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Resolving local reaction environment toward an optimized CO 2 -to-CO conversion performance

https://doi.org/10.1039/d1ee02966e
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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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Electrochemical CO 2 Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design
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High Selectivity for Ethylene from Carbon Dioxide Reduction over Copper Nanocube Electrocatalysts
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Selective and Efficient Reduction of Carbon Dioxide to Carbon Monoxide on Oxide‐Derived Nanostructured Silver Electrocatalysts
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Tuning of Silver Catalyst Mesostructure Promotes Selective Carbon Dioxide Conversion into Fuels
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Electrochemical Real‐Time Mass Spectrometry (EC‐RTMS): Monitoring Electrochemical Reaction Products in Real Time
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Direct Evidence of Local pH Change and the Role of Alkali Cation during CO2 Electroreduction in Aqueous Media
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Flow Electrolyzer Mass Spectrometry with a Gas‐Diffusion Electrode Design
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Inside Cover: Mn−O Covalency Governs the Intrinsic Activity of Co‐Mn Spinel Oxides for Boosted Peroxymonosulfate Activation (Angew. Chem. Int. Ed. 1/2021)
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System Design Rules for Intensifying the Electrochemical Reduction of CO 2 to CO on Ag Nanoparticles
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A Gross‐Margin Model for Defining Technoeconomic Benchmarks in the Electroreduction of CO2
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A DEMS Study of the Reduction of CO2, CO, and HCHO Pre-Adsorbed on Cu Electrodes: Empirical Inferences on the CO2RR Mechanism
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Differential electrochemical mass spectrometry
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What Should We Make with CO2 and How Can We Make It?
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Study of structure and optical properties of silver oxide films by ellipsometry, XRD and XPS methods
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Electrochemical reduction of CO2 on single crystal electrodes of silver Ag(111), Ag(100) and Ag(110)
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An improved k−ω turbulence model applied to recirculating flows
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Differential Electrochemical Mass Spectrometer Cell Design for Online Quantification of Products Produced during Electrochemical Reduction of CO2
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Progress and Perspectives of Electrochemical CO2 Reduction on Copper in Aqueous Electrolyte
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General Techno-Economic Analysis of CO 2 Electrolysis Systems
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Probing CO 2 Conversion Chemistry on Nanostructured Surfaces with Operando Vibrational Spectroscopy
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Insights into Liquid Product Formation during Carbon Dioxide Reduction on Copper and Oxide-Derived Copper from Quantitative Real-Time Measurements
inferredcites →https://doi.org/10.1021/acscatal.1c00338openalex-snapshot
Dramatic HER Suppression on Ag Electrodes via Molecular Films for Highly Selective CO2 to CO Reduction
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Mechanistic Insights into the Electrochemical Reduction of CO2 to CO on Nanostructured Ag Surfaces
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Electric Field Effects in Electrochemical CO 2 Reduction
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Probing the Reaction Mechanism of CO2 Electroreduction over Ag Films via Operando Infrared Spectroscopy
inferredcites →https://doi.org/10.1021/acscatal.8b01738openalex-snapshot
Beyond Copper in CO2 Electrolysis: Effective Hydrocarbon Production on Silver-Nanofoam Catalysts
inferredcites →https://doi.org/10.1021/acscatal.9b00260openalex-snapshot
Influence of Atomic Surface Structure on the Activity of Ag for the Electrochemical Reduction of CO 2 to CO
inferredcites →https://doi.org/10.1021/acsenergylett.0c00482openalex-snapshot
Effects of Surface Roughness on the Electrochemical Reduction of CO 2 over Cu
inferredcites →https://doi.org/10.1021/acsenergylett.0c01606openalex-snapshot
pH Matters When Reducing CO2 in an Electrochemical Flow Cell
inferredcites →https://doi.org/10.1021/acsenergylett.0c02401openalex-snapshot
Self-Cleaning CO2 Reduction Systems: Unsteady Electrochemical Forcing Enables Stability
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CO 2 Reduction at Low Overpotential on Cu Electrodes Resulting from the Reduction of Thick Cu 2 O Films
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Two Pathways for the Formation of Ethylene in CO Reduction on Single-Crystal Copper Electrodes
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Aqueous CO 2 Reduction at Very Low Overpotential on Oxide-Derived Au Nanoparticles
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Suppression of Hydrogen Evolution in Acidic Electrolytes by Electrochemical CO2 Reduction
inferredcites →https://doi.org/10.1021/jacs.6b07612openalex-snapshot
Hydrolysis of Electrolyte Cations Enhances the Electrochemical Reduction of CO 2 over Ag and Cu
inferredcites →https://doi.org/10.1021/jacs.7b06765openalex-snapshot
Promoter Effects of Alkali Metal Cations on the Electrochemical Reduction of Carbon Dioxide
inferredcites →https://doi.org/10.1021/jacs.8b04058openalex-snapshot
Direct Observation of the Local Reaction Environment during the Electrochemical Reduction of CO 2
inferredcites →https://doi.org/10.1021/jacs.8b12766openalex-snapshot
Enhanced Stability and CO/Formate Selectivity of Plasma-Treated SnO x /AgO x Catalysts during CO2 Electroreduction
inferredcites →https://doi.org/10.1021/jacs.9b04956openalex-snapshot
Identifying Active Sites for CO2 Reduction on Dealloyed Gold Surfaces by Combining Machine Learning with Multiscale Simulations
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A selective and efficient electrocatalyst for carbon dioxide reduction
inferredcites →https://doi.org/10.1038/s41467-021-23582-2openalex-snapshot
Electrokinetic and in situ spectroscopic investigations of CO electrochemical reduction on copper
inferredcites →https://doi.org/10.1038/s41560-019-0450-yopenalex-snapshot
Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
inferredcites →https://doi.org/10.1038/s41560-020-00761-xopenalex-snapshot
Designing anion exchange membranes for CO2 electrolysers
inferredcites →https://doi.org/10.1038/s41560-021-00813-wopenalex-snapshot
Operando cathode activation with alkali metal cations for high current density operation of water-fed zero-gap carbon dioxide electrolysers
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The technological and economic prospects for CO2 utilization and removal
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Understanding heterogeneous electrocatalytic carbon dioxide reduction through operando techniques
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Absence of CO2 electroreduction on copper, gold and silver electrodes without metal cations in solution
inferredcites →https://doi.org/10.1039/c1cp22700aopenalex-snapshot
The importance of surface morphology in controlling the selectivity of polycrystalline copper for CO2 electroreduction
inferredcites →https://doi.org/10.1039/c1sc00277eopenalex-snapshot
A new mechanism for the selectivity to C1 and C2 species in the electrochemical reduction of carbon dioxide on copper electrodes
inferredcites →https://doi.org/10.1039/c2ee21234jopenalex-snapshot
New insights into the electrochemical reduction of carbon dioxide on metallic copper surfaces
inferredcites →https://doi.org/10.1039/c7cp06087dopenalex-snapshot
Probing promoting effects of alkali cations on the reduction of CO at the aqueous electrolyte/copper interface
inferredcites →https://doi.org/10.1039/c9ee01341eopenalex-snapshot
Understanding cation effects in electrochemical CO 2 reduction
inferredcites →https://doi.org/10.1039/c9ee02410gopenalex-snapshot
Transforming the carbon economy: challenges and opportunities in the convergence of low-cost electricity and reductive CO 2 utilization
inferredcites →https://doi.org/10.1039/c9ee02485aopenalex-snapshot
Modeling the electrical double layer to understand the reaction environment in a CO 2 electrocatalytic system
inferredcites →https://doi.org/10.1039/d0ee00047gopenalex-snapshot
Insights into the carbon balance for CO 2 electroreduction on Cu using gas diffusion electrode reactor designs
inferredcites →https://doi.org/10.1039/d1ee01664dopenalex-snapshot
Rigorous assessment of CO 2 electroreduction products in a flow cell
inferredcites →https://doi.org/10.1073/pnas.0603395103openalex-snapshot
Powering the planet: Chemical challenges in solar energy utilization
inferredcites →https://doi.org/10.1073/pnas.1900761116openalex-snapshot
Hydrogen bonding steers the product selectivity of electrocatalytic CO reduction
inferredcites →https://doi.org/10.1126/sciadv.abd2569openalex-snapshot
Understanding the electric and nonelectric field components of the cation effect on the electrochemical CO reduction reaction
inferredcites →https://doi.org/10.1126/science.aad4998openalex-snapshot
Combining theory and experiment in electrocatalysis: Insights into materials design
inferredcites →https://doi.org/10.1371/journal.pone.0153755openalex-snapshot
Turbulence Model Selection for Low Reynolds Number Flows
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Designing Electrolyzers for Electrocatalytic CO2 Reduction

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

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Chloride Ion Adsorption Enables Ampere‐Level CO 2 Electroreduction over Silver Hollow Fiber
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Enriching Surface‐Accessible CO2 in the Zero‐Gap Anion‐Exchange‐Membrane‐Based CO2 Electrolyzer
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Mechanism of Cations Suppressing Proton Diffusion Kinetics for Electrocatalysis
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Favoring CO Intermediate Stabilization and Protonation by Crown Ether for CO2 Electromethanation in Acidic Media
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Time‐Resolved Product Observation for CO 2 Electroreduction Using Synchronised Electrochemistry‐Mass Spectrometry with Soft Ionisation (sEC‐MS‐SI)
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Anchoring Cs + Ions on Carbon Vacancies for Selective CO 2 Electroreduction to CO at High Current Densities in Membrane Electrode Assembly Electrolyzers
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Fundamentals and Challenges of Ligand Modification in Heterogeneous Electrocatalysis
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Heteroarchitectural Gas Diffusion Layer Promotes CO 2 Reduction Coupled with Biomass Oxidation at Ampere‐Level Current Density
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Bifurcation of *COOH Pathway Determines HCOOH Formation in CO 2 Electroreduction on Bismuth
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Overcoming Salt Precipitation in CO 2 Reduction Membrane Electrode Assembly Electrolyzer Enables Over 4200 Hours Stable Operation
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Design and Synthesis of Ag‐based Catalysts for Electrochemical CO 2 Reduction: Advances and Perspectives
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Tuning Sb Atoms on Cu‐Based Catalysts for Electrochemical Conversion of CO2 to Syngas
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Quantification of CO and Further CO2 Reduction Products by On‐line Mass Spectrometry
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Recent Advances in Microenvironment Engineering for Selective Electrochemical C–N Coupling
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Selective Acidic CO 2 Electroreduction to Methane Using Crown Ether‐Functionalized Copper‐Based Electrodes
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Highly Efficient CO2 Reduction at Steady 2 A cm−2 by Surface Reconstruction of Silver Penetration Electrode
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Microenvironment Engineering in Electrochemical CO 2 Reduction: From Multiscale Reaction Fields to Coupled Operating Windows
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H–C Bond Elongation Induced by Dipolar Rh Adatoms and Vacancies: Site Polarity-Driven Many-Body Cooperativity
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Self-Tandem Electrocatalytic NO Reduction to NH 3 on a W Single-Atom Catalyst
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inferred← citeshttps://doi.org/10.1021/acsenergylett.5c04199openalex-snapshot
Molecularly Engineered Polystyrene-Imidazolium Polyelectrolytes for CO 2 Electrolysis in Strongly Acidic Media
inferred← citeshttps://doi.org/10.1021/acssuschemeng.5c06219openalex-snapshot
Solvated Electrons-Induced CO 2 Valorization via Plasma–Liquid Interface for Sustainable Organic Acid Production
inferred← citeshttps://doi.org/10.1021/jacs.4c10661openalex-snapshot
Anion Effect in Electrochemical CO 2 Reduction: From Spectators to Orchestrators
inferred← citeshttps://doi.org/10.1021/jacs.5c04023openalex-snapshot
Bicarbonate-Dependence for Pd-Catalyzed CO 2 Hydrogenation to Formate over an Electronegativity-Induced Bimetallic Center
inferred← citeshttps://doi.org/10.1038/s41467-023-43118-0openalex-snapshot
Data-driven discovery of electrocatalysts for CO2 reduction using active motifs-based machine learning
inferred← citeshttps://doi.org/10.1038/s41467-024-51926-1openalex-snapshot
Disentangling heterogeneous thermocatalytic formic acid dehydrogenation from an electrochemical perspective
inferred← citeshttps://doi.org/10.1038/s41467-024-54122-3openalex-snapshot
Molecular level insights on the pulsed electrochemical CO2 reduction
inferred← citeshttps://doi.org/10.1038/s41467-025-59604-6openalex-snapshot
Non-isothermal CO2 electrolysis enables simultaneous enhanced electrochemical and anti-precipitation performance
inferred← citeshttps://doi.org/10.1038/s41467-025-63178-8openalex-snapshot
Localized mass transport channels for electro-upgrade of dilute CO2 toward high-yield C2+ products
inferred← citeshttps://doi.org/10.1038/s41467-025-63181-zopenalex-snapshot
Adsorbed oxygen dynamics at forced convection interface in the oxygen evolution reaction
inferred← citeshttps://doi.org/10.1038/s41467-026-71584-9openalex-snapshot
Differentiating interfacial water structures via alkali metal cation promotor for H2O2 electrosynthesis in acid
inferred← citeshttps://doi.org/10.1039/9781837679812-00186openalex-snapshot
Catalysis for intermediate temperature chemical production and relevance to protonic ceramic electrochemical cells
inferred← citeshttps://doi.org/10.1039/d2cc05081aopenalex-snapshot
Top-down manufacturing of efficient CO 2 reduction catalysts from the gasification residue carbon
inferred← citeshttps://doi.org/10.1039/d2cs00441kopenalex-snapshot
Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction
inferred← citeshttps://doi.org/10.1039/d2se01174copenalex-snapshot
In situ oxidative etching-enabled synthesis of hollow Cu 2 O nanocrystals for efficient CO 2 RR into C 2+ products
inferred← citeshttps://doi.org/10.1039/d2ta06567copenalex-snapshot
A co-carbonization strategy for confining ultralow-loaded Fe/Mn dual sites in hierarchically porous N-doped carbon for synergistic CO 2 electroreduction
inferred← citeshttps://doi.org/10.1039/d3cc05277jopenalex-snapshot
Enhanced CO 2 reduction with hydrophobic cationic-ionomer layer-modified zero-gap MEA in acidic electrolyte
inferred← citeshttps://doi.org/10.1039/d3cs00186eopenalex-snapshot
Aryl ether-free polymer electrolytes for electrochemical and energy devices
inferred← citeshttps://doi.org/10.1039/d3cs00840aopenalex-snapshot
Recent development and applications of differential electrochemical mass spectrometry in emerging energy conversion and storage solutions
inferred← citeshttps://doi.org/10.1039/d3ee01866kopenalex-snapshot
Hydrophobized electrospun nanofibers of hierarchical porosity as the integral gas diffusion electrode for full-pH CO 2 electroreduction in membrane electrode assemblies
inferred← citeshttps://doi.org/10.1039/d3gc02329jopenalex-snapshot
Techno-economic analysis and life-cycle assessment of the electrochemical conversion process with captured CO 2 in an amine-based solvent
inferred← citeshttps://doi.org/10.1039/d5cs00780aopenalex-snapshot
Optimizing CO 2 electroreduction: theoretical insights for enhancing efficiency across elementary steps
inferred← citeshttps://doi.org/10.1039/d5ee02225hopenalex-snapshot
Innovative electrode designs for low-temperature electrochemical CO 2 reduction with ampere-level performance
inferred← citeshttps://doi.org/10.1039/d5ta00927hopenalex-snapshot
Recent advances in surface modification for enhanced electrocatalytic CO 2 reduction
inferred← citeshttps://doi.org/10.1039/d6ra03997aopenalex-snapshot
Decoding non-fullerene acceptors for organic solar cells: a theoretical structure–property–performance perspective
inferred← citeshttps://doi.org/10.1063/5.0223542openalex-snapshot
Metal–metal oxide hybrid catalysts for electrocatalytic CO2 reduction reaction
inferred← citeshttps://doi.org/10.1073/pnas.2400898121openalex-snapshot
Electrifying HCOOH synthesis from CO 2 building blocks over Cu–Bi nanorod arrays
inferred← citeshttps://doi.org/10.3389/fctls.2025.1657848openalex-snapshot
Experimental study of operating parameters in zero-gap CO2 electrolysis
inferred← citeshttps://doi.org/10.3390/membranes15020055openalex-snapshot
Challenges and Opportunities of Choosing a Membrane for Electrochemical CO2 Reduction
inferred← citeshttps://doi.org/10.35848/1347-4065/addd2aopenalex-snapshot
Understanding the CO2 reduction reaction anolyte flooding problem in polymer electrolyte type reactor through the cation and water transport properties of ion exchange membranes
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