generation of (sub) nanometer pores in MoS2 membranes for ion-selective transport

inferred← citeshttps://doi.org/10.1038/s41467-026-68800-xopenalex-snapshot

Chemistry-driven autonomous nanopore membranes

inferred← citeshttps://doi.org/10.1038/s41467-026-75929-2openalex-snapshot

Synthesis of ZIF-62 Glass and Solid-state Lithium Superconductor Composite Membranes for Electrodialytic Lithium Extraction

inferred← citeshttps://doi.org/10.1038/s41565-020-0713-6openalex-snapshot

Towards single-species selectivity of membranes with subnanometre pores

inferred← citeshttps://doi.org/10.1038/s41565-026-02182-5openalex-snapshot

Anomalous ultrafast lithium-ion transport through boron nitride nanotube membranes

inferred← citeshttps://doi.org/10.1038/s41565-026-02245-7openalex-snapshot

Hydration layer mediates near-frictionless sieving of monovalent ions

inferred← citeshttps://doi.org/10.1038/s41598-024-72245-xopenalex-snapshot

Highly selective removal of thallous ions from wastewater using Prussian Blue biochar composite

inferred← citeshttps://doi.org/10.1038/s41893-020-0474-0openalex-snapshot

Effective ion sieving with Ti3C2Tx MXene membranes for production of drinking water from seawater

inferred← citeshttps://doi.org/10.1038/s43246-021-00162-xopenalex-snapshot

Origin and control of ionic hydration patterns in nanopores

inferred← citeshttps://doi.org/10.1038/s43246-026-01082-4openalex-snapshot

Quantum correlation of channel-confined ions in graphene-based transistors for energy-efficient neuromorphic chips

inferred← citeshttps://doi.org/10.1039/c7cp07924aopenalex-snapshot

Maxwell-Hall access resistance in graphene nanopores

inferred← citeshttps://doi.org/10.1039/c7nr03838kopenalex-snapshot

Ionic selectivity and filtration from fragmented dehydration in multilayer graphene nanopores

inferred← citeshttps://doi.org/10.1039/c8en01400kopenalex-snapshot

A surface-modified EDTA-reduced graphene oxide membrane for nanofiltration and anti-biofouling prepared by plasma post-treatment

inferred← citeshttps://doi.org/10.1039/c8nr00050fopenalex-snapshot

Fabrication of sub-nanometer pores on graphene membrane for ion selective transport

inferred← citeshttps://doi.org/10.1039/c8nr04962aopenalex-snapshot

A coupled effect of dehydration and electrostatic interactions on selective ion transport through charged nanochannels

inferred← citeshttps://doi.org/10.1039/c8nr07557copenalex-snapshot

Heterogeneous graphene oxide membrane for rectified ion transport

inferred← citeshttps://doi.org/10.1039/c8ra07795aopenalex-snapshot

Ion transport through a nanoporous C 2 N membrane: the effect of electric field and layer number

inferred← citeshttps://doi.org/10.1039/c9cp05551gopenalex-snapshot

Theory and simulation developments of confined mass transport through graphene-based separation membranes

inferred← citeshttps://doi.org/10.1039/c9nr00317gopenalex-snapshot

Dehydration impeding ionic conductance through two-dimensional angstrom-scale slits

inferred← citeshttps://doi.org/10.1039/c9ta12293aopenalex-snapshot

Proton conductivity of a hexagonal boron nitride membrane and its energy applications

inferred← citeshttps://doi.org/10.1039/d0cp00805bopenalex-snapshot

The mechanism and energetics of a ligand-controlled hydrophobic gate in a mammalian two pore channel

inferred← citeshttps://doi.org/10.1039/d0cp02993aopenalex-snapshot

Controlling ion transport in a C 2 N-based nanochannel with tunable interlayer spacing

inferred← citeshttps://doi.org/10.1039/d0nr04496bopenalex-snapshot

Selectivity of nitrate and chloride ions in microporous carbons: the role of anisotropic hydration and applied potentials

inferred← citeshttps://doi.org/10.1039/d1cs01061aopenalex-snapshot

The coming of age of water channels for separation membranes: from biological to biomimetic to synthetic

inferred← citeshttps://doi.org/10.1039/d1dt02206gopenalex-snapshot

Two-dimensional materials as solid-state nanopores for chemical sensing

inferred← citeshttps://doi.org/10.1039/d1nr02169aopenalex-snapshot

High-throughput molecular simulations reveal the origin of ion free energy barriers in graphene oxide membranes

inferred← citeshttps://doi.org/10.1039/d2cp00025copenalex-snapshot

Asymmetric transport and desalination in graphene channels

inferred← citeshttps://doi.org/10.1039/d2cp02564gopenalex-snapshot

Nanoconfinement effects on water in narrow graphene-based slit pores as revealed by THz spectroscopy

inferred← citeshttps://doi.org/10.1039/d2nr05552jopenalex-snapshot

Coupling solute interactions with functionalized graphene membranes: towards facile membrane-level engineering

inferred← citeshttps://doi.org/10.1039/d3ew00769copenalex-snapshot

Mechanism of lithium ion selectivity through membranes: a brief review

inferred← citeshttps://doi.org/10.1039/d3fd00062aopenalex-snapshot

Spiers Memorial Lecture: Towards understanding of iontronic systems: electroosmotic flow of monovalent and divalent electrolyte through charged cylindrical nanopores

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