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Scope and Mechanism of the Iridium-Catalyzed Cleavage of Alkyl Ethers with Triethylsilane

https://doi.org/10.1021/ja806419h
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Divergent Synthesis of Chromones and Chromanones from Diketones Using an Agotf/[Si]H System by Switching Hydrosilanes
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Ionic and Organometallic‐Catalyzed Organosilane Reductions
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Homogeneous Transition‐Metal‐Catalyzed C–O Bond Activation
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Catalytic Depolymerization of Plastic Waste
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Si ─ H Bond Activation by Transition‐Metal L ewis Acids
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Chemoselective Ruthenium‐Catalyzed Reduction of Acid Chlorides to Aldehydes with Dimethylphenylsilane
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Preferential α‐Hydrosilylation of Terminal Alkynes by Bis‐N‐Heterocyclic Carbene Rhodium(III) Catalysts
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Practical Conversion of Chlorosilanes into Alkoxysilanes without Generating HCl
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Si‐H‐Bindungsaktivierung: Parallelen der Lewis‐Säure‐Katalyse mit Brookharts Iridium(III)‐Pincerkomplex und B(C6F5)3
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Metal‐Free Deoxygenation of Carbohydrates
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Bor‐katalysierte regioselektive Desoxygenierung von terminalen 1,2‐Diolen zu 2‐Alkanolen durch die strategische Bildung eines cyclischen Siloxan‐Intermediates
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Elektrophile Aktivierung von Silicium‐Wasserstoff‐ Bindungen in katalytischen Hydrosilierungen
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Selective C−O Bond Cleavage of Sugars with Hydrosilanes Catalyzed by Piers’ Borane Generated In Situ
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Bis(perchlorocatecholato)silan – eine neutrale Silicium‐Lewis‐Supersäure
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Reversible Silylium Transfer between P‐H and Si‐H Donors
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Kohlenstoff‐Basierte Schwach Koordinierende Anionen: Molekulares Design, Synthese und Anwendung
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Catalytic Hydrosilylation Deoxygenation: Synthesizing Polysiloxanes While Upcycling Polymers to Alkanes
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Practical Conversion of Chlorosilanes into Alkoxysilanes without Generating HCl
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SiH Bond Activation: Bridging Lewis Acid Catalysis with Brookhart’s Iridium(III) Pincer Complex and B(C6F5)3
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Metal‐Free Deoxygenation of Carbohydrates
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Boron‐Catalyzed Regioselective Deoxygenation of Terminal 1,2‐Diols to 2‐Alkanols Enabled by the Strategic Formation of a Cyclic Siloxane Intermediate
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Electrophilic Activation of Silicon–Hydrogen Bonds in Catalytic Hydrosilations
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Selective C−O Bond Cleavage of Sugars with Hydrosilanes Catalyzed by Piers’ Borane Generated In Situ
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Bis(perchlorocatecholato)silane—A Neutral Silicon Lewis Super Acid
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Reversible Silylium Transfer between P‐H and Si‐H Donors
inferred← citeshttps://doi.org/10.1002/anie.202405936openalex-snapshot
Carbon‐Based Weakly Coordinating Anions: Molecular Design, Synthesis and Applications
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Catalytic Hydrosilylation Deoxygenation: Synthesizing Polysiloxanes While Upcycling Polymers to Alkanes
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Catalytic Reduction of Cyclic Ethers with Hydrosilanes
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Outer‐Sphere Ionic Hydrosilylation Catalysis
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Efficient and Selective Hydrosilylation of Secondary and Tertiary Amides Catalyzed by an Iridium(III) Metallacycle: Development and Mechanistic Investigation
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Proton‐Transfer Reactions on Hexanuclear Platinum Clusters: Reversible Heterolytic Cleavage of H2 and CH Activation Affording a Linear, Cluster‐Containing Polymer
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Selective Hydrosilylation of Esters to Aldehydes Catalysed by Iridium(III) Metallacycles through Trapping of Transient Silyl Cations
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Is the R3Si Moiety in Metal–Silyl Complexes a Z ligand? An Answer from the Interaction Energy
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Highly Electrophilic Mononuclear Cationic Aluminium Alkoxide Complexes: Syntheses, Reactivity and Catalytic Applications
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Role of the Isolable Hydride Intermediate in the Hydrosilylation of Carbonyl Compounds Catalyzed by the High‐Valent Mono‐Oxido–Rhenium(V) Complex
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A Versatile Iridium(III) Metallacycle Catalyst for the Effective Hydrosilylation of Carbonyl and Carboxylic Acid Derivatives
inferred← citeshttps://doi.org/10.1002/ejoc.202001061openalex-snapshot
One‐Pot Controlled Reduction of Conjugated Amides by Sequential Double Hydrosilylation Catalyzed by an Iridium(III) Metallacycle
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Large‐scale preparation and labelling reactions of deuterated silanes
inferred← citeshttps://doi.org/10.1007/978-981-287-769-7_2openalex-snapshot
Homogeneous Catalysts for the Hydrodeoxygenation of Biomass-Derived Carbohydrate Feedstocks
inferred← citeshttps://doi.org/10.1007/bf03249092openalex-snapshot
Palladium chloride-catalyzed reductive cleavage of benzylic acetal, ketal and ether compounds with triethylsilane
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Review: Mechanism and multifunctional integration progress of self-healing polybenzoxazine
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Embedding Sustainability in Product and Process Development—The Role of Process Systems Engineers
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Synthetic Applications of C–O and C–E Bond Activation Reactions
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Modern mechanistic approaches for the depolymerization of commodity plastics via organometallic catalysis
inferred← citeshttps://doi.org/10.1016/j.ccr.2019.02.003openalex-snapshot
Non-classical hydrosilane mediated reductions promoted by transition metal complexes
inferred← citeshttps://doi.org/10.1016/j.eurpolymj.2024.113073openalex-snapshot
Combining Siloxane-Based polybenzoxazine with Poly(ethylene-co-vinyl acetate/hydroxyl) for tougher, more Stable, and Self-Healable materials
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A fluorene-based diphosphinite ligand, its Ni, Pd, Pt, Fe, Co and Zn complexes and the first structurally characterized diphosphinate metal chelates
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Cleavage of the βO4 linkage of lignin using group 8 pincer complexes: A DFT study
inferred← citeshttps://doi.org/10.1016/j.molcata.2015.01.019openalex-snapshot
A computational study on high-valent mono-oxo-rhenium(V) complex-catalyzed hydrosilylation of carbonyls: What a difference an oxo ligand makes
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Regioselective hydrosilylation of terminal alkynes using pentamethylcyclopentadienyl iridium(III) metallacycle catalysts
inferred← citeshttps://doi.org/10.1016/j.tet.2018.05.078openalex-snapshot
DFT study on mechanism of carbonyl hydrosilylation catalyzed by high-valent molybdenum (IV) hydrides
inferred← citeshttps://doi.org/10.1016/j.tet.2024.134087openalex-snapshot
Divergent synthesis of chromones and chromanones from diketones using an AgOTf/[Si]H system by switching hydrosilanes
inferred← citeshttps://doi.org/10.1016/j.xcrp.2023.101341openalex-snapshot
Metal-catalyzed plastic depolymerization
inferred← citeshttps://doi.org/10.1021/acs.chemmater.2c02853openalex-snapshot
Polyolefins Vitrimers: Design Principles and Applications
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Silylium Ions: From Elusive Reactive Intermediates to Potent Catalysts
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Deducing Reaction Mechanism: A Guide for Students, Researchers, and Instructors
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Cobalt-Catalyzed Secondary Alkylation of Arenes and Olefins with Alkyl Ethers through the Cleavage of C(sp2)–H and C(sp3)–O Bonds
inferred← citeshttps://doi.org/10.1021/acs.jpca.5b00567openalex-snapshot
New Insights into Hydrosilylation of Unsaturated Carbon–Heteroatom (C═O, C═N) Bonds by Rhenium(V)–Dioxo Complexes
inferred← citeshttps://doi.org/10.1021/acs.macromol.6c00768openalex-snapshot
Synthesis of Alternating Silylether-Carbosilane Copolymers via Tandem Hydrosilylation–Condensation/Ring-Opening and Addition Polymerization
inferred← citeshttps://doi.org/10.1021/acs.organomet.1c00391openalex-snapshot
Light-Promoted Transfer of an Iridium Hydride in Alkyl Ether Cleavage
inferred← citeshttps://doi.org/10.1021/acs.organomet.1c00576openalex-snapshot
The Role of ( t Bu POCOP)Ir(I) and Iridium(III) Pincer Complexes in the Catalytic Hydrogenolysis of Silyl Triflates into Hydrosilanes
inferred← citeshttps://doi.org/10.1021/acs.organomet.4c00162openalex-snapshot
Pincer-Ligated Iridium Complexes with Low-Field Ancillary Ligands: Complexes of ( i Pr PCP)IrCl 2 and Comparison with ( i Pr PCP)IrHCl
inferred← citeshttps://doi.org/10.1021/acs.organomet.5b00958openalex-snapshot
Half-Sandwich Silane σ-Complexes of Ruthenium Supported by NHC Carbene
inferred← citeshttps://doi.org/10.1021/acs.organomet.6b00248openalex-snapshot
Evidence of a Donor–Acceptor (Ir–H)→SiR3Interaction in a Trapped Ir(III) Silane Catalytic Intermediate
inferred← citeshttps://doi.org/10.1021/acs.organomet.6b00347openalex-snapshot
Theoretical Study of Ir-Catalyzed Chemoselective C1–O Reduction of Glucose with Silane
inferred← citeshttps://doi.org/10.1021/acs.organomet.7b00688openalex-snapshot
Cationic (η5-C5Me4R)RhIII Complexes with Metalated Aryl Phosphines Featuring η4-Phosphorus plus Pseudo-Allylic Coordination
inferred← citeshttps://doi.org/10.1021/acs.orglett.6b02050openalex-snapshot
Diastereoselective B(C 6 F 5 ) 3 -Catalyzed Reductive Carbocyclization of Unsaturated Carbohydrates
inferred← citeshttps://doi.org/10.1021/acs.orglett.9b02572openalex-snapshot
Reductive C–O, C–N, and C–S Cleavage by a Zirconium Catalyzed Hydrometalation/β-Elimination Approach
inferred← citeshttps://doi.org/10.1021/acscatal.0c01718openalex-snapshot
Selectivity and Mechanism of Iridium-Catalyzed Cyclohexyl Methyl Ether Cleavage
inferred← citeshttps://doi.org/10.1021/acscatal.0c03180openalex-snapshot
In Situ Generation of Catalytically Relevant Nanoparticles from a Molecular Pincer Iridium Precatalyst during Polyol Deoxygenation
inferred← citeshttps://doi.org/10.1021/acscatal.3c00973openalex-snapshot
Deoxygenative Silylation of C(sp3)–O Bonds with Hydrosilane by Cooperative Catalysis of Gold Nanoparticles and Solid Acids
inferred← citeshttps://doi.org/10.1021/acscatal.7b02992openalex-snapshot
Positional Selectivity in the Hydrosilylative Partial Deoxygenation of Disaccharides by Boron Catalysts
inferred← citeshttps://doi.org/10.1021/acssuschemeng.8b01842openalex-snapshot
Depolymerization of Waste Plastics to Monomers and Chemicals Using a Hydrosilylation Strategy Facilitated by Brookhart’s Iridium(III) Catalyst
inferred← citeshttps://doi.org/10.1021/ic300010copenalex-snapshot
Mechanistic Aspects of Hydrosilylation Catalyzed by (ArN=)Mo(H)(Cl)(PMe3)3
inferred← citeshttps://doi.org/10.1021/ic302589bopenalex-snapshot
Synthesis, Structure, and Reactivity of Iridium(III) Complexes Containing a 4,6-Dimethyl-1,3-benzenediphenylimine Pincer Ligand
inferred← citeshttps://doi.org/10.1021/ic401931yopenalex-snapshot
POP-Pincer Silyl Complexes of Group 9: Rhodium versus Iridium
inferred← citeshttps://doi.org/10.1021/ja101583mopenalex-snapshot
Cationic Silane σ-Complexes of Ruthenium with Relevance to Catalysis
inferred← citeshttps://doi.org/10.1021/ja209567mopenalex-snapshot
Development and Mechanistic Investigation of a Highly Efficient Iridium(V) Silyl Complex for the Reduction of Tertiary Amides to Amines
inferred← citeshttps://doi.org/10.1021/ja305318copenalex-snapshot
An Efficient Iridium Catalyst for Reduction of Carbon Dioxide to Methane with Trialkylsilanes
inferred← citeshttps://doi.org/10.1021/ja3110494openalex-snapshot
Iridium-Catalyzed Hydrosilylative Reduction of Glucose to Hexane(s)
inferred← citeshttps://doi.org/10.1021/ja404655vopenalex-snapshot
Dehydrocoupling Reactions of Dimethylamine-Borane by Pt(II) Complexes: A New Mechanism Involving Deprotonation of Boronium Cations
inferred← citeshttps://doi.org/10.1021/ja404910hopenalex-snapshot
Silane–Isocyanide Coupling Involving 1,1-Insertion of XylNC into the Si–H Bond of a σ-Silane Ligand
inferred← citeshttps://doi.org/10.1021/ja503254fopenalex-snapshot
Insight into the Mechanism of Carbonyl Hydrosilylation Catalyzed by Brookhart’s Cationic Iridium(III) Pincer Complex
inferred← citeshttps://doi.org/10.1021/jacs.4c16699openalex-snapshot
Alkane Dehydrogenation and H/D Exchange by a Cationic Pincer-Ir(III) Hydride: Cooperative C–H Addition and β-H Elimination Modes Induce Anomalous Selectivity
inferred← citeshttps://doi.org/10.1021/jacs.4c18445openalex-snapshot
3-Center-3-Electron σ-Adduct Enables Silyl Radical Transfer below the Minimum Barrier for Silyl Radical Formation
inferred← citeshttps://doi.org/10.1021/jacs.9b08876openalex-snapshot
Direct Silyl Ether Metathesis for Vitrimers with Exceptional Thermal Stability
inferred← citeshttps://doi.org/10.1021/jo501730nopenalex-snapshot
Ligand-Controlled Reactivity, Selectivity, and Mechanism of Cationic Ruthenium-Catalyzed Hydrosilylations of Alkynes, Ketones, and Nitriles: A Theoretical Study
inferred← citeshttps://doi.org/10.1021/ol2012007openalex-snapshot
Ruthenium-Catalyzed Conversion of sp3 C–O Bonds in Ethers to C–C Bonds Using Triarylboroxines
inferred← citeshttps://doi.org/10.1021/ol202117topenalex-snapshot
Rhodium-Catalyzed, Efficient Deutero- and Tritiosilylation of Carbonyl Compounds from Hydrosilanes and Deuterium or Tritium
inferred← citeshttps://doi.org/10.1021/om100818yopenalex-snapshot
Hydrosilylation of Carbonyl-Containing Substrates Catalyzed by an Electrophilic η1-Silane Iridium(III) Complex
inferred← citeshttps://doi.org/10.1021/om200256hopenalex-snapshot
Catalytic Hydrogen Generation from the Hydrolysis of Silanes by Ruthenium Complexes
inferred← citeshttps://doi.org/10.1021/om300943eopenalex-snapshot
Multiple Si–H Bond Activations bytBu2PCH2CH2PtBu2andtBu2PCH2PtBu2Di(phosphine) Complexes of Rhodium and Iridium
inferred← citeshttps://doi.org/10.1021/om400634wopenalex-snapshot
Theoretical Study of POCOP-Pincer Iridium(III)/Iron(II) Hydride Catalyzed Hydrosilylation of Carbonyl Compounds: Hydride Not Involved in the Iridium(III) System but Involved in the Iron(II) System
inferred← citeshttps://doi.org/10.1021/om500758jopenalex-snapshot
Activation of Dihydrogen and Silanes by Cationic Iron Bis(phosphinite) Pincer Complexes
inferred← citeshttps://doi.org/10.1021/om801192bopenalex-snapshot
Steric and Electronic Effects in Half-Sandwich Ruthenium Silane σ-Complexes with Si−H and Si−Cl Interligand Interactions
inferred← citeshttps://doi.org/10.1038/nchem.2277openalex-snapshot
Chemoselective conversion of biologically sourced polyols into chiral synthons
inferred← citeshttps://doi.org/10.1039/9781788016490-00579openalex-snapshot
Noncovalent Interactions in Key Metal-centred Catalytic Intermediates: Structure–Electronic Relationship
inferred← citeshttps://doi.org/10.1039/c003097jopenalex-snapshot
Silylium ions in catalysis
inferred← citeshttps://doi.org/10.1039/c0cc05714bopenalex-snapshot
Hydrosilylation of epoxides catalyzed by a cationic η1-silane iridium(iii) complex
inferred← citeshttps://doi.org/10.1039/c1dt10339copenalex-snapshot
Cleavage of unreactive bonds with pincer metal complexes
inferred← citeshttps://doi.org/10.1039/c1nj20399aopenalex-snapshot
[Cp′FeI]2 as convenient entry into iron-modified pincer complexes: bimetallic η6,κ1-POCOP-pincer iron iridium compounds
inferred← citeshttps://doi.org/10.1039/c3cc43616kopenalex-snapshot
Fe-promoted cross coupling of homobenzylic methyl ethers with Grignard reagents via sp3 C–O bond cleavage
inferred← citeshttps://doi.org/10.1039/c3sc22256jopenalex-snapshot
Lewis-base silane activation: from reductive cleavage of aryl ethers to selective ortho-silylation
inferred← citeshttps://doi.org/10.1039/c4cc02852jopenalex-snapshot
A novel iron complex for highly efficient catalytic hydrogen generation from the hydrolysis of organosilanes
inferred← citeshttps://doi.org/10.1039/c4cy01233jopenalex-snapshot
Efficient hydrosilylation of imines using catalysts based on iridium( iii ) metallacycles
inferred← citeshttps://doi.org/10.1039/c4cy01259copenalex-snapshot
Mechanistic insights into hydrogen generation for catalytic hydrolysis and alcoholysis of silanes with high-valent oxorhenium( v ) complexes
inferred← citeshttps://doi.org/10.1039/c6ra20864aopenalex-snapshot
Synthesis of tetraline derivatives through depolymerization of polyethers with aromatic compounds using a heterogeneous titanium-exchanged montmorillonite catalyst
inferred← citeshttps://doi.org/10.1039/c7dt00727bopenalex-snapshot
A family of rhodium and iridium complexes with semirigid benzylsilyl phosphines: from bidentate to tetradentate coordination modes
inferred← citeshttps://doi.org/10.1039/c7gc00817aopenalex-snapshot
Effective management of polyethers through depolymerization to symmetric and unsymmetric glycol diesters using a proton-exchanged montmorillonite catalyst
inferred← citeshttps://doi.org/10.1039/c7gc03743kopenalex-snapshot
Efficient reductive depolymerization of hardwood and softwood lignins with Brookhart's iridium( iii ) catalyst and hydrosilanes
inferred← citeshttps://doi.org/10.1039/c8cy01236aopenalex-snapshot
Revisiting the iridacycle-catalyzed hydrosilylation of enolizable imines
inferred← citeshttps://doi.org/10.1039/c8ob02298dopenalex-snapshot
Selective alkyl ether cleavage by cationic bis(phosphine)iridium complexes
inferred← citeshttps://doi.org/10.1039/d0cy00775gopenalex-snapshot
Catalytic reductive deoxygenation of esters to ethers driven by hydrosilane activation through non-covalent interactions with a fluorinated borate salt
inferred← citeshttps://doi.org/10.1039/d1cc00496dopenalex-snapshot
Selective demethylation of O -aryl glycosides by iridium-catalyzed hydrosilylation
inferred← citeshttps://doi.org/10.1039/d2sc02324eopenalex-snapshot
Activation of Si–H and B–H bonds by Lewis acidic transition metals and p-block elements: same, but different
inferred← citeshttps://doi.org/10.1039/d3gc02517aopenalex-snapshot
Co(dppbsa)-catalyzed reductive N , N -dimethylation of nitroaromatics with CO 2 and hydrosilane
inferred← citeshttps://doi.org/10.1039/d3qo01277hopenalex-snapshot
Palladium-catalyzed C(sp 3 )–Si cross-coupling silylation of benzyl halides with hydrosilanes
inferred← citeshttps://doi.org/10.1039/d4dt02555eopenalex-snapshot
Depolymerization by transition metal complexes: strategic approaches to convert polymeric waste into feedstocks
inferred← citeshttps://doi.org/10.1039/d4su00093eopenalex-snapshot
Chemical degradation of oxygenated polymers: the case of polyethers and polysiloxanes
inferred← citeshttps://doi.org/10.1039/d6sc03745copenalex-snapshot
Beyond a single structure: complementary IR and NMR signatures of multi-minima noncovalent binding
inferred← citeshttps://doi.org/10.1080/02603594.2020.1737026openalex-snapshot
Metal/Organosilicon Complexes: Structure, Reactivity, and Considerations for Catalysis
inferred← citeshttps://doi.org/10.1627/jpi.62.255openalex-snapshot
Carbon Dioxide to Organic Compounds Assisted by Silanes: Successive Transformation of Silyl Formate to Various Products
inferred← citeshttps://doi.org/10.70675/8b66a4abz9625z4b59z9bafze696008052b0openalex-snapshot
Synthèse et applications de complexes de nickel(II) pour l’optimisation et la compréhension des réactions d’hydrofonctionnalisation et d’activation C–H.
inferred← citeshttps://doi.org/10.70675/9482d6deze3c3z4faazae6ez5413dbfd5725openalex-snapshot
Nouveaux procédés catalytiques pour le recyclage de déchets ligno-cellulosiques, de polymères et de dérivés du CO₂
inferred← citeshttps://doi.org/10.70675/ad5bccabzb9b4z4700z81bczd2c18418950eopenalex-snapshot
Catalyseurs d’hydrosilylation pour la réduction de liaisons C-O dans les polymères oxygénés
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