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Atomistic Insights into Medium-Entropy Perovskites for Efficient and Robust CO 2 Electrolysis

https://doi.org/10.1021/acsami.3c09913
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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

inferredcites →https://doi.org/10.1002/adfm.201600243openalex-snapshot
Understanding and Controlling the Work Function of Perovskite Oxides Using Density Functional Theory
inferredcites →https://doi.org/10.1002/adfm.202101632openalex-snapshot
Advanced High Entropy Perovskite Oxide Electrocatalyst for Oxygen Evolution Reaction
inferredcites →https://doi.org/10.1002/adfm.202112157openalex-snapshot
High Configuration Entropy Activated Lattice Oxygen for O 2 Formation on Perovskite Electrocatalyst
inferredcites →https://doi.org/10.1002/adma.201806236openalex-snapshot
High‐Entropy Oxides: Fundamental Aspects and Electrochemical Properties
inferredcites →https://doi.org/10.1002/adma.202209469openalex-snapshot
An Efficient High‐Entropy Perovskite‐Type Air Electrode for Reversible Oxygen Reduction and Water Splitting in Protonic Ceramic Cells
inferredcites →https://doi.org/10.1002/aenm.201803156openalex-snapshot
Perovskite Oxyfluoride Electrode Enabling Direct Electrolyzing Carbon Dioxide with Excellent Electrochemical Performances
inferredcites →https://doi.org/10.1002/aenm.202102845openalex-snapshot
Unraveling the Enhanced Kinetics of Sr2Fe1+xMo1‐xO6‐δ Electrocatalysts for High‐Performance Solid Oxide Cells
inferredcites →https://doi.org/10.1002/aenm.202202175openalex-snapshot
Building Efficient and Durable Hetero‐Interfaces on a Perovskite‐Based Electrode for Electrochemical CO 2 Reduction
inferredcites →https://doi.org/10.1002/anie.202006536openalex-snapshot
Atomic‐Scale Insight into Exsolution of CoFe Alloy Nanoparticles in La 0.4 Sr 0.6 Co 0.2 Fe 0.7 Mo 0.1 O 3− δ with Efficient CO 2 Electrolysis
inferredcites →https://doi.org/10.1002/fuce.201400196openalex-snapshot
CO/CO2 Study of High Performance La0.3Sr0.7Fe0.7Cr0.3O3–δ Reversible SOFC Electrodes
inferredcites →https://doi.org/10.1002/smll.201803513openalex-snapshot
Unfolding BOB Bonds for an Enhanced ORR Performance in ABO3‐Type Perovskites
inferredcites →https://doi.org/10.1007/s40820-022-00967-6openalex-snapshot
High-Entropy Perovskite Oxide: A New Opportunity for Developing Highly Active and Durable Air Electrode for Reversible Protonic Ceramic Electrochemical Cells
inferredcites →https://doi.org/10.1016/0927-0256(96)00008-0openalex-snapshot
Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
inferredcites →https://doi.org/10.1016/j.apcatb.2019.118389openalex-snapshot
Enhancing CO2 catalytic activation and direct electroreduction on in-situ exsolved Fe/MnOx nanoparticles from (Pr,Ba)2Mn2-yFeyO5+δ layered perovskites for SOEC cathodes
inferredcites →https://doi.org/10.1016/j.apcatb.2020.118656openalex-snapshot
Oxygen vacancies-rich Ce0.9Gd0.1O2-δ decorated Pr0.5Ba0.5CoO3-δ bifunctional catalyst for efficient and long-lasting rechargeable Zn-air batteries
inferredcites →https://doi.org/10.1016/j.apcatb.2020.118842openalex-snapshot
In-situ growth of nanoparticles-decorated double perovskite electrode materials for symmetrical solid oxide cells
inferredcites →https://doi.org/10.1016/j.apcatb.2020.119642openalex-snapshot
Coke formation during high-temperature CO2 electrolysis over AFeO3 (A = La/Sr) cathode: Effect of A-site metal segregation
inferredcites →https://doi.org/10.1016/j.apcatb.2021.120264openalex-snapshot
Medium-Entropy perovskites Sr(FeαTiβCoγMnζ)O3- as promising cathodes for intermediate temperature solid oxide fuel cell
inferredcites →https://doi.org/10.1016/j.apcatb.2021.120562openalex-snapshot
Electronic tuning of SrIrO3 perovskite nanosheets by sulfur incorporation to induce highly efficient and long-lasting oxygen evolution in acidic media
inferredcites →https://doi.org/10.1016/j.apcatb.2022.121579openalex-snapshot
Realizing robust and efficient acidic oxygen evolution by electronic modulation of 0D/2D CeO2 quantum dots decorated SrIrO3 nanosheets
inferredcites →https://doi.org/10.1016/j.apcatb.2022.121754openalex-snapshot
Two-fold improvement in chemical adsorption ability to achieve effective carbon dioxide electrolysis
inferredcites →https://doi.org/10.1016/j.apcatb.2023.122968openalex-snapshot
Engineering dual-exsolution on self-assembled cathode to achieve efficient electrocatalytic CO2 reduction
inferredcites →https://doi.org/10.1016/j.apmate.2023.100129openalex-snapshot
Novel high-entropy perovskite-type symmetrical electrode for efficient and durable carbon dioxide reduction reaction
inferredcites →https://doi.org/10.1016/j.elecom.2016.06.008openalex-snapshot
Efficient electrolysis of CO2 in symmetrical solid oxide electrolysis cell with highly active La0.3Sr0.7Fe0.7Ti0.3O3 electrode material
inferredcites →https://doi.org/10.1016/j.jallcom.2021.159633openalex-snapshot
A high-entropy perovskite cathode for solid oxide fuel cells
inferredcites →https://doi.org/10.1016/j.jcou.2016.11.014openalex-snapshot
Efficient conversion of CO 2 in solid oxide electrolytic cells with Pd doped perovskite cathode on ceria nanofilm interlayer
inferredcites →https://doi.org/10.1016/j.jcou.2019.07.021openalex-snapshot
Electrochemical reduction of CO2 in a symmetrical solid oxide electrolysis cell with La0.4Sr0.6Co0.2Fe0.7Nb0.1O3-δ electrode
inferredcites →https://doi.org/10.1016/j.jcou.2019.10.017openalex-snapshot
An efficient symmetrical solid oxide electrolysis cell with LSFM-based electrodes for direct electrolysis of pure CO2
inferredcites →https://doi.org/10.1016/j.jechem.2018.11.002openalex-snapshot
Infiltration of Ce0.8Gd0.2O1.9 nanoparticles on Sr2Fe1.5Mo0.5O6- cathode for CO2 electroreduction in solid oxide electrolysis cell
inferredcites →https://doi.org/10.1016/j.jpowsour.2012.12.068openalex-snapshot
Direct electrolysis of CO2 using an oxygen-ion conducting solid oxide electrolyzer based on La0.75Sr0.25Cr0.5Mn0.5O3 − electrode
inferredcites →https://doi.org/10.1016/j.jpowsour.2018.08.017openalex-snapshot
(La0.75Sr0.25)0.95(Cr0.5Mn0.5)O3-δ-Ce0.8Gd0.2O1.9 scaffolded composite cathode for high temperature CO2 electroreduction in solid oxide electrolysis cell
inferredcites →https://doi.org/10.1016/j.jpowsour.2020.228959openalex-snapshot
A novel facile strategy to suppress Sr segregation for high-entropy stabilized La0·8Sr0·2MnO3-δ cathode
inferredcites →https://doi.org/10.1016/j.nanoen.2020.104598openalex-snapshot
Pd single site-anchored perovskite cathode for CO2 electrolysis in solid oxide electrolysis cells
inferredcites →https://doi.org/10.1016/j.nanoen.2020.105207openalex-snapshot
Multi-functionalities enabled fivefold applications of LaCo0.6Ni0.4O3−δ in intermediate temperature symmetrical solid oxide fuel/electrolysis cells
inferredcites →https://doi.org/10.1016/j.seppur.2022.122287openalex-snapshot
Efficient electrochemical CO2 reduction reaction on a robust perovskite type cathode with in-situ exsolved Fe-Ru alloy nanocatalysts
inferredcites →https://doi.org/10.1021/acs.accounts.1c00674openalex-snapshot
Electrochemical Approaches for CO2 Conversion to Chemicals: A Journey toward Practical Applications
inferredcites →https://doi.org/10.1021/acsaem.1c03822openalex-snapshot
A Strategy to Enhance the Catalytic Activity of Electrode Materials by Doping Bismuth for Symmetrical Solid Oxide Electrolysis Cells
inferredcites →https://doi.org/10.1021/acsami.2c03657openalex-snapshot
High-Entropy Perovskite as a High-Performing Chromium-Tolerant Cathode for Solid Oxide Fuel Cells
inferredcites →https://doi.org/10.1021/acsenergylett.8b02525openalex-snapshot
CO2 Electrochemical Reduction As Probed through Infrared Spectroscopy
inferredcites →https://doi.org/10.1021/acssuschemeng.1c07576openalex-snapshot
Anion Fluorine-Doped La 0.6 Sr 0.4 Fe 0.8 Ni 0.2 O 3−δ Perovskite Cathodes with Enhanced Electrocatalytic Activity for Solid Oxide Electrolysis Cell Direct CO 2 Electrolysis
inferredcites →https://doi.org/10.1021/acssuschemeng.7b02511openalex-snapshot
Mixed-Conductor Sr 2 Fe 1.5 Mo 0.5 O 6−δ as Robust Fuel Electrode for Pure CO 2 Reduction in Solid Oxide Electrolysis Cell
inferredcites →https://doi.org/10.1038/s41467-018-05774-5openalex-snapshot
High entropy oxides for reversible energy storage
inferredcites →https://doi.org/10.1038/s41467-022-32393-yopenalex-snapshot
Boosting the stability of perovskites with exsolved nanoparticles by B-site supplement mechanism
inferredcites →https://doi.org/10.1039/c4cp01503gopenalex-snapshot
A Raman spectroscopic study of the carbon deposition mechanism on Ni/CGO electrodes during CO/CO 2 electrolysis
inferredcites →https://doi.org/10.1039/c7ta05750dopenalex-snapshot
A novel fuel electrode enabling direct CO 2 electrolysis with excellent and stable cell performance
inferredcites →https://doi.org/10.1039/c9cc03455bopenalex-snapshot
Cu-Doped Sr 2 Fe 1.5 Mo 0.5 O 6−δ as a highly active cathode for solid oxide electrolytic cells
inferredcites →https://doi.org/10.1039/c9ta00643eopenalex-snapshot
A self-recovering robust electrode for highly efficient CO 2 electrolysis in symmetrical solid oxide electrolysis cells
inferredcites →https://doi.org/10.1039/c9ta03065dopenalex-snapshot
In situ exsolved FeNi 3 nanoparticles on nickel doped Sr 2 Fe 1.5 Mo 0.5 O 6−δ perovskite for efficient electrochemical CO 2 reduction reaction
inferredcites →https://doi.org/10.1039/c9ta07689aopenalex-snapshot
Sr 2 Fe 1.4 Mn 0.1 Mo 0.5 O 6−δ perovskite cathode for highly efficient CO 2 electrolysis
inferredcites →https://doi.org/10.1039/d0ta06356hopenalex-snapshot
An innovative approach to design SOFC air electrode materials: high entropy La 1−x Sr x (Co,Cr,Fe,Mn,Ni)O 3−δ ( x = 0, 0.1, 0.2, 0.3) perovskites synthesized by the sol–gel method
inferredcites →https://doi.org/10.1039/d0ta09585kopenalex-snapshot
Ruddlesden–Popper oxide SrEu 2 Fe 2 O 7 as a promising symmetrical electrode for pure CO 2 electrolysis
inferredcites →https://doi.org/10.1039/d1ta06196hopenalex-snapshot
Antimony doping to greatly enhance the electrocatalytic performance of Sr 2 Fe 1.5 Mo 0.5 O 6− δ perovskite as a ceramic anode for solid oxide fuel cells
inferredcites →https://doi.org/10.1039/d1ta07275gopenalex-snapshot
Tailoring high-temperature stability and electrical conductivity of high entropy lanthanum manganite for solid oxide fuel cell cathodes
inferredcites →https://doi.org/10.1103/physrevb.50.17953openalex-snapshot
Projector augmented-wave method
inferredcites →https://doi.org/10.1103/physrevb.54.11169openalex-snapshot
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
inferredcites →https://doi.org/10.1103/physrevb.59.1758openalex-snapshot
From ultrasoft pseudopotentials to the projector augmented-wave method
inferredcites →https://doi.org/10.1103/physrevlett.77.3865openalex-snapshot
Generalized Gradient Approximation Made Simple
inferredcites →https://doi.org/10.1126/sciadv.aar5100openalex-snapshot
Highly efficient electrochemical reforming of CH 4 /CO 2 in a solid oxide electrolyser
inferredcites →https://doi.org/10.1149/1.2943664openalex-snapshot
Efficient Reduction of CO[sub 2] in a Solid Oxide Electrolyzer
inferredcites →https://doi.org/10.1149/2.0351802jesopenalex-snapshot
Direct Electrolysis of CO 2 in Symmetrical Solid Oxide Electrolysis Cell Based on La 0.6 Sr 0.4 Fe 0.8 Ni 0.2 O 3-δ Electrode

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

inferred← citeshttps://doi.org/10.2139/ssrn.4764798openalex-extracted
A Symmetrical Solid Oxide Electrolysis Cell Supported by Nanostructured Perovskite Electrodes for Co2 Electrolysis
inferred← citeshttps://doi.org/10.1002/adfm.202403922openalex-snapshot
In Situ Exsolution of Quaternary Alloy Nanoparticles for CO2‐CO Mutual Conversion Using Reversible Solid Oxide Cells
inferred← citeshttps://doi.org/10.1002/adfm.202411216openalex-snapshot
An Active and Stable High‐Entropy Ruddlesden‐Popper Type La1.4Sr0.6Co0.2Fe0.2Ni0.2Mn0.2Cu0.2O4±δ Oxygen Electrode for Reversible Solid Oxide Cells
inferred← citeshttps://doi.org/10.1002/adfm.202411622openalex-snapshot
Recent Progress in Sr 2 Fe 1.5 Mo 0.5 O 6‐δ ‐Based Multifunctional Materials for Energy Conversion and Storage
inferred← citeshttps://doi.org/10.1002/adma.202312119openalex-snapshot
A High‐Entropy Layered Perovskite Coated with In Situ Exsolved Core‐Shell CuFe@FeO x Nanoparticles for Efficient CO 2 Electrolysis
inferred← citeshttps://doi.org/10.1002/adma.202512310openalex-snapshot
Single‐Atom Anchored on Perovskite With Strong Metal‐Oxide Interaction for Efficient High Temperature CO 2 Electrolysis
inferred← citeshttps://doi.org/10.1002/adma.202521863openalex-snapshot
A‐Site High‐Entropy Engineering of Oxygen Electrode: A Promising Route to Durable and Active Reversible Solid Oxide Cells
inferred← citeshttps://doi.org/10.1002/adma.75331openalex-snapshot
High‐Entropy Perovskites for Solid Oxide Cells: Mechanistic Insights to Practical Applications
inferred← citeshttps://doi.org/10.1002/cssc.70851openalex-snapshot
Beyond Single‐Active Sites: The Emergence of High‐Entropy Perovskites in Energy and Environment Catalysis
inferred← citeshttps://doi.org/10.1002/eem2.70128openalex-snapshot
Dopant Engineering in Perovskite Cathodes for Efficient CO 2 Electrolysis
inferred← citeshttps://doi.org/10.1007/s12598-024-03119-4openalex-snapshot
Enhanced stability of perovskite cathode via entropy engineering for CO 2 electrolysis
inferred← citeshttps://doi.org/10.1007/s12613-025-3201-zopenalex-snapshot
Synergistic multielement effect at the B-site of high entropy double perovskite oxide: A promising fuel electrode for efficient co-electrolysis of H2O and CO2
inferred← citeshttps://doi.org/10.1016/j.apcatb.2025.125812openalex-snapshot
Rational engineering of symmetrical perovskite electrodes with alloy@FeOx dual-active centers for efficient methane-assisted CO2 electrolysis
inferred← citeshttps://doi.org/10.1016/j.apsusc.2026.166835openalex-snapshot
Sinter‑resistant cathodes via vapor‑phase precursor migration for stable high-temperature CO2 electrolysis
inferred← citeshttps://doi.org/10.1016/j.cej.2025.165404openalex-snapshot
Perovskite-socketed FeCoNiCu quaternary alloy nanoparticles for efficient CO2 reduction in solid oxide electrolyzer
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Bismuth-induced exsolution in a durable and high-performance fuel electrode for reversible solid oxide cells
inferred← citeshttps://doi.org/10.1016/j.ceja.2026.101117openalex-snapshot
Exploring the parametric and electrolyte-dependent behavior of SOEC for syngas production via CO2/H2O electrolysis: A 3D multi-physics study
inferred← citeshttps://doi.org/10.1016/j.ceramint.2025.03.338openalex-snapshot
Development of high-performance functional electrode using Cr stabilized La0.6Sr0.4FeO3-based perovskite oxide for revisable solid oxide cells
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Electrolyte influence on electrode activity evaluation in lab-scale solid oxide electrolyzers for carbon dioxide reduction (CO2-SOECs)
inferred← citeshttps://doi.org/10.1016/j.ces.2024.120034openalex-snapshot
Medium-entropy perovskite Pr0.4Ba0.2Ca0.2La0.2Co0.2Fe0.8O3 as a promising bifunctional electrocatalyst for electrochemical energy conversion device
inferred← citeshttps://doi.org/10.1016/j.checat.2025.101604openalex-snapshot
Orbital-engineered high-entropy perovskite cathode for cascaded CO2 electrolysis
inferred← citeshttps://doi.org/10.1016/j.electacta.2025.146749openalex-snapshot
Enhanced CO2 electrolysis performance of medium-entropy perovskite cathode through in situ exsolution of Co nanoparticles
inferred← citeshttps://doi.org/10.1016/j.esci.2026.100635openalex-snapshot
Efficient tandem electrocatalysis: in situ exsolved Pd nanoparticles driving concurrent CO2 reduction and ethane oxidative dehydrogenation
inferred← citeshttps://doi.org/10.1016/j.ijhydene.2024.11.068openalex-snapshot
In situ exsolved FeTe alloy nanoparticles of a double perovskite cathode for efficient CO2 electrolysis
inferred← citeshttps://doi.org/10.1016/j.ijhydene.2025.01.298openalex-snapshot
A robust high-entropy perovskite fuel electrode for direct CO2 electrolysis on air electrode-supported solid oxide electrolysis cells
inferred← citeshttps://doi.org/10.1016/j.jallcom.2024.177585openalex-snapshot
Entropy engineering strategies for optimizing solid oxide cell air electrode performance: A review
inferred← citeshttps://doi.org/10.1016/j.jcis.2024.11.161openalex-snapshot
Entropy-engineered perovskite cathodes: A novel approach for efficient and durable CO2 electrolysis
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Progress in modification strategies of perovskite oxides for CO2 electrolysis in solid oxide electrolysis cells
inferred← citeshttps://doi.org/10.1016/j.jechem.2024.05.030openalex-snapshot
Novel medium entropy perovskite oxide Sr(FeCoNiMo)1/4O3− for zinc-air battery cathode
inferred← citeshttps://doi.org/10.1016/j.jechem.2024.12.009openalex-snapshot
High-entropy materials for solid oxide cells: Synthesis, applications, and prospects
inferred← citeshttps://doi.org/10.1016/j.jil.2025.100163openalex-snapshot
Enhanced stability and optical performance of MAPbI3 perovskite films through B4PBF4 ionic liquid integration: A route to durable photovoltaics
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A symmetrical solid oxide electrolysis cell supported by nanostructured electrodes for highly efficient CO2 electrolysis
inferred← citeshttps://doi.org/10.1016/j.jpowsour.2025.236498openalex-snapshot
Synergistically boosting high-temperature CO2 electrolysis performance via high-entropy engineering and anion doping strategy
inferred← citeshttps://doi.org/10.1016/j.jpowsour.2026.240291openalex-snapshot
Quasi-symmetrical perovskite electrodes of solid oxide electrolysis cells for energy-efficient CO2 electrolysis
inferred← citeshttps://doi.org/10.1016/j.jssc.2025.125565openalex-snapshot
Targeting a medium-entropy perovskite: Single-crystal growth and phase competition in the PbSc1/2Ta1/2O3–PbIn1/2Nb1/2O3–PbIn1/2Ta1/2O3–PbSc1/2Nb1/2O3 system
inferred← citeshttps://doi.org/10.1016/j.seppur.2024.128950openalex-snapshot
Enhancing CO2 electrolysis efficiency via in-situ exsolution in high-entropy perovskite electrodes
inferred← citeshttps://doi.org/10.1016/j.seppur.2025.135490openalex-snapshot
Nanofiber-architected SOEC cathodes with in situ exsolved metallic nanoparticles for efficient and robust high-temperature carbon dioxide reduction reaction
inferred← citeshttps://doi.org/10.1021/acsami.4c05465openalex-snapshot
Realizing Efficient Activity and High Conductivity of Perovskite Symmetrical Electrode by Vanadium Doping for CO 2 Electrolysis
inferred← citeshttps://doi.org/10.1021/acsnano.4c14279openalex-snapshot
Precise Regulation of In Situ Exsolution Components of Nanoparticles for Constructing Active Interfaces toward Carbon Dioxide Reduction
inferred← citeshttps://doi.org/10.1039/d4sc03306jopenalex-snapshot
Advancements and prospects of perovskite-based fuel electrodes in solid oxide cells for CO 2 electrolysis to CO
inferred← citeshttps://doi.org/10.1039/d4ta02372bopenalex-snapshot
Probing metal/high-entropy perovskite heterointerfaces for efficient and sustainable CO 2 electroreduction
inferred← citeshttps://doi.org/10.1039/d5nj01436kopenalex-snapshot
In situ exsolution of FeCo alloy nanoparticles for highly efficient CO 2 electrolysis
inferred← citeshttps://doi.org/10.1039/d5se01240fopenalex-snapshot
A critical review on the design strategies of SFM-based perovskite oxides for high-temperature CO 2 electrolysis in solid oxide electrolysis cells
inferred← citeshttps://doi.org/10.1039/d6ee02221aopenalex-snapshot
Electronic-structure descriptor-guided design of high-entropy perovskites for efficient CO 2 electrolysis
inferred← citeshttps://doi.org/10.1039/d6ta05594jopenalex-snapshot
Synergistic anion–cation co-doping in perovskite as a bifunctional cathode for high-performance reversible solid oxide cells
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Investigation of the Local Atomic Structure of Ordered Medium-entropy Perovskite PbSc1/4Fe1/4Nb1/4Ta1/4O3 by Mössbauer and XAFS Spectroscopy
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High-Entropy La0.2Pr0.2Sm0.2Nd0.2Sr0.2Co0.2Fe0.8O3 Air Electrode for Solid Oxide Electrolysis Cells
inferred← citeshttps://doi.org/10.1360/ssc-2025-0102openalex-snapshot
Research progress on high-entropy oxides as cathodes for solid oxide cells
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Enhanced Stability and Optical Performance of Mapbi₃ Perovskite Films Through B4pbf₄ Ionic Liquid Integration: A Route to Durable Photovoltaics
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Enhanced Gas-Sensing Behavior of ErFeO3-Based Material via Medium-Entropy Engineering and Applied Magnetic Fields
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The Study on the Electrochemical Efficiency of Yttrium-Doped High-Entropy Perovskite Cathodes for Proton-Conducting Fuel Cells
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