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N-Heterocyclic-Carbene-Catalyzed C–H Acylation via Radical Relay

https://doi.org/10.1021/acs.orglett.1c04317

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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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Electron-Transfer Properties of Active Aldehydes of Thiamin Coenzyme Models, and Mechanism of Formation of the Reactive Intermediates

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Direct Observation of Radical Intermediates While Investigating the Redox Behavior of Thiamin Coenzyme Models

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Biomimetic Carbene‐Catalyzed Oxidations of Aldehydes Using TEMPO

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N‐Heterocyclic Carbene Catalyzed γ‐Dihalomethylenation of Enals by Single‐Electron Transfer

inferredcites →https://doi.org/10.1002/anie.201709684openalex-snapshot

N‐Heterocyclic Carbene Catalysis via Azolium Dienolates: An Efficient Strategy for Remote Enantioselective Functionalizations

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Sulfamate Esters Guide Selective Radical‐Mediated Chlorination of Aliphatic C−H Bonds

inferredcites →https://doi.org/10.1002/anie.201807455openalex-snapshot

Site‐Selective Remote Radical C−H Functionalization of Unactivated C−H Bonds in Amides Using Sulfone Reagents

inferredcites →https://doi.org/10.1002/anie.201807623openalex-snapshot

Copper‐Catalyzed Arylation of Remote C(sp 3 )−H Bonds in Carboxamides and Sulfonamides

inferredcites →https://doi.org/10.1002/anie.201813425openalex-snapshot

Copper‐Catalyzed Remote C(sp 3 )−H Trifluoromethylation of Carboxamides and Sulfonamides

inferredcites →https://doi.org/10.1002/anie.201903726openalex-snapshot

The Persistent Radical Effect in Organic Synthesis

inferredcites →https://doi.org/10.1002/anie.201909017openalex-snapshot

Visible‐Light‐Driven N‐Heterocyclic Carbene Catalyzed γ‐ and ϵ‐Alkylation with Alkyl Radicals

inferredcites →https://doi.org/10.1002/anie.201912450openalex-snapshot

Radical Acylfluoroalkylation of Olefins through N‐Heterocyclic Carbene Organocatalysis

inferredcites →https://doi.org/10.1002/anie.201913042openalex-snapshot

Generation and Reactivity of Amidyl Radicals: Manganese‐Mediated Atom‐Transfer Reaction

inferredcites →https://doi.org/10.1002/anie.201914456openalex-snapshot

N‐Heterocyclic Carbene Catalyzed Photoenolization/Diels–Alder Reaction of Acid Fluorides

inferredcites →https://doi.org/10.1002/anie.202001824openalex-snapshot

Combined Photoredox and Carbene Catalysis for the Synthesis of Ketones from Carboxylic Acids**

inferredcites →https://doi.org/10.1002/chem.202004059openalex-snapshot

Single‐Electron Transfer Reactions Enabled by N‐Heterocyclic Carbene Organocatalysis

inferredcites →https://doi.org/10.1002/cjoc.202000107openalex-snapshot

N‐Heterocyclic Carbene Organocatalysis: Activation Modes and Typical Reactive Intermediates

inferredcites →https://doi.org/10.1016/j.chempr.2019.09.010openalex-snapshot

Chiral Piperidines from Acyclic Amines Via Enantioselective, Radical-Mediated δ C-H Cyanation

inferredcites →https://doi.org/10.1021/acs.accounts.9b00635openalex-snapshot

Bifunctional N-Heterocyclic Carbenes Derived from l -Pyroglutamic Acid and Their Applications in Enantioselective Organocatalysis

inferredcites →https://doi.org/10.1021/acs.chemrev.5b00060openalex-snapshot

Organocatalytic Reactions Enabled by N-Heterocyclic Carbenes

inferredcites →https://doi.org/10.1021/acs.chemrev.8b00067openalex-snapshot

Electronic Properties of N-Heterocyclic Carbenes and Their Experimental Determination

inferredcites →https://doi.org/10.1021/acs.chemrev.9b00634openalex-snapshot

N-Heterocyclic Carbene Complexes in C–H Activation Reactions

inferredcites →https://doi.org/10.1021/acs.orglett.0c00829openalex-snapshot

Copper-Catalyzed Remote C(sp3)–H Amination of Carboxamides

inferredcites →https://doi.org/10.1021/acs.orglett.0c01072openalex-snapshot

Redox Neutral Radical-Relay Cobalt Catalysis toward C–H Fluorination and Amination

inferredcites →https://doi.org/10.1021/acs.orglett.0c01199openalex-snapshot

N-Heterocyclic Carbene-Catalyzed Radical Relay Enabling Synthesis of δ-Ketocarbonyls

inferredcites →https://doi.org/10.1021/acs.orglett.0c02008openalex-snapshot

Enantioselective Remote C(sp 3 )–H Cyanation via Dual Photoredox and Copper Catalysis

inferredcites →https://doi.org/10.1021/acs.orglett.0c02202openalex-snapshot

Bio- and Medicinally Compatible α-Amino-Acid Modification via Merging Photoredox and N-Heterocyclic Carbene Catalysis

inferredcites →https://doi.org/10.1021/acs.orglett.0c03883openalex-snapshot

N-Heterocyclic Carbene/Magnesium Cocatalyzed Radical Relay Assembly of Aliphatic Keto Nitriles

inferredcites →https://doi.org/10.1021/acs.orglett.0c03907openalex-snapshot

Organocatalytic Three-Component 1,2-Cyanoalkylacylation of Alkenes via Radical Relay

inferredcites →https://doi.org/10.1021/acs.orglett.0c04248openalex-snapshot

C–C Bond Acylation of Oxime Ethers via NHC Catalysis

inferredcites →https://doi.org/10.1021/acs.orglett.1c01400openalex-snapshot

Construction of Quaternary Carbon Center via NHC Catalysis Initiated by an Intermolecular Heck-Type Alkyl Radical Addition

inferredcites →https://doi.org/10.1021/acs.orglett.1c01443openalex-snapshot

Iron-Catalyzed, Site-Selective Difluoromethylthiolation (−SCF2H) and Difluoromethylselenation (−SeCF2H) of Unactivated C(sp3)–H Bonds in N-Fluoroamides

inferredcites →https://doi.org/10.1021/acs.orglett.1c02564openalex-snapshot

(1-Selenocyanatoethyl)benzene: A Selenocyanation Reagent for Site-Selective Selenocyanation of Inert Alkyl C(sp3)–H Bonds

inferredcites →https://doi.org/10.1021/acs.orglett.1c02639openalex-snapshot

Radical Relay Trichloromethylacylation of Alkenes through N-Heterocyclic Carbene Catalysis

inferredcites →https://doi.org/10.1021/acs.orglett.1c03059openalex-snapshot

Synthesis of Functionalized Dihydrocoumarins by NHC-Catalyzed [3 + 3] Annulation of Enals with 2-Substituted Naphthoquinones

inferredcites →https://doi.org/10.1021/acs.orglett.1c03075openalex-snapshot

Copper-Catalyzed N-Directed Distal C(sp3)–H Sulfonylation and Thiolation with Sulfinate Salts

inferredcites →https://doi.org/10.1021/acs.orglett.6b03792openalex-snapshot

Carbene-Catalyzed Reductive Coupling of Nitrobenzyl Bromide and Nitroalkene via the Single-Electron-Transfer (SET) Process and Formal 1,4-Addition

inferredcites →https://doi.org/10.1021/acs.orglett.8b02514openalex-snapshot

Remote Site-Specific Radical Alkynylation of Unactivated C–H Bonds

inferredcites →https://doi.org/10.1021/acs.orglett.9b04203openalex-snapshot

NHC-Catalyzed Radical Trifluoromethylation Enabled by Togni Reagent

inferredcites →https://doi.org/10.1021/acscatal.0c01795openalex-snapshot

N-Heterocyclic Carbene-Based Catalysis Enabling Cross-Coupling Reactions

inferredcites →https://doi.org/10.1021/acscatal.1c03459openalex-snapshot

Recent Progress toward the Construction of Axially Chiral Molecules Catalyzed by an N-heterocyclic Carbene

inferredcites →https://doi.org/10.1021/acscatal.1c03861openalex-snapshot

1,4-Alkylcarbonylation of 1,3-Enynes to Access Tetra-Substituted Allenyl Ketones via an NHC-Catalyzed Radical Relay

inferredcites →https://doi.org/10.1021/cr00017a013openalex-snapshot

Photochemistry on nonreactive and reactive (semiconductor) surfaces

inferredcites →https://doi.org/10.1021/cr60221a004openalex-snapshot

Cyclization of N-Halogenated Amines (The Hofmann-Löffler Reaction).

inferredcites →https://doi.org/10.1021/cr900096xopenalex-snapshot

Transition Metal Catalyzed Alkene and Alkyne Hydroacylation

inferredcites →https://doi.org/10.1021/ja3030164openalex-snapshot

Catalytic Asymmetric α-Acylation of Tertiary Amines Mediated by a Dual Catalysis Mode: N-Heterocyclic Carbene and Photoredox Catalysis

inferredcites →https://doi.org/10.1021/jacs.6b08171openalex-snapshot

Iron-Catalyzed, Fluoroamide-Directed C–H Fluorination

inferredcites →https://doi.org/10.1021/jacs.9b00880openalex-snapshot

N-Heterocyclic Carbene-Catalyzed Decarboxylative Alkylation of Aldehydes

inferredcites →https://doi.org/10.1021/jacs.9b07194openalex-snapshot

N-Heterocyclic Carbene-Catalyzed Radical Relay Enabling Vicinal Alkylacylation of Alkenes

inferredcites →https://doi.org/10.1021/jacs.9b10316openalex-snapshot

Copper-Catalyzed, N-Directed Csp 3 –H Trifluoromethylthiolation (−SCF 3 ) and Trifluoromethylselenation (−SeCF 3 )

inferredcites →https://doi.org/10.1021/jacs.9b11549openalex-snapshot

Copper-Catalyzed, Chloroamide-Directed Benzylic C–H Difluoromethylation

inferredcites →https://doi.org/10.1021/ol5027415openalex-snapshot

N-Heterocyclic Carbene Organocatalytic Reductive β,β-Coupling Reactions of Nitroalkenes via Radical Intermediates

inferredcites →https://doi.org/10.1038/nature07367openalex-snapshot

The advent and development of organocatalysis

inferredcites →https://doi.org/10.1038/nature13384openalex-snapshot

An overview of N-heterocyclic carbenes

inferredcites →https://doi.org/10.1038/ncomms12933openalex-snapshot

Carbene-catalysed reductive coupling of nitrobenzyl bromides and activated ketones or imines via single-electron-transfer process

inferredcites →https://doi.org/10.1038/s41467-019-08741-wopenalex-snapshot

Copper-catalyzed remote C(sp3)–H azidation and oxidative trifluoromethylation of benzohydrazides

inferredcites →https://doi.org/10.1038/s41467-019-13705-1openalex-snapshot

Copper-catalyzed enantioselective Sonogashira-type oxidative cross-coupling of unactivated C(sp3)−H bonds with alkynes

inferredcites →https://doi.org/10.1038/s41467-021-22292-zopenalex-snapshot

Benzylic C−H acylation by cooperative NHC and photoredox catalysis

inferredcites →https://doi.org/10.1039/b100919mopenalex-snapshot

Structure-based design of agrochemicals

inferredcites →https://doi.org/10.1039/c1cs15109fopenalex-snapshot

Palladium-catalyzed carbonylative coupling reactions between Ar–X and carbon nucleophiles

inferredcites →https://doi.org/10.1039/c8sc04366copenalex-snapshot

δ C–H (hetero)arylation via Cu-catalyzed radical relay

inferredcites →https://doi.org/10.1039/c9cc09272bopenalex-snapshot

N-Heterocyclic carbene/photo-cocatalyzed oxidative Smiles rearrangement: synthesis of aryl salicylates from O -aryl salicylaldehydes

inferredcites →https://doi.org/10.1039/c9sc04055bopenalex-snapshot

N-Directed fluorination of unactivated Csp 3 –H bonds

inferredcites →https://doi.org/10.1039/d0qo00494dopenalex-snapshot

Dual N-heterocyclic carbene/photocatalysis: a new strategy for radical processes

inferredcites →https://doi.org/10.1039/d0sc00225aopenalex-snapshot

N-Heterocyclic carbene-catalyzed deaminative cross-coupling of aldehydes with Katritzky pyridinium salts

inferredcites →https://doi.org/10.1039/d0sc01538eopenalex-snapshot

Recent advances in N-heterocyclic carbene-based radical catalysis

inferredcites →https://doi.org/10.1039/d0sc03595eopenalex-snapshot

Light opens a new window for N-heterocyclic carbene catalysis

inferredcites →https://doi.org/10.1039/d1qo01127hopenalex-snapshot

Generation of azolium dienolates as versatile nucleophilic synthons via N -heterocyclic carbene catalysis

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

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Generation and Radical-Radical Cross-Coupling of Alkenyloxy Radical: Ester and Ketone Synthesis

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Recent Advances in the Functionalization of Remote C−H Bonds by Hofmann‐Löffler‐Freytag‐type Reactions

inferred← citeshttps://doi.org/10.1002/ajoc.202400663openalex-snapshot

Site‐Selective C‐Alkylation of Fluoroamides with Active Methylene Compounds

inferred← citeshttps://doi.org/10.1002/ange.202207824openalex-snapshot

Oxidative Radical NHC Catalysis: Divergent Difunctionalization of Olefins through Intermolecular Hydrogen Atom Transfer

inferred← citeshttps://doi.org/10.1002/ange.202303388openalex-snapshot

Carbene‐Catalyzed Intermolecular Dehydrogenative Coupling of Aldehydes with C(sp3)−H Bonds

inferred← citeshttps://doi.org/10.1002/anie.202207824openalex-snapshot

Oxidative Radical NHC Catalysis: Divergent Difunctionalization of Olefins through Intermolecular Hydrogen Atom Transfer

inferred← citeshttps://doi.org/10.1002/anie.202303388openalex-snapshot

Carbene‐Catalyzed Intermolecular Dehydrogenative Coupling of Aldehydes with C(sp3)−H Bonds

inferred← citeshttps://doi.org/10.1002/cctc.202201320openalex-snapshot

Merging N‐Heterocyclic Carbene Organocatalysis with Hydrogen Atom Transfer Strategy

inferred← citeshttps://doi.org/10.1002/chem.202203716openalex-snapshot

Synthesis of Thioesters from Aldehydes via N‐Heterocyclic Carbene (NHC) Catalyzed Radical Relay

inferred← citeshttps://doi.org/10.1002/chem.202401811openalex-snapshot

N‐Heterocyclic Carbene Enabled Functionalization of Inert C(Sp3)−H Bonds via Hydrogen Atom Transfer (HAT) Processes

inferred← citeshttps://doi.org/10.1002/chem.202402288openalex-snapshot

Cooperative NHC and Photoredox Catalyzed Radical Aminoacylation of Alkenes to Tetrahydropyridazines

inferred← citeshttps://doi.org/10.1002/ejoc.202400027openalex-snapshot

Copper‐Catalyzed Fluoroamide‐Directed Remote C( sp 3 )‐H Bond Functionalization Through Intramolecular Hydrogen Atom Transfer

inferred← citeshttps://doi.org/10.1002/ejoc.202501155openalex-snapshot

Copper‐Catalyzed Chloroamide‐Directed Benzylic CH Perfluoroalkylation

inferred← citeshttps://doi.org/10.1007/s11426-024-2309-5openalex-snapshot

Benzoyl cyanide, a general radical acylating reagent for photoredox-catalyzed benzylic site-selective acylation reactions

inferred← citeshttps://doi.org/10.1007/s11426-025-2680-2openalex-snapshot

Cooperative N-heterocyclic carbenes and photocatalysis for the three-component alkylacylation of alkenes: divergent ketone synthesis

inferred← citeshttps://doi.org/10.1016/j.cclet.2024.109495openalex-snapshot

Enones from aldehydes and alkenes by carbene-catalyzed dehydrogenative couplings

inferred← citeshttps://doi.org/10.1016/j.gresc.2024.04.007openalex-snapshot

Recent advances in transition-metal-free conversion of aldehydes to ketones

inferred← citeshttps://doi.org/10.1016/j.tet.2025.134451openalex-snapshot

Copper-catalyzed remote C(sp3)-H heteroarylation of N-fluorocarboxamides with azoles

inferred← citeshttps://doi.org/10.1016/j.tetlet.2023.154483openalex-snapshot

N-Heterocyclic carbene-catalyzed remote C(sp3)–H acylation of amides

inferred← citeshttps://doi.org/10.1021/acs.chemrev.4c00661openalex-snapshot

Nitrogen-Based Organofluorine Functional Molecules: Synthesis and Applications

inferred← citeshttps://doi.org/10.1021/acs.joc.2c00881openalex-snapshot

BF3-Mediated Acetylation of Pyrazolo[1,5-a]pyrimidines and Other π-Excedent (N-Hetero)arenes

inferred← citeshttps://doi.org/10.1021/acs.joc.2c02461openalex-snapshot

Fluorosulfonamide-Directed Heteroarylation of Aliphatic C(sp3)–H Bonds

inferred← citeshttps://doi.org/10.1021/acs.joc.3c02427openalex-snapshot

Cross-Coupling of Benzylic and Aldehydic C–H Bonds via Photocatalytic Tandem Radical–Radical Coupling and Acceptorless Alcohol Dehydrogenation

inferred← citeshttps://doi.org/10.1021/acs.joc.5c02667openalex-snapshot

Direct γ-C(sp3)–H Acylation of Amide Derivatives via Cooperative NHC and Photoredox Catalysis

inferred← citeshttps://doi.org/10.1021/acs.orglett.2c01427openalex-snapshot

Copper-Catalyzed Hydrogen Atom Transfer and Aryl Migration Strategy for the Arylalkylation of Activated Alkenes

inferred← citeshttps://doi.org/10.1021/acs.orglett.2c03148openalex-snapshot

Divergent Construction of Heterocycles by SOMOphilic Isocyanide Insertion under N-Heterocyclic Carbene Catalysis

inferred← citeshttps://doi.org/10.1021/acs.orglett.3c00006openalex-snapshot

Iminoacylation of Alkenes via Photoredox N-Heterocyclic Carbene Catalysis

inferred← citeshttps://doi.org/10.1021/acs.orglett.3c00654openalex-snapshot

Redox Neutral Radical-Relay Nickel-Catalyzed Remote Carbonylation

inferred← citeshttps://doi.org/10.1021/acs.orglett.3c01168openalex-snapshot

Synthesis of β-Ketonitriles via N-Heterocyclic-Carbene-Catalyzed Radical Coupling of Aldehydes and Azobis(isobutyronitrile)

inferred← citeshttps://doi.org/10.1021/acs.orglett.3c03588openalex-snapshot

Synthesis of Pyrroloindolines via N-Heterocyclic Carbene Catalyzed Dearomative Amidoacylation of Indole Derivatives

inferred← citeshttps://doi.org/10.1021/acs.orglett.4c00234openalex-snapshot

Synthesis of γ-Oxo-phosphonates via N -Heterocyclic Carbene-Catalyzed Acylphosphorylation of Alkenes

inferred← citeshttps://doi.org/10.1021/acs.orglett.4c00627openalex-snapshot

Generation and Radical–Radical Cross-Coupling of Alkenyloxy Radical

inferred← citeshttps://doi.org/10.1021/acs.orglett.6c03213openalex-snapshot

Nickel-Catalyzed Strain-Release Alkyl–Alkyl Cross-Coupling of N -Chlorocyclopropamides with Tertiary α-Bromo Esters

inferred← citeshttps://doi.org/10.1021/acscatal.2c03996openalex-snapshot

Radical NHC Catalysis

inferred← citeshttps://doi.org/10.1021/acsorginorgau.3c00008openalex-snapshot

On the Redox Properties of the Dimers of Thiazol-2-ylidenes That Are Relevant for Radical Catalysis

inferred← citeshttps://doi.org/10.1021/jacs.2c12845openalex-snapshot

Photoinduced Acylations Via Azolium-Promoted Intermolecular Hydrogen Atom Transfer

inferred← citeshttps://doi.org/10.1021/jacs.5c01642openalex-snapshot

Photobiocatalytic Enantioselective Benzylic C(sp 3 )–H Acylation Enabled by Thiamine-Dependent Enzymes via Intermolecular Hydrogen Atom Transfer

inferred← citeshttps://doi.org/10.1021/jacs.6c10645openalex-snapshot

NHC-Mediated Olefin Amidoacylation via Amidyl Radical Intermediates Leading to 5- and 6-Membered Keto-Lactams

inferred← citeshttps://doi.org/10.1039/d2gc02874copenalex-snapshot

Remote C(sp 3 )–H heteroarylation of N -fluorocarboxamides with quinoxalin-2(1 H )-ones under visible-light-induced photocatalyst-free conditions

inferred← citeshttps://doi.org/10.1039/d2nj01078jopenalex-snapshot

A DFT study of NHC-catalyzed reactions between 2-bromo-2-enals and acylhydrazones: mechanisms, and chemo- and stereoselectivities

inferred← citeshttps://doi.org/10.1039/d2ob01711copenalex-snapshot

Copper-catalyzed intramolecular iminolactonization cyclization reactions of remote C(sp 3 )–H bonds in carboxamides

inferred← citeshttps://doi.org/10.1039/d2qo01846bopenalex-snapshot

Radical acylation: concepts, synthetic applications and directions

inferred← citeshttps://doi.org/10.1039/d3qo00544eopenalex-snapshot

Synthesis of 2-pyrrolidinone derivatives via N-heterocyclic carbene catalyzed radical tandem cyclization/coupling reactions

inferred← citeshttps://doi.org/10.1039/d3qo01129aopenalex-snapshot

Direct coupling of inert C–H bonds in NHC organocatalysis

inferred← citeshttps://doi.org/10.1039/d3qo01435eopenalex-snapshot

Nucleophilic organocatalysis involving radical intermediates

inferred← citeshttps://doi.org/10.1039/d3qo01933kopenalex-snapshot

Cu-catalyzed alkylarylation of alkenes via N -directed remote C(sp 3 )–H functionalization

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Mechanisms and origins of stereoselectivity in the NHC-catalyzed oxidative reaction of enals and pyrroles: a density functional theory study

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Remote C(sp 3 )–H acylation of amides under photoredox cooperative N-heterocyclic carbene/palladium catalysis

inferred← citeshttps://doi.org/10.1039/d5cs00600gopenalex-snapshot

Advances in N-heterocyclic carbene organocatalysis from 2015 to 2024

inferred← citeshttps://doi.org/10.1039/d6cc01204copenalex-snapshot

Cross-coupling of aryl aldehydes and benzyl chlorides enabled by dual N-heterocyclic carbene/cobalt catalysis

inferred← citeshttps://doi.org/10.1039/d6cc04481fopenalex-snapshot

Copper-catalyzed [3+2] annulation of N -chlorocyclopropylamides with alkenes to cyclopentenes

inferred← citeshttps://doi.org/10.1039/d6cp01100dopenalex-snapshot

A computational study of NHC-catalyzed [3+3] annulation of enals with pyrazol-5-amines: mechanism, and regio- and stereoselectivities

inferred← citeshttps://doi.org/10.1055/a-1822-4690openalex-snapshot

Research Progress on N-Heterocyclic Carbene Catalyzed Reactions for Synthesizing Ketones through Radical Mechanism

inferred← citeshttps://doi.org/10.1055/a-2145-8697openalex-snapshot

Aminoacylation of Alkenes by Cooperative NHC and Photoredox Catalysis

inferred← citeshttps://doi.org/10.3762/bjoc.21.153openalex-snapshot

Photochemical reduction of acylimidazolium salts

inferred← citeshttps://doi.org/10.6023/cjoc202206057openalex-snapshot

Synthesis of Bibenzyl Derivatives via Visible-Light-Promoted 1,5-Hydrogen Atom Transfer/Radical Coupling Reactions of N-Fluorocarboxamides

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Recent Advances in Copper-Catalyzed C(sp 3 )—H Bond Functionalization of N-Fluorosulfonamides via Hydrogen Atom Transfer

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