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Closed-loop additive manufacturing of upcycled commodity plastic through dynamic cross-linking

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What this work says

Outgoing claims: the papers this work cites, builds on, or argues with.

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Plastics: Thermoplastics, Thermosets, and Elastomers
inferredcites →https://doi.org/10.1002/adfm.201404553openalex-snapshot
Vinylogous Urethane Vitrimers
inferredcites →https://doi.org/10.1002/adfm.201700318openalex-snapshot
Diels–Alder Reversible Thermoset 3D Printing: Isotropic Thermoset Polymers via Fused Filament Fabrication
inferredcites →https://doi.org/10.1002/adma.201400317openalex-snapshot
Heat‐ or Water‐Driven Malleability in a Highly Recyclable Covalent Network Polymer
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3D‐Printing of Lightweight Cellular Composites
inferredcites →https://doi.org/10.1002/adma.201505245openalex-snapshot
Repairable Woven Carbon Fiber Composites with Full Recyclability Enabled by Malleable Polyimine Networks
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Dynamic Covalent Polymer Networks: from Old Chemistry to Modern Day Innovations
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Additive Manufacturing: Unlocking the Evolution of Energy Materials
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Thiol–Ene Click Chemistry
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Beyond Mechanical Recycling: Giving New Life to Plastic Waste
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Nanofiber‐reinforced polymers prepared by fused deposition modeling
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Infrared preheating to improve interlayer strength of big area additive manufacturing (BAAM) components
inferredcites →https://doi.org/10.1016/j.addma.2019.05.020openalex-snapshot
Extrusion control for high quality printing on Big Area Additive Manufacturing (BAAM) systems
inferredcites →https://doi.org/10.1016/j.compositesb.2019.107496openalex-snapshot
A review of recent research on bio-inspired structures and materials for energy absorption applications
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Cysteamine as a Future Intervention in Cystic Fibrosis Against Current and Emerging Pathogens: A Patient-based ex vivo Study Confirming its Antimicrobial and Mucoactive Potential in Sputum
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Selective separation of ABS/PC containing BFRs from ABSs mixture of WEEE by developing hydrophilicity with ZnO coating under microwave treatment
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Energy absorption characteristics of bio-inspired honeycomb column thin-walled structure under impact loading
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Manufacturing energy and greenhouse gas emissions associated with plastics consumption
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Imine-linked polymer/silica composites for CO2 sequestration
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Additive manufacturing: scientific and technological challenges, market uptake and opportunities
inferredcites →https://doi.org/10.1016/j.pmatsci.2020.100710openalex-snapshot
Functional epoxy vitrimers and composites
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Vitrimers: Permanently crosslinked polymers with dynamic network topology
inferredcites →https://doi.org/10.1021/acs.chemrev.7b00074openalex-snapshot
Polymers for 3D Printing and Customized Additive Manufacturing
inferredcites →https://doi.org/10.1021/acs.macromol.8b01601openalex-snapshot
Robust, Fire-Safe, Monomer-Recovery, Highly Malleable Thermosets from Renewable Bioresources
inferredcites →https://doi.org/10.1021/acsami.0c13976openalex-snapshot
4D Printing via an Unconventional Fused Deposition Modeling Route to High-Performance Thermosets
inferredcites →https://doi.org/10.1021/acsami.6b05118openalex-snapshot
Design Paradigm Utilizing Reversible Diels–Alder Reactions to Enhance the Mechanical Properties of 3D Printed Materials
inferredcites →https://doi.org/10.1021/acsapm.0c01008openalex-snapshot
Synthesis of Vanillin-Based Polyimine Vitrimers with Excellent Reprocessability, Fast Chemical Degradability, and Adhesion
inferredcites →https://doi.org/10.1021/acscentsci.0c00567openalex-snapshot
Reprocessable Cross-Linked Polymer Networks: Are Associative Exchange Mechanisms Desirable?
inferredcites →https://doi.org/10.1021/acsmaterialslett.1c00132openalex-snapshot
Highly Recyclable, Mechanically Isotropic and Healable 3D-Printed Elastomers via Polyurea Vitrimers
inferredcites →https://doi.org/10.1021/cm402180topenalex-snapshot
The Thiol-Michael Addition Click Reaction: A Powerful and Widely Used Tool in Materials Chemistry
inferredcites →https://doi.org/10.1021/jacs.9b07922openalex-snapshot
Adaptable Crosslinks in Polymeric Materials: Resolving the Intersection of Thermoplastics and Thermosets
inferredcites →https://doi.org/10.1021/ma801630nopenalex-snapshot
Development of Thermal and Photochemical Strategies for Thiol−Ene Click Polymer Functionalization
inferredcites →https://doi.org/10.1038/nature21003openalex-snapshot
Printing soft matter in three dimensions
inferredcites →https://doi.org/10.1038/ncomms14857openalex-snapshot
Chemical control of the viscoelastic properties of vinylogous urethane vitrimers
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Structural optimization of 3D-printed synthetic spider webs for high strength
inferredcites →https://doi.org/10.1038/s41467-018-04292-8openalex-snapshot
Reprocessable thermosets for sustainable three-dimensional printing
inferredcites →https://doi.org/10.1038/s41467-019-11144-6openalex-snapshot
Detecting topology freezing transition temperature of vitrimers by AIE luminogens
inferredcites →https://doi.org/10.1038/s41467-021-20953-7openalex-snapshot
In situ mechanical reinforcement of polymer hydrogels via metal-coordinated crosslink mineralization
inferredcites →https://doi.org/10.1038/s41557-019-0249-2openalex-snapshot
Closed-loop recycling of plastics enabled by dynamic covalent diketoenamine bonds
inferredcites →https://doi.org/10.1038/s41558-019-0459-zopenalex-snapshot
Strategies to reduce the global carbon footprint of plastics
inferredcites →https://doi.org/10.1038/s41570-017-0046openalex-snapshot
Chemical recycling of waste plastics for new materials production
inferredcites →https://doi.org/10.1038/s41578-020-00234-3openalex-snapshot
The global rise of 3D printing during the COVID-19 pandemic
inferredcites →https://doi.org/10.1038/s41586-020-03149-9openalex-snapshot
Closed-loop recycling of polyethylene-like materials
inferredcites →https://doi.org/10.1038/s41598-019-56350-wopenalex-snapshot
Revealing interactions of layered polymeric materials at solid-liquid interface for building solvent compatibility charts for 3D printing applications
inferredcites →https://doi.org/10.1039/c4py00339jopenalex-snapshot
Thiol–ene “click” reactions and recent applications in polymer and materials synthesis: a first update
inferredcites →https://doi.org/10.1039/c5sc02223aopenalex-snapshot
Vitrimers: permanent organic networks with glass-like fluidity
inferredcites →https://doi.org/10.1039/c6mh00029kopenalex-snapshot
Epoxy resin with exchangeable disulfide crosslinks to obtain reprocessable, repairable and recyclable fiber-reinforced thermoset composites
inferredcites →https://doi.org/10.1039/c7me00023eopenalex-snapshot
2D and 3D-printing of self-healing gels: design and extrusion of self-rolling objects
inferredcites →https://doi.org/10.1039/c7mh00043jopenalex-snapshot
Recyclable 3D printing of vitrimer epoxy
inferredcites →https://doi.org/10.1039/c7py00310bopenalex-snapshot
3D printed remendable polylactic acid blends with uniform mechanical strength enabled by a dynamic Diels–Alder reaction
inferredcites →https://doi.org/10.1039/c7py01945aopenalex-snapshot
3D-printing of dynamic self-healing cryogels with tuneable properties
inferredcites →https://doi.org/10.1039/c7ta07076dopenalex-snapshot
Rehealable imide–imine hybrid polymers with full recyclability
inferredcites →https://doi.org/10.1039/c9gc00540dopenalex-snapshot
A fully bio-based polyimine vitrimer derived from fructose
inferredcites →https://doi.org/10.1039/c9py01826copenalex-snapshot
Tuning the mechanical and dynamic properties of imine bond crosslinked elastomeric vitrimers by manipulating the crosslinking degree
inferredcites →https://doi.org/10.1039/d0an00879fopenalex-snapshot
Quantitative 1 H-NMR spectroscopy as an efficient method for identification and quantification of PVC, ABS and PA microparticles
inferredcites →https://doi.org/10.1108/13552540210441166openalex-snapshot
Anisotropic material properties of fused deposition modeling ABS
inferredcites →https://doi.org/10.1126/sciadv.1602800openalex-snapshot
Self-assembled micro-organogels for 3D printing silicone structures
inferredcites →https://doi.org/10.1126/sciadv.abf0187openalex-snapshot
Leveling the cost and carbon footprint of circular polymers that are chemically recycled to monomer
inferredcites →https://doi.org/10.1126/science.1212648openalex-snapshot
Silica-Like Malleable Materials from Permanent Organic Networks
inferredcites →https://doi.org/10.1126/science.1252291openalex-snapshot
Ultralight, ultrastiff mechanical metamaterials
inferredcites →https://doi.org/10.1126/science.267.5206.1924openalex-snapshot
Formation of Glasses from Liquids and Biopolymers
inferredcites →https://doi.org/10.1126/science.aad2688openalex-snapshot
Additive manufacturing of polymer-derived ceramics
inferredcites →https://doi.org/10.1126/science.aah5281openalex-snapshot
High-performance vitrimers from commodity thermoplastics through dioxaborolane metathesis
inferredcites →https://doi.org/10.1126/science.aao6749openalex-snapshot
Beyond plastic waste
inferredcites →https://doi.org/10.1126/science.abb0354openalex-snapshot
Plastics in the Earth system
inferredcites →https://doi.org/10.1126/science.abg4503openalex-snapshot
Toward polymer upcycling—adding value and tackling circularity
inferredcites →https://doi.org/10.1126/science.abg9853openalex-snapshot
Achieving net-zero greenhouse gas emission plastics by a circular carbon economy
inferredcites →https://doi.org/10.1295/polymj.35.560openalex-snapshot
Energy Absorption in Chopped Carbon Fiber Epoxy Composites for Automotive Crashworthiness
inferredcites →https://doi.org/10.1371/journal.pone.0034437openalex-snapshot
Cysteamine Suppresses Invasion, Metastasis and Prolongs Survival by Inhibiting Matrix Metalloproteinases in a Mouse Model of Human Pancreatic Cancer
inferredcites →https://doi.org/10.1557/s43579-020-00006-8openalex-snapshot
Direct ink writing techniques for in situ gelation and solidification
inferredcites →https://doi.org/10.2172/1616517openalex-snapshot
Report of the Basic Energy Sciences Roundtable on Chemical Upcycling of Polymers
inferredcites →https://doi.org/10.3390/technologies5020020openalex-snapshot
Compression Tests of ABS Specimens for UAV Components Produced via the FDM Technique
inferredcites →https://doi.org/10.7494/jcme.2017.1.2.39openalex-snapshot
Bending and Compression Properties of ABS and PET Structural Materials Printed Using FDM Technology

What points at this work

Incoming claims: where this work appears in other papers’ reference lists and arguments.

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Recent Progress on the 3D Printing of Dynamically Cross‐Linked Polymers
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Photoreforming and Photoelectroreforming of Waste‐Derived Feedstocks for Solar‐Driven Production of Fuels and Chemicals
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Glucose‐Derived Circular Thermoset Platform Breaks the Industrial Trilemma of Recyclable Structural Polymers
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Understanding Depolymerization and Repolymerization Toward Repurposing Polymer Waste Into Valuable Chemicals & Materials
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Modular chem‐bio upcycling of waste poly(ethylene terephthalate) to glycolic acid and 2,4‐pyridine dicarboxylic acid
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Polymer Multi‐Block and Multi‐Block+ Strategies for the Upcycling of Mixed Polyolefins and Other Plastics
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Polyurethane with β‐Selenocarbonyl Structure Enabling the Combination of Plastic Degradation and Waste Upcycling
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From Plastic Waste to Green Hydrogen and Valuable Chemicals Using Sunlight and Water
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Polymer Multi‐Block and Multi‐Block + Strategies for the Upcycling of Mixed Polyolefins and Other Plastics
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Polyurethane with β‐Selenocarbonyl Structure Enabling the Combination of Plastic Degradation and Waste Upcycling
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From Plastic Waste to Green Hydrogen and Valuable Chemicals Using Sunlight and Water
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Research on the High‐Temperature Performance of Asphalt Modified With Covalently Crosslinked Polyethylene Waste Plastic
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Extrudable Thermosets Based on Dynamic Covalent Polymers
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Synthesis of Graft‐Modified Polyolefin Compatibilizers for Compatibilizing Mixed Plastics
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Modular Molecular Editing for Polymer‐to‐Polymer Recycling of Postconsumer Plastics
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Plastic Waste Conversion by Leveraging Renewable Photo/Electro‐Catalytic Technologies
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Closed‐Loop Recyclable Vitrimer Plastics from PET Waste: A Design for Circularity
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Thiol‐X Chemistry: A Skeleton Key Unlocking Advanced Polymers in Additive Manufacturing
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Toward Circular Polymer Materials and Manufacturing: Dynamic Bonding Strategies for Upcycling Thermoplastics and Thermosets
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Upcycling of thermoplastic polyurethane into covalent adaptable networks via chain breaking‐crosslinking strategy
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Recycling and Healing of Vitrimers: Double Layer of Sustainability Using Green Approaches
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Sustainable Materials and Manufacturing: Innovations Driving Circular Product Design
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Fabrication of effective polyamide-amine acrylonitrile-butadiene-styrene composites using recycled ABS waste plastic for removal of malachite green from aqueous solutions
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Recent Advances in Vitrimers: A Detailed Study on the Synthesis, Properties and Applications of Bio-Vitrimers
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Polyolefin containing multi-block polymers and upcycling of mixed plastics
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RETRACTED ARTICLE: Functional organic materials for energy storage and conversion: recent developments and future perspectives
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Biopolymers: a comprehensive review of sustainability, environmental impact, and lifecycle analysis
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Tuning crosslinking of hybrid preceramic polymers in vat photopolymerization toward controlled ceramic yields
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Designing from biobased to closed-loop circularity: Flexible dynamic polyimine-amide networks
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The conformational preference of dynamic crosslinker modulates the ‘closed-loop’ circular economy in polypropylene vitrimer
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Closed-loop recyclable bio-based covalent adaptable networks for high-efficiency UV shielding
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Additive manufacturing of vitrimers: Interplay between polymer physics and processing approaches
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Ionic network engineering for one-pot upcycling of waste acrylonitrile–butadiene–styrene
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Top-down vitrimerization of commercial polymer materials: A practical pathway toward sustainability
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Dually dynamic printable Diels–Alder polyurethane networks with robust recyclability, self-healing, and shape memory
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3D printing of fully recyclable continuous fiber self-reinforced composites utilizing supercooled polymer melts
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Technologies for room-temperature self-healing polymer materials and their applications in energetic materials
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Closed-loop circular economy in ‘upcycled’ acrylonitrile–butadiene–styrene vitrimer
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High-strength self-healable polyurethane elastomer based on tandem dynamic covalent bonds and sextuple hydrogen bonding
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Thiol-ene click chemistry incorporates carboxylic acid-terminated alkane pendants on polycyclooctene to tune properties
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Application of green dissolution separation and recycling of waste polyester/cotton/polyurethane blended fabric
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Advances in 3D printing of structural and functional ceramics: Technologies, properties, and applications
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A review on formation and suppression mechanisms of porosity and cracks in wire arc-directed energy deposition Al-Zn-Mg-Cu alloys
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Sustainable fabrication of 3D printing filament from recycled PET plastic
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Bio-inspired 4D printed regenerative thermosets enabled by synergistic dynamic reactions
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High-strength supramolecular covalent adaptable networks with reprocessability and closed-loop recyclability
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Thermomechanical properties and self-healing behavior of vitrimers with dual dynamic disulfide and ester networks: Insights from molecular dynamics simulations
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Thermomechanical analysis (TMA) of vitrimers
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Upcycled PET vitrimer filaments via reactive extrusion for high strength heat resistant and repairable FDM parts
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Mechanical and dimensional assessment of threaded fasteners manufactured using 3D printing
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Recent advances of sustainable and recyclable polymer materials from renewable resources
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Well-Tunable, 3D-printable, and Fast Autonomous Self-Healing Elastomers
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Polyolefins Vitrimers: Design Principles and Applications
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Intrinsically Self-Healing Polymers: From Mechanistic Insight to Current Challenges
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Covalent Adaptable Networks: Reprocessable Cross-Linked Polymers
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Dynamic Bond Chemistry in Soft Materials: Bridging Adaptability and Mechanical Robustness
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One-Step Compatibilization and Upcycling of Mixed Polyolefins Using a Dynamic Disulfide-Linked Bismaleimide Cross-Linker
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Harnessing β-Hydroxyl Groups in Poly(β-Amino Esters) toward Robust and Fast Reprocessing Covalent Adaptable Networks
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Time–Temperature Superposition of Polybutadiene Vitrimers
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Chemically Recyclable Supramolecular Thermosets toward Strong and Reusable Hot-Melt Adhesives
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Healable and Recyclable Polyurethane with Natural-Rubber-like Resilience via π-Type Tweezer Structure Stabilizing Dynamical Hard Domains
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Unveiling the Multiscale Dynamics of Polymer Vitrimers Via Molecular Dynamics Simulations
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Source of Processable Vitrimer Viscosities: Swap Frequencies and Steric Factors
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Incorporation of Thioacetate Pendants on a Polyalkenamer Enables High Extensibility
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Linear Viscoelasticity of Polystyrene Vitrimers: Segmental Motions and the Slow Arrhenius Process
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Network Topology and Linear Viscoelasticity of Vitrimers─A Polymer Physics Perspective
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Highly Filled Coextruded Dual-Layer Polymer/Ceramic Filament for Material Extrusion Additive Manufacturing
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Mechanically Interlocked Vitrimer Based on Polybenzoxazine and Polyrotaxane
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3D Printing of Vinylogous Urethane-Based Methacrylic Covalent Adaptable Networks by Vat Photopolymerization
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Dynamic Cross-Linker Facilitates a Closed-Loop Circular Economy in Upcycled Acrylonitrile-Butadiene-Styrene
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Thiol–ene Click Chemistry Incorporates Hydroxyl Functionality on Polycyclooctene to Tune Properties
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Ionic-Liquid-Mediated Deconstruction of Polymers for Advanced Recycling and Upcycling
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Catalyst-Free Dynamic Crosslinking of Polydicyclopentadiene via Thiol–Ene/Imine Chemistry
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Fabrication and Properties of Silicon-Containing Resin-Based Covalent Adaptable Networks via Hybrid Exchange Reaction between Ph–OH Groups and Si–O–Si Bonds
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Upcycling Post-Consumer Recycled Polypropylene Using a “Tailor-Made” Dynamic Cross-Linker with Controlled “Cross-Link Distribution”
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Toward Sustainable Polydienes
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Fostering the waste management with environmental-resource interacting attribute
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Photoinduced bulk polymerization strategy in melt state for recyclable polydiene derivatives
inferred← citeshttps://doi.org/10.1039/d2mh01549hopenalex-snapshot
Recent development of end-of-life strategies for plastic in industry and academia: bridging their gap for future deployment
inferred← citeshttps://doi.org/10.1039/d3lp00268copenalex-snapshot
Closing the loop: polyimine thermosets from furfural derived bioresources
inferred← citeshttps://doi.org/10.1039/d3py01054fopenalex-snapshot
Reprocessable and chemically recyclable poly(acylhydrazone–imine) covalent adaptable networks with enhanced mechanical strength and creep resistance
inferred← citeshttps://doi.org/10.1039/d3sc00551hopenalex-snapshot
Circularity in polymers: addressing performance and sustainability challenges using dynamic covalent chemistries
inferred← citeshttps://doi.org/10.1039/d5ra07879bopenalex-snapshot
Development of biobased dynamic thiol–acrylate photopolymers: 3D-printed self-healing and shape memory materials
inferred← citeshttps://doi.org/10.1080/15583724.2023.2227692openalex-snapshot
3D Printing of Covalent Adaptable Networks: Overview, Applications and Future Prospects
inferred← citeshttps://doi.org/10.1080/17452759.2026.2690309openalex-snapshot
Olfactory-Interactive 4D materials from a carvone-based photocurable resin
inferred← citeshttps://doi.org/10.1109/iarce68366.2025.11485763openalex-snapshot
Design and Manufacturing of a Device for Obtaining 3D Filament from Plastic Bottles
inferred← citeshttps://doi.org/10.1109/ic3et64989.2026.11467200openalex-snapshot
Automated 3D Printing Filament Making Machine Using PET Bottles
inferred← citeshttps://doi.org/10.1126/sciadv.adl2737openalex-snapshot
Bicontinuous vitrimer heterogels with wide-span switchable stiffness-gated iontronic coordination
inferred← citeshttps://doi.org/10.1146/annurev-matsci-072924-115520openalex-snapshot
Beyond Recycling: Vitrimer and Chemical Valorization Strategies for Thermoplastic Polyolefin Upcycling
inferred← citeshttps://doi.org/10.1360/ssc-2025-0278openalex-snapshot
Synthesis of linear multi-block copolymers and their application in plastic recycling and modification
inferred← citeshttps://doi.org/10.21203/rs.3.rs-3618604/v1openalex-snapshot
Upcycling acrylonitrile-butadiene-styrene Vitrimer ‘in melt’ using a dynamic crosslinker
inferred← citeshttps://doi.org/10.3390/app152111755openalex-snapshot
Dynamic Covalent Bonds in 3D-Printed Polymers: Strategies, Principles, and Applications
inferred← citeshttps://doi.org/10.3390/polym14204338openalex-snapshot
Bio-Vitrimers for Sustainable Circular Bio-Economy
inferred← citeshttps://doi.org/10.3390/polym15214219openalex-snapshot
Recycling as a Key Enabler for Sustainable Additive Manufacturing of Polymer Composites: A Critical Perspective on Fused Filament Fabrication
inferred← citeshttps://doi.org/10.3390/pr13010171openalex-snapshot
Influence of Additional Devices and Polymeric Matrix on In Situ Welding in Material Extrusion: A Review
inferred← citeshttps://doi.org/10.3390/technologies13100428openalex-snapshot
Additive Manufacturing as a Catalyst for Low-Carbon Production and the Renewable Energy Transition in Electric Vehicles
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