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Mechanism of Hydrocarbon Formation in Methane and Methanol Conversion over Copper-Containing Mordenite

https://doi.org/10.1021/acscatal.2c06312

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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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Understanding Methane Aromatization on a Zn‐Modified High‐Silica Zeolite

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Formation Mechanism of the First Carbon–Carbon Bond and the First Olefin in the Methanol Conversion into Hydrocarbons

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Initial Carbon–Carbon Bond Formation during the Early Stages of the Methanol‐to‐Olefin Process Proven by Zeolite‐Trapped Acetate and Methyl Acetate

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Extra‐Framework Aluminum‐Assisted Initial C−C Bond Formation in Methanol‐to‐Olefins Conversion on Zeolite H‐ZSM‐5

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Pathways of Methane Transformation over Copper‐Exchanged Mordenite as Revealed by In Situ NMR and IR Spectroscopy

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Carbonylation of Methanol on Metal–Acid Zeolites: Evidence for a Mechanism Involving a Multisite Active Center

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Methanol Behavior in Direct Methanol Fuel Cells

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Solid Catalysts for the Selective Low‐Temperature Oxidation of Methane to Methanol

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Conversion of Methanol to Hydrocarbons: How Zeolite Cavity and Pore Size Controls Product Selectivity

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Direct Observation of Cyclic Carbenium Ions and Their Role in the Catalytic Cycle of the Methanol‐to‐Olefin Reaction over Chabazite Zeolites

inferredcites →https://doi.org/10.1002/anie.201803279openalex-snapshot

Bridging the Gap between the Direct and Hydrocarbon Pool Mechanisms of the Methanol‐to‐Hydrocarbons Process

inferredcites →https://doi.org/10.1002/anie.202101628openalex-snapshot

Identification of Kinetic and Spectroscopic Signatures of Copper Sites for Direct Oxidation of Methane to Methanol

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Zeolite Surface Methoxy Groups as Key Intermediates in the Stepwise Conversion of Methane to Methanol

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Mechanism of Methanol‐to‐hydrocarbon Reaction over Zeolites: A solid‐state NMR Perspective

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Frontispiece: New Insight into the Hydrocarbon‐Pool Chemistry of the Methanol‐to‐Olefins Conversion over Zeolite H‐ZSM‐5 from GC‐MS, Solid‐State NMR Spectroscopy, and DFT Calculations

inferredcites →https://doi.org/10.1002/chem.202103984openalex-snapshot

Binding Interactions in Copper, Silver and Gold π‐Complexes

inferredcites →https://doi.org/10.1002/cssc.201200299openalex-snapshot

Oxidative Methane Upgrading

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Structurally Characterized Coinage‐Metal–Ethylene Complexes

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Dehydrogenation of methane on supported molybdenum oxides. Formation of benzene from methane

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Natural gas conversion to liquid fuels and chemicals: Where does it stand?

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Methanol to hydrocarbons reaction over Hβ zeolites studied by high resolution solid-state NMR spectroscopy: Carbenium ions formation and reaction mechanism

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Natural gas to synthesis gas – Catalysts and catalytic processes

inferredcites →https://doi.org/10.1016/j.micromeso.2023.112448openalex-snapshot

Propene transformation on Cu-modified ZSM-5 zeolite: Aromatization and oxidation

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Efficient methanol synthesis: Perspectives, technologies and optimization strategies

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1H and 13C MAS NMR studies of light alkanes activation over MFI zeolite modified by Zn vapour

inferredcites →https://doi.org/10.1016/j.ssnmr.2016.10.003openalex-snapshot

Methanol carbonylation over copper-modified mordenite zeolite: A solid-state NMR study

inferredcites →https://doi.org/10.1016/s0167-2991(08)64152-xopenalex-snapshot

Copper exchanged zeolites studied with 13C and 129Xe NMR of adsorbed carbon monoxide and xenon

inferredcites →https://doi.org/10.1016/s0360-0564(02)47006-xopenalex-snapshot

Hydrogen and synthesis gas by steam- and C02 reforming

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Methanol-to-hydrocarbons: catalytic materials and their behavior

inferredcites →https://doi.org/10.1016/s1387-1811(98)00320-5openalex-snapshot

Methanol-to-hydrocarbons: process technology

inferredcites →https://doi.org/10.1021/acs.accounts.7b00354openalex-snapshot

Novel Strategies for the Production of Fuels, Lubricants, and Chemicals from Biomass

inferredcites →https://doi.org/10.1021/acs.inorgchem.9b03462openalex-snapshot

Methane Activation on H-ZSM-5 Zeolite with Low Copper Loading. The Nature of Active Sites and Intermediates Identified with the Combination of Spectroscopic Methods

inferredcites →https://doi.org/10.1021/acs.jpcc.0c00311openalex-snapshot

Nature of the Surface Intermediates Formed from Methane on Cu-ZSM-5 Zeolite: A Combined Solid-State Nuclear Magnetic Resonance and Density Functional Theory Study

inferredcites →https://doi.org/10.1021/acs.jpcc.1c10026openalex-snapshot

Probing Acid Sites in MOR Zeolite Using Low-Temperature 13C Solid-State NMR Spectroscopy of Adsorbed Carbon Monoxide

inferredcites →https://doi.org/10.1021/acscatal.1c00543openalex-snapshot

Effect of the Co-cation on Cu Speciation in Cu-Exchanged Mordenite and ZSM-5 Catalysts for the Oxidation of Methane to Methanol

inferredcites →https://doi.org/10.1021/acscatal.1c02547openalex-snapshot

Methane Transformation over Copper-Exchanged Zeolites: From Partial Oxidation to C–C Coupling and Formation of Hydrocarbons

inferredcites →https://doi.org/10.1021/acscatal.2c05299openalex-snapshot

Structure of Selective and Nonselective Dicopper (II) Sites in CuMFI for Methane Oxidation to Methanol

inferredcites →https://doi.org/10.1021/acscatal.6b00428openalex-snapshot

Strategies for the Direct Catalytic Valorization of Methane Using Heterogeneous Catalysis: Challenges and Opportunities

inferredcites →https://doi.org/10.1021/acscatal.8b02385openalex-snapshot

Evolution of C–C Bond Formation in the Methanol-to-Olefins Process: From Direct Coupling to Autocatalysis

inferredcites →https://doi.org/10.1021/acscatal.9b01534openalex-snapshot

Methane-to-Methanol: Activity Descriptors in Copper-Exchanged Zeolites for the Rational Design of Materials

inferredcites →https://doi.org/10.1021/acscatal.9b02898openalex-snapshot

Mechanistic Insights on the Direct Conversion of Methane into Methanol over Cu/Na–ZSM-5 Zeolite: Evidence from EPR and Solid-State NMR

inferredcites →https://doi.org/10.1021/acscentsci.6b00139openalex-snapshot

Catalytic Oxidation of Methane into Methanol over Copper-Exchanged Zeolites with Oxygen at Low Temperature

inferredcites →https://doi.org/10.1021/acsearthspacechem.8b00214openalex-snapshot

13C Nuclear Magnetic Resonance Spectroscopy of Methane and Carbon Dioxide in a Natural Shale

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A comprehensive mechanism for the Fischer-Tropsch synthesis

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Solid-State NMR Investigation of the Alkylation of Toluene with Methanol over Basic Zeolite X

inferredcites →https://doi.org/10.1021/ja00117a032openalex-snapshot

NMR Observation of the Koch Reaction in Zeolite H-ZSM-5 under Mild Conditions

inferredcites →https://doi.org/10.1021/ja00157a004openalex-snapshot

Solid-state NMR studies of the shape-selective catalytic conversion of methanol into gasoline on zeolite ZSM-5

inferredcites →https://doi.org/10.1021/ja0304244openalex-snapshot

Evidence for an Initiation of the Methanol-to-Olefin Process by Reactive Surface Methoxy Groups on Acidic Zeolite Catalysts

inferredcites →https://doi.org/10.1021/ja036172oopenalex-snapshot

Sorptive Reconstruction of the CuAlCl4 Framework upon Reversible Ethylene Binding

inferredcites →https://doi.org/10.1021/ja047158uopenalex-snapshot

Selective Oxidation of Methane by the Bis(μ-oxo)dicopper Core Stabilized on ZSM-5 and Mordenite Zeolites

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On the Reactivity of Surface Methoxy Species in Acidic Zeolites

inferredcites →https://doi.org/10.1021/ja406978qopenalex-snapshot

Mechanistic Insight into the Formation of Acetic Acid from the Direct Conversion of Methane and Carbon Dioxide on Zinc-Modified H–ZSM-5 Zeolite

inferredcites →https://doi.org/10.1021/ja5106927openalex-snapshot

Methane to Acetic Acid over Cu-Exchanged Zeolites: Mechanistic Insights from a Site-Specific Carbonylation Reaction

inferredcites →https://doi.org/10.1021/ja994103xopenalex-snapshot

Roles for Cyclopentenyl Cations in the Synthesis of Hydrocarbons from Methanol on Zeolite Catalyst HZSM-5

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On the Mechanism Underlying the Direct Conversion of Methane to Methanol by Copper Hosted in Zeolites; Braiding Cu K-Edge XANES and Reactivity Studies

inferredcites →https://doi.org/10.1021/jacs.8b08071openalex-snapshot

The Nuclearity of the Active Site for Methane to Methanol Conversion in Cu-Mordenite: A Quantitative Assessment

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Role of Surface Methoxy Species in the Conversion of Methanol to Dimethyl Ether on Acidic Zeolites Investigated by in Situ Stopped-Flow MAS NMR Spectroscopy

inferredcites →https://doi.org/10.1021/jp4006795openalex-snapshot

Methane Activation and Transformation on Ag/H-ZSM-5 Zeolite Studied with Solid-State NMR

inferredcites →https://doi.org/10.1021/jp8067766openalex-snapshot

Methane Activation over Zn-Modified MFI Zeolite: NMR Evidence for Zn−Methyl Surface Species Formation

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Direct observation of shape selectivity in zeolite ZSM-5 by magic-angle-spinning NMR

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Recent trends and fundamental insights in the methanol-to-hydrocarbons process

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Homoleptic Cu–phosphorus and Cu–ethene complexes

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Insights into reaction mechanisms in heterogeneous catalysis revealed by in situ NMR spectroscopy

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Room temperature activation of methane over Zn modified H-ZSM-5 zeolites: Insight from solid-state NMR and theoretical calculations

inferredcites →https://doi.org/10.1039/c5cs00304kopenalex-snapshot

The formation and degradation of active species during methanol conversion over protonated zeotype catalysts

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Methanol conversion on ZSM-22, ZSM-35 and ZSM-5 zeolites: effects of 10-membered ring zeolite structures on methylcyclopentenyl cations and dual cycle mechanism

inferredcites →https://doi.org/10.1039/c7cs00709dopenalex-snapshot

Active sites and mechanisms in the direct conversion of methane to methanol using Cu in zeolitic hosts: a critical examination

inferredcites →https://doi.org/10.1039/c8cc03921fopenalex-snapshot

Revisiting copper reduction in zeolites: the impact of autoreduction and sample synthesis procedure

inferredcites →https://doi.org/10.1039/c8cy01055bopenalex-snapshot

Effect of Brønsted acid sites on the direct conversion of methane into methanol over copper-exchanged mordenite

inferredcites →https://doi.org/10.1039/c9cy01711aopenalex-snapshot

Kinetic study and effect of water on methane oxidation to methanol over copper-exchanged mordenite

inferredcites →https://doi.org/10.1039/c9ra02280eopenalex-snapshot

Identification of different carbenium ion intermediates in zeolites with identical chabazite topology via 13 C– 13 C through-bond NMR correlations

inferredcites →https://doi.org/10.1039/d1cc00397fopenalex-snapshot

Selective methanethiol-to-olefins conversion over HSSZ-13 zeolite

inferredcites →https://doi.org/10.1063/1.470372openalex-snapshot

Heteronuclear decoupling in rotating solids

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The Different Catalytic Routes for Methane Valorization: An Assessment of Processes for Liquid Fuels

inferredcites →https://doi.org/10.1126/science.1253150openalex-snapshot

Direct, Nonoxidative Conversion of Methane to Ethylene, Aromatics, and Hydrogen

inferredcites →https://doi.org/10.1126/science.264.5165.1563openalex-snapshot

Methane to Ethylene with 85 Percent Yield in a Gas Recycle Electrocatalytic Reactor-Separator

inferredcites →https://doi.org/10.1126/science.280.5363.560openalex-snapshot

Platinum Catalysts for the High-Yield Oxidation of Methane to a Methanol Derivative

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Selective anaerobic oxidation of methane enables direct synthesis of methanol

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

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An Efficient Methanol Upgrading of Methane Dehydro-Aromatization Route Over Mo-Zsm-5/Zsm-11 Intergrown Zeolites

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Selective Oxidative Dehydrogenation of Ethane and Propane over Copper‐Containing Mordenite: Insights into Reaction Mechanism and Product Protection

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Redox and Kinetic Properties of Composition‐Dependent Active Sites in Copper‐Exchanged Chabazite for Direct Methane‐to‐Methanol Oxidation

inferred← citeshttps://doi.org/10.1002/anie.202309180openalex-snapshot

Selective Oxidative Dehydrogenation of Ethane and Propane over Copper‐Containing Mordenite: Insights into Reaction Mechanism and Product Protection

inferred← citeshttps://doi.org/10.1002/anie.202411662openalex-snapshot

Redox and Kinetic Properties of Composition‐Dependent Active Sites in Copper‐Exchanged Chabazite for Direct Methane‐to‐Methanol Oxidation

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Methane to Methanol Transformation on Cu2+/H‐ZSM‐5 Zeolite. Characterization of Copper State and Mechanism of the Reaction

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Direct partial oxidation of low-concentration methane to methanol with copper-based clay catalysts

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