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Enantioselective epoxidation of unfunctionalized olefins catalyzed by salen manganese complexes

https://doi.org/10.1021/ja00163a052
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A Possible Mechanism for Enantioselectivity in the Chiral Epoxidation of Olefins with [Mn(salen)] Catalysts
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Rate Enhancement and Enantioselectivity of the Jacobsen-Katsuki Epoxidation: The Significance of the Sixth Coordination Site This work was made possible through generous allocation of computer resources by the OIT at Notre Dame, the National Computational Science Alliance and the Competence Center…
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meso‐Epoxide in der asymmetrischen Synthese: enantioselektive öffnung durch Nucleophile in Gegenwart von chiralen Lewis‐Säuren
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Highly Enantioselective Epoxidation of Styrenes Catalyzed by Proline‐Derived C1‐Symmetric Titanium(Salan) Complexes
inferred← citeshttps://doi.org/10.1002/ange.200905332openalex-snapshot
Asymmetrische Gegenanion‐vermittelte Übergangsmetallkatalyse: enantioselektive Epoxidierung von Alkenen mit Mangan(III)‐Salen‐Phosphatkomplexen
inferred← citeshttps://doi.org/10.1002/ange.201005577openalex-snapshot
One‐Pot Synthesis of Chiral α‐Substituted β,γ‐Epoxy Aldehyde Derivatives through an Asymmetric Aldol Reaction of Chloroacetaldehyde
inferred← citeshttps://doi.org/10.1002/ange.201102028openalex-snapshot
Snapshots of Complete Nitrogen Atom Transfer from an Iron(IV) Nitrido Complex
inferred← citeshttps://doi.org/10.1002/ange.201104086openalex-snapshot
Actuation of Asymmetric Cyclopropanation Catalysts: Reversible Single‐Crystal to Single‐Crystal Reduction of Metal–Organic Frameworks
inferred← citeshttps://doi.org/10.1002/ange.201205343openalex-snapshot
Asymmetrische Gegenanionen‐vermittelte Katalyse: Konzept, Definition und Anwendungen
inferred← citeshttps://doi.org/10.1002/ange.201209355openalex-snapshot
Enantioselective Synthesis of Epoxides Having a Tetrasubstituted Trifluoromethylated Carbon Center: Methylhydrazine‐Induced Aerobic Epoxidation of β,β‐Disubstituted Enones
inferred← citeshttps://doi.org/10.1002/ange.201301097openalex-snapshot
Manganese‐Catalyzed Oxidative Benzylic C–H Fluorination by Fluoride Ions
inferred← citeshttps://doi.org/10.1002/ange.201400241openalex-snapshot
Organokatalytische asymmetrische Epoxidierungen – Reaktionen, Mechanismen und Anwendungen
inferred← citeshttps://doi.org/10.1002/ange.201501271openalex-snapshot
Stereochemische Kommunikation innerhalb eines chiralen Ionenpaares
inferred← citeshttps://doi.org/10.1002/ange.201602433openalex-snapshot
Eric N. Jacobsen
inferred← citeshttps://doi.org/10.1002/ange.201612462openalex-snapshot
Enantioselektive Chemo‐ und Biokatalyse: Partner in der Retrosynthese
inferred← citeshttps://doi.org/10.1002/ange.201700632openalex-snapshot
Rhodium‐Catalyzed Enantioselective Isomerization of meso‐Oxabenzonorbornadienes to 1,2‐Naphthalene Oxides
inferred← citeshttps://doi.org/10.1002/ange.201704184openalex-snapshot
Mechanism‐Based Enantiodivergence in Manganese Reduction Catalysis: A Chiral Pincer Complex for the Highly Enantioselective Hydroboration of Ketones
inferred← citeshttps://doi.org/10.1002/ange.201706682openalex-snapshot
Direct and Stereospecific [3+2] Synthesis of Pyrrolidines from Simple Unactivated Alkenes
inferred← citeshttps://doi.org/10.1002/ange.201812432openalex-snapshot
Biomimetic and Biocatalytic Synthesis of Bruceol
inferred← citeshttps://doi.org/10.1002/ange.201814457openalex-snapshot
Fluorierung von C‐H‐Bindungen: Entwicklungen und Perspektiven
inferred← citeshttps://doi.org/10.1002/ange.202000016openalex-snapshot
Asymmetric Electrochemical Transformations
inferred← citeshttps://doi.org/10.1002/ange.202002844openalex-snapshot
A General Regioselective Synthesis of Alcohols by Cobalt‐Catalyzed Hydrogenation of Epoxides
inferred← citeshttps://doi.org/10.1002/ange.202101439openalex-snapshot
Concise Asymmetric Syntheses of Streptazone A and Abikoviromycin**
inferred← citeshttps://doi.org/10.1002/ange.202105562openalex-snapshot
Enantioselective Synthesis of Spiro‐oxiranes: An Asymmetric Addition/Aldol/Spirocyclization Domino Cascade
inferred← citeshttps://doi.org/10.1002/ange.202309263openalex-snapshot
Iridium(III)‐Catalyzed Intermolecular C(sp3)‐H Amidation for the Synthesis of Chiral 1,2‐Diamines
inferred← citeshttps://doi.org/10.1002/ange.202400177openalex-snapshot
Manganese(I)‐Catalyzed Enantioselective C(sp2)−C(sp3) Bond‐Forming for the Synthesis of Skipped Dienes with Synergistic Aminocatalysis
inferred← citeshttps://doi.org/10.1002/ange.202405911openalex-snapshot
Stereoconvergent Approach to the Enantioselective Construction of α‐Quaternary Alcohols by Radical Epoxide Allylation
inferred← citeshttps://doi.org/10.1002/ange.202418147openalex-snapshot
Current‐Regulated Selective Nickel‐Catalyzed Electroreductive Cross‐Electrophile Carbonylation to β/γ‐Hydroxy Ketones
inferred← citeshttps://doi.org/10.1002/ange.202503054openalex-snapshot
Engineering 2‐Deoxy‐D‐ribose‐5‐phosphate Aldolase for anti ‐ and syn ‐Selective Epoxidations of α , β ‐Unsaturated Aldehydes
inferred← citeshttps://doi.org/10.1002/anie.199101031openalex-snapshot
Stereoselective Synthesis of Vicinal Diamines
inferred← citeshttps://doi.org/10.1002/anie.199104031openalex-snapshot
Catalytic Enantioselective Epoxidations of Simple Olefins
inferred← citeshttps://doi.org/10.1002/anie.199211791openalex-snapshot
meso Epoxides in Asymmetric Synthesis: Enantioselective Opening by Nucleophiles in the Presence of Chiral Lewis Acids
inferred← citeshttps://doi.org/10.1002/anie.199404971openalex-snapshot
Nitrogen Donors in Organometallic Chemistry and Homogeneous Catalysis
inferred← citeshttps://doi.org/10.1002/anie.199524431openalex-snapshot
Synthetic Aspects of Metal‐Catalyzed Oxidations of Amines and Related Reactions
inferred← citeshttps://doi.org/10.1002/anie.199617251openalex-snapshot
Asymmetric Epoxidation of Enones With Oxygen in the Presence of Diethylzinc and (R,R)‐N‐Methylpseudoephedrine
inferred← citeshttps://doi.org/10.1002/anie.199624871openalex-snapshot
Highly Diastereoselective Synthesis and Epoxidation of Chiral 1,2‐Dihydronaphthalenes
inferred← citeshttps://doi.org/10.1002/anie.199717181openalex-snapshot
Direct Proof for OMnv (salen) Complexes
inferred← citeshttps://doi.org/10.1002/anie.199717201openalex-snapshot
On the Viability of Oxametallacyclic Intermediates in the (salen)Mn‐Catalyzed Asymmetric Epoxidation
inferred← citeshttps://doi.org/10.1002/anie.199720601openalex-snapshot
The Jacobsen–Katsuki Epoxidation and Its Controversial Mechanism
inferred← citeshttps://doi.org/10.1002/anie.200290024openalex-snapshot
New Ferrocenyl Ligands with Broad Applications in Asymmetric Catalysis
inferred← citeshttps://doi.org/10.1002/anie.200300599openalex-snapshot
Industrial Methods for the Production of Optically Active Intermediates
inferred← citeshttps://doi.org/10.1002/anie.200300629openalex-snapshot
Functional Models for Rhodium‐Mediated Olefin‐Oxygenation Catalysis
inferred← citeshttps://doi.org/10.1002/anie.200601742openalex-snapshot
Enantioselective Oxidation of Olefins Catalyzed by a Chiral Bishydroxamic Acid Complex of Molybdenum
inferred← citeshttps://doi.org/10.1002/anie.200700949openalex-snapshot
Titanium‐Catalyzed Asymmetric Epoxidation of Non‐Activated Olefins with Hydrogen Peroxide
inferred← citeshttps://doi.org/10.1002/anie.200703771openalex-snapshot
Superhyperfine Interaction in [MnF 6 ] 3−
inferred← citeshttps://doi.org/10.1002/anie.200704185openalex-snapshot
Asymmetric Counteranion‐Directed Catalysis for the Epoxidation of Enals
inferred← citeshttps://doi.org/10.1002/anie.200803238openalex-snapshot
Catalytic Asymmetric Hydroperoxidation of α,β‐Unsaturated Ketones: An Approach to Enantiopure Peroxyhemiketals, Epoxides, and Aldols
inferred← citeshttps://doi.org/10.1002/anie.200900600openalex-snapshot
Epoxide‐Opening Cascades in the Synthesis of Polycyclic Polyether Natural Products
inferred← citeshttps://doi.org/10.1002/anie.200900682openalex-snapshot
A Sequential O‐Nitrosoaldol and Grignard Addition Process: An Enantio‐ and Diastereoselective Entry to Chiral 1,2‐Diols
inferred← citeshttps://doi.org/10.1002/anie.200903567openalex-snapshot
Highly Enantioselective Epoxidation of Styrenes Catalyzed by Proline‐Derived C1‐Symmetric Titanium(Salan) Complexes
inferred← citeshttps://doi.org/10.1002/anie.200905332openalex-snapshot
Asymmetric Counteranion‐Directed Transition‐Metal Catalysis: Enantioselective Epoxidation of Alkenes with Manganese(III) Salen Phosphate Complexes
inferred← citeshttps://doi.org/10.1002/anie.201005577openalex-snapshot
One‐Pot Synthesis of Chiral α‐Substituted β,γ‐Epoxy Aldehyde Derivatives through an Asymmetric Aldol Reaction of Chloroacetaldehyde
inferred← citeshttps://doi.org/10.1002/anie.201102028openalex-snapshot
Snapshots of Complete Nitrogen Atom Transfer from an Iron(IV) Nitrido Complex
inferred← citeshttps://doi.org/10.1002/anie.201104086openalex-snapshot
Actuation of Asymmetric Cyclopropanation Catalysts: Reversible Single‐Crystal to Single‐Crystal Reduction of Metal–Organic Frameworks
inferred← citeshttps://doi.org/10.1002/anie.201205343openalex-snapshot
Asymmetric Counteranion‐Directed Catalysis: Concept, Definition, and Applications
inferred← citeshttps://doi.org/10.1002/anie.201209355openalex-snapshot
Enantioselective Synthesis of Epoxides Having a Tetrasubstituted Trifluoromethylated Carbon Center: Methylhydrazine‐Induced Aerobic Epoxidation of β,β‐Disubstituted Enones
inferred← citeshttps://doi.org/10.1002/anie.201301097openalex-snapshot
Manganese‐Catalyzed Oxidative Benzylic C–H Fluorination by Fluoride Ions
inferred← citeshttps://doi.org/10.1002/anie.201400241openalex-snapshot
Asymmetric Organocatalytic Epoxidations: Reactions, Scope, Mechanisms, and Applications
inferred← citeshttps://doi.org/10.1002/anie.201501271openalex-snapshot
Stereochemical Communication within a Chiral Ion Pair Catalyst
inferred← citeshttps://doi.org/10.1002/anie.201602433openalex-snapshot
Eric N. Jacobsen
inferred← citeshttps://doi.org/10.1002/anie.201612462openalex-snapshot
Enantioselective Chemo‐ and Biocatalysis: Partners in Retrosynthesis
inferred← citeshttps://doi.org/10.1002/anie.201700632openalex-snapshot
Rhodium‐Catalyzed Enantioselective Isomerization of meso‐Oxabenzonorbornadienes to 1,2‐Naphthalene Oxides
inferred← citeshttps://doi.org/10.1002/anie.201704184openalex-snapshot
Mechanism‐Based Enantiodivergence in Manganese Reduction Catalysis: A Chiral Pincer Complex for the Highly Enantioselective Hydroboration of Ketones
inferred← citeshttps://doi.org/10.1002/anie.201706682openalex-snapshot
Direct and Stereospecific [3+2] Synthesis of Pyrrolidines from Simple Unactivated Alkenes
inferred← citeshttps://doi.org/10.1002/anie.201812432openalex-snapshot
Biomimetic and Biocatalytic Synthesis of Bruceol
inferred← citeshttps://doi.org/10.1002/anie.201814457openalex-snapshot
The Fluorination of C−H Bonds: Developments and Perspectives
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