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Atom-economic and stereoselective catalytic synthesis of fully substituted enol esters/carbonates of amides in acyclic systems enabled by boron Lewis acid catalysis

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Stereoselective Formation of Quaternary Carbon Centers: Alkylation ofα,α-Disubstituted Amide Enolates

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CH Functionalization/CO Bond Cleavage of Benzyl Silyl Ethers with Ynamides for the Chemoselective Synthesis of Skeletally Diverse Compounds

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B(C6F5)3‐Catalyzed Hydroarylation of Terminal Alkynes with Phenols

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Propargylic Esters in Gold Catalysis: Access to Diversity

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Highly Enantioselective Palladium‐Catalyzed Alkylation of Acyclic Amides

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Frustrated Lewis Pairs: Metal‐free Hydrogen Activation and More

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Ynamides: Versatile Tools in Organic Synthesis

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Insertion of an Alkene into an Ester: Intramolecular Oxyacylation Reaction of Alkenes through Acyl CO Bond Activation

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Palladium‐Catalyzed Allylic Alkylation of Carboxylic Acid Derivatives: N‐Acyloxazolinones as Ester Enolate Equivalents

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Pseudoephenamine: A Practical Chiral Auxiliary for Asymmetric Synthesis

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Frustrated Lewis Pair Catalyzed Hydroamination of Terminal Alkynes

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Generation of Stereochemically Defined Tetrasubstituted Enolborinates by 1,4‐Hydroboration of α,β‐Unsaturated Morpholine Carboxamides with (Diisopinocampheyl)borane

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Hydrocarbation of CC Bonds: Quantification of the Nucleophilic Reactivity of Ynamides

inferredcites →https://doi.org/10.1002/anie.201407002openalex-snapshot

Trans ‐Selective Radical Silylzincation of Ynamides

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Rhodium(III)/Copper(II)‐Promoted trans‐Selective Heteroaryl Acyloxylation of Alkynes: Stereodefined Access to trans‐Enol Esters

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Stereodefined Acyclic Polysubstituted Silyl Ketene Aminals: Asymmetric Formation of Aldol Products with Quaternary Carbon Stereocenters

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Frustrated Lewis Pair‐Catalyzed Cycloisomerization of 1,5‐Enynes via a 5‐endo‐dig Cyclization/Protodeborylation Sequence

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Regiodivergent Intermolecular [3+2] Cycloadditions of Vinyl Aziridines and Allenes: Stereospecific Synthesis of Chiral Pyrrolidines

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Rhodium(I)‐Catalyzed Intermolecular Aza‐[4+3] Cycloaddition of Vinyl Aziridines and Dienes: Atom‐Economical Synthesis of Enantiomerically Enriched Functionalized Azepines

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Brønsted Acid Catalyzed Oxygenative Bimolecular Friedel–Crafts‐type Coupling of Ynamides

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One‐Pot Multicomponent Synthesis of β‐Amino Amides

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Stoichiometric and Catalytic C−C and C−H Bond Formation with B(C6F5)3 via Cationic Intermediates

inferredcites →https://doi.org/10.1002/anie.201911722openalex-snapshot

Efficient and Divergent Synthesis of α‐Halogenated Amides and Esters by Double Electrophilic Activation of Ynamides

inferredcites →https://doi.org/10.1002/anie.201915522openalex-snapshot

Keteniminium‐Driven Umpolung Difunctionalization of Ynamides

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Triarylborane‐Catalyzed Alkenylation Reactions of Aryl Esters with Diazo Compounds

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Frustrated Radical Pairs: Insights from EPR Spectroscopy

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Bifunctional Borane Catalysis of a Hydride Transfer/Enantioselective [2+2] Cycloaddition Cascade

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Palladium‐Catalyzed Dearomative Methoxyallylation of 3‐Nitroindoles with Allyl Carbonates

inferredcites →https://doi.org/10.1002/anie.202107647openalex-snapshot

Regio‐ and Stereoselective 1,2‐Carboboration of Ynamides with Aryldichloroboranes

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Tris(pentafluorophenyl)borane‐Catalyzed Carbenium Ion Generation and Autocatalytic Pyrazole Synthesis—A Computational and Experimental Study

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Brønsted Acid Catalyzed Dearomatization by Intramolecular Hydroalkoxylation/Claisen Rearrangement: Diastereo‐ and Enantioselective Synthesis of Spirolactams

inferredcites →https://doi.org/10.1002/anie.202200204openalex-snapshot

Palladium‐Catalyzed Silylcyanation of Ynamides: Regio‐ and Stereoselective Access to Tetrasubstituted 3‐Silyl‐2‐Aminoacrylonitriles

inferredcites →https://doi.org/10.1002/cctc.202001949openalex-snapshot

Nickel‐Catalyzed Acyl Group Transfer of o‐Alkynylphenol Esters Accompanied by C−O Bond Fission for Synthesis of Benzo[b]furan

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Ruthenium‐Catalysed Synthesis of Functional Conjugated Dienes from Propargylic Carbonates and Silyl Diazo Compounds

inferredcites →https://doi.org/10.1002/chem.201501535openalex-snapshot

Stoichiometric and Catalytic Inter‐ and Intramolecular Hydroamination of Terminal Alkynes by Frustrated Lewis Pairs

inferredcites →https://doi.org/10.1002/chem.201502774openalex-snapshot

Cu‐Catalyzed Alkylative Carboxylation of Ynamides with Dialkylzinc Reagents and Carbon Dioxide

inferredcites →https://doi.org/10.1002/chem.201803147openalex-snapshot

Stereodivergent Alkyne Reduction by using Water as the Hydrogen Source

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DoE‐Driven Development of an Organocatalytic Enantioselective Addition of Acetaldehyde to Nitrostyrenes in Water**

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The M06 suite of density functionals for main group thermochemistry, thermochemical kinetics, noncovalent interactions, excited states, and transition elements: two new functionals and systematic testing of four M06-class functionals and 12 other functionals

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Recent advances in the synthesis of 1,1-diarylalkanes by transition-metal catalysis

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The anionic chemistry of ynamides: A review

inferredcites →https://doi.org/10.1016/j.xcrp.2020.100016openalex-snapshot

Radical Reactivity of Frustrated Lewis Pairs with Diaryl Esters

inferredcites →https://doi.org/10.1016/s0040-4039(00)00937-0openalex-snapshot

Novel stereoselective construction of a quaternary carbon: application to synthesis of the cyclopentenedione moiety of madindolines

inferredcites →https://doi.org/10.1021/acs.accounts.0c00417openalex-snapshot

Transition Metal-Catalyzed Tandem Reactions of Ynamides for Divergent N‑Heterocycle Synthesis

inferredcites →https://doi.org/10.1021/acs.joc.9b03512openalex-snapshot

Synthesis of Amide Enol Carbamates and Carbonates through Cu(OTf)2-Catalyzed Reactions of Ynamides with t-Butyl Carbamates/Carbonates

inferredcites →https://doi.org/10.1021/acs.organomet.7b00174openalex-snapshot

Mechanistic Insights into the B(C6F5)3-Initiated Aldehyde–Aniline–Alkyne Reaction To Form Substituted Quinolines

inferredcites →https://doi.org/10.1021/acs.organomet.7b00779openalex-snapshot

N-Heterocycle-Ligated Borocations as Highly Tunable Carbon Lewis Acids

inferredcites →https://doi.org/10.1021/acs.orglett.1c00631openalex-snapshot

Catalytic Asymmetric Hydroacyloxylation/Ring-Opening Reaction of Ynamides, Acids, and Aziridines

inferredcites →https://doi.org/10.1021/acs.orglett.1c02003openalex-snapshot

Tandem (2 + 2) Annulation/Retro-4π Electrocyclization/Imino-Nazarov Cyclization Reaction of p-Quinone Methides with Ynamides: Expeditious Construction of Functionalized Aminoindenes

inferredcites →https://doi.org/10.1021/acs.orglett.2c00197openalex-snapshot

Palladium-Catalyzed Regioselective Arylalkenylation of Ynamides

inferredcites →https://doi.org/10.1021/acs.orglett.2c00574openalex-snapshot

Boron Lewis Acid Catalyzed Intermolecular trans-Hydroarylation of Ynamides with Hydroxyarenes

inferredcites →https://doi.org/10.1021/acs.orglett.2c02161openalex-snapshot

Synthesis of Amide Enol 2-Iodobenzoates by the Regio- and Stereoselective Gold-Catalyzed Acyloxyalkynylation of Ynamides with Hypervalent Iodine Reagents

inferredcites →https://doi.org/10.1021/acs.orglett.7b00437openalex-snapshot

trans -Aminoboration across Internal Alkynes Catalyzed by B(C6F5)3 for the Synthesis of Borylated Indoles

inferredcites →https://doi.org/10.1021/acs.orglett.9b03468openalex-snapshot

Copper-Catalyzed Amino-oxymethylation of Ynamides with N,O-Acetals

inferredcites →https://doi.org/10.1021/acscatal.1c00461openalex-snapshot

Gold-Catalyzed 1,1-Carboalkoxylation of Oxetane-Ynamides via Exocyclic Metal Carbenes: Divergent and Atom-Economical Synthesis of Tricyclic N-Heterocycles

inferredcites →https://doi.org/10.1021/acscatal.2c00546openalex-snapshot

Catalytic Enantioselective Hydrovinylation of Trialkylsilyloxy and Acetoxy-1,3-Dienes: Cationic Co(I) Complexes for the Synthesis of Chiral Enolate Surrogates and Their Applications for Synthesis of Ketones and Cross-Coupling Reagents in High Enantiomeric Purity

inferredcites →https://doi.org/10.1021/acscatal.6b02072openalex-snapshot

Synthesis of Unsaturated N-Heterocycles by Cycloadditions of Aziridines and Alkynes

inferredcites →https://doi.org/10.1021/acscatal.6b02206openalex-snapshot

Highly Regio- and Stereoselective Synthesis of Z and E Enol Esters by an Amine-Catalyzed Conjugate Addition–Rearrangement Reaction of Ynals with Carboxylic Acids

inferredcites →https://doi.org/10.1021/acscatal.6b03399openalex-snapshot

Rhodium-Catalyzed Stereoselective Intramolecular Tandem Reaction of Vinyloxiranes with Alkynes: Atom- and Step-Economical Synthesis of Multifunctional Mono-, Bi-, and Tricyclic Compounds

inferredcites →https://doi.org/10.1021/acscatal.8b00955openalex-snapshot

Boron-Catalyzed Double Hydrofunctionalization Reactions of Unactivated Alkynes

inferredcites →https://doi.org/10.1021/acscatal.9b01851openalex-snapshot

Reversal of Regioselectivity in Ynamide Chemistry

inferredcites →https://doi.org/10.1021/acscatal.9b02275openalex-snapshot

Gold and Palladium Mediated Bimetallic Catalysis: Mechanistic Investigation through the Isolation of the Organogold(I) Intermediates

inferredcites →https://doi.org/10.1021/acscatal.9b04285openalex-snapshot

Palladium-Catalyzed Amide-Directed Hydrocarbofunctionalization of 3-Alkenamides with Alkynes

inferredcites →https://doi.org/10.1021/ar100082dopenalex-snapshot

Exploration of New C−O Electrophiles in Cross-Coupling Reactions

inferredcites →https://doi.org/10.1021/ar400193gopenalex-snapshot

Ynamides in Ring Forming Transformations

inferredcites →https://doi.org/10.1021/ar500375jopenalex-snapshot

Frustrated Lewis Pairs: From Concept to Catalysis

inferredcites →https://doi.org/10.1021/ar7001107openalex-snapshot

Asymmetric Hydrogenation Using Monodentate Phosphoramidite Ligands

inferredcites →https://doi.org/10.1021/ar700111aopenalex-snapshot

Density Functionals with Broad Applicability in Chemistry

inferredcites →https://doi.org/10.1021/cr00031a013openalex-snapshot

Molecular Interactions in Solution: An Overview of Methods Based on Continuous Distributions of the Solvent

inferredcites →https://doi.org/10.1021/cr100259topenalex-snapshot

Nickel-Catalyzed Cross-Couplings Involving Carbon−Oxygen Bonds

inferredcites →https://doi.org/10.1021/ja0058280openalex-snapshot

Stereoselective Generation of E- and Z-Disubstituted Amide Enolates. Reductive Enolate Formation from Bicyclic Thioglycolate Lactams

inferredcites →https://doi.org/10.1021/ja034369aopenalex-snapshot

Enol Ester as an Olefinic Partner in Enyne Cyclization. A Novel Tandem Cyclization to Stereodefined Bicyclo[3.3.0]octenes

inferredcites →https://doi.org/10.1021/ja044812xopenalex-snapshot

The Enantioselective Tsuji Allylation

inferredcites →https://doi.org/10.1021/ja055968fopenalex-snapshot

Palladium-Catalyzed Asymmetric Allylic α-Alkylation of Acyclic Ketones

inferredcites →https://doi.org/10.1021/ja103771wopenalex-snapshot

Palladium-Catalyzed Asymmetric Allylic Alkylation of 2-Acylimidazoles as Ester Enolate Equivalents

inferredcites →https://doi.org/10.1021/ja803480bopenalex-snapshot

Preparation of Substituted Enol Derivatives From Terminal Alkynes and Their Synthetic Utility

inferredcites →https://doi.org/10.1021/ja806021yopenalex-snapshot

Stereocontrolled Alkylative Construction of Quaternary Carbon Centers

inferredcites →https://doi.org/10.1021/ja900946hopenalex-snapshot

Stereoselective Synthesis of Multisubstituted Enamides via Rhodium-Catalyzed Carbozincation of Ynamides

inferredcites →https://doi.org/10.1021/ja901048wopenalex-snapshot

Gold-Catalyzed Homogeneous Oxidative C−O Bond Formation: Efficient Synthesis of 1-Benzoxyvinyl Ketones

inferredcites →https://doi.org/10.1021/ja9053948openalex-snapshot

Palladium-Catalyzed Decarboxylative Asymmetric Allylic Alkylation of Enol Carbonates

inferredcites →https://doi.org/10.1021/ja9068497openalex-snapshot

Catalyzed Catalysis Using Carbophilic Lewis Acidic Gold and Lewis Basic Palladium: Synthesis of Substituted Butenolides and Isocoumarins

inferredcites →https://doi.org/10.1021/ja982857qopenalex-snapshot

Enantioselective Aldol Reactions Catalyzed by Tin Methoxide and BINAP·Silver(I) Complex

inferredcites →https://doi.org/10.1021/jacs.1c01622openalex-snapshot

Site-Selective Csp3–Csp/Csp3–Csp2 Cross-Coupling Reactions Using Frustrated Lewis Pairs

inferredcites →https://doi.org/10.1021/jacs.1c09148openalex-snapshot

Ternary Catalysis Enabled Three-Component Asymmetric Allylic Alkylation as a Concise Track to Chiral α,α-Disubstituted Ketones

inferredcites →https://doi.org/10.1021/jacs.5b06794openalex-snapshot

Frustrated Lewis Pairs

inferredcites →https://doi.org/10.1021/jacs.7b04086openalex-snapshot

Enantioselective Construction of Acyclic Quaternary Carbon Stereocenters: Palladium-Catalyzed Decarboxylative Allylic Alkylation of Fully Substituted Amide Enolates

inferredcites →https://doi.org/10.1021/jacs.8b05560openalex-snapshot

Catalytic Enantioselective Synthesis of Acyclic Quaternary Centers: Palladium-Catalyzed Decarboxylative Allylic Alkylation of Fully Substituted Acyclic Enol Carbonates

inferredcites →https://doi.org/10.1021/jacs.8b09851openalex-snapshot

Radical Germylzincation of α-Heteroatom-Substituted Alkynes

inferredcites →https://doi.org/10.1021/jacs.8b13757openalex-snapshot

Enantioselective Conia-Ene-Type Cyclizations of Alkynyl Ketones through Cooperative Action of B(C6F5)3, N-Alkylamine and a Zn-Based Catalyst

inferredcites →https://doi.org/10.1021/jo01047a022openalex-snapshot

The Chemistry of Carbanions. V. The Enolates Derived from Unsymmetrical Ketones1a

inferredcites →https://doi.org/10.1021/jo0105181openalex-snapshot

Palladium(II)-Catalyzed Asymmetric Cyclization of (Z)-4‘-Acetoxy-2‘-butenyl 2-Alkynoates. Role of Nitrogen-Containing Ligands in Palladium(II)-Mediated Reactions

inferredcites →https://doi.org/10.1021/jo048414oopenalex-snapshot

Cycloisomerization of 1,6-Enynes Using Acetate as a Nucleophile under Palladium(II) Catalysis

inferredcites →https://doi.org/10.1021/jo9522466openalex-snapshot

Palladium-Catalyzed Nucleophile−Alkyne−α,β-Unsaturated Carbonyl Coupling through Tandem Nucleopalladation and Conjugate Addition

inferredcites →https://doi.org/10.1021/np970576aopenalex-snapshot

Grenadadiene and Grenadamide, Cyclopropyl-Containing Fatty Acid Metabolites from the Marine Cyanobacterium Lyngbya majuscula

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Palladium(II)-Catalyzed Three-Component Coupling Reaction Initiated by Acetoxypalladation of Alkynes: An Efficient Route to γ,δ-Unsaturated Carbonyls

inferredcites →https://doi.org/10.1021/ol300158dopenalex-snapshot

Regiodivergent Synthesis of Functionalized Indene Derivatives via Pt-Catalyzed Rautenstrauch Reaction of Propargyl Carbonates

inferredcites →https://doi.org/10.1021/ol301563gopenalex-snapshot

[Pd(μ-Br)(PtBu3)]2 as a Highly Active Isomerization Catalyst: Synthesis of Enol Esters from Allylic Esters

inferredcites →https://doi.org/10.1021/ol303474aopenalex-snapshot

Synthesis of 3-Alkyl- or 3-Allenyl-2-amidobenzofurans via Electrophilic Cyclization of o-Anisole-Substituted Ynamides with Carbocations

inferredcites →https://doi.org/10.1021/ol4013712openalex-snapshot

Copper-Catalyzed Nondecarboxylative Cross Coupling of Alkenyltrifluoroborate Salts with Carboxylic Acids or Carboxylates: Synthesis of Enol Esters

inferredcites →https://doi.org/10.1021/ol701717zopenalex-snapshot

Enol Esters: Versatile Substrates for Mannich-Type Multicomponent Reactions

inferredcites →https://doi.org/10.1021/ol8019567openalex-snapshot

Bismuth-Catalyzed Intramolecular Carbo-oxycarbonylation of 3-Alkynyl Esters

inferredcites →https://doi.org/10.1038/nature11569openalex-snapshot

Forming all-carbon quaternary stereogenic centres in acyclic systems from alkynes

inferredcites →https://doi.org/10.1038/nchem.131openalex-snapshot

A unique approach to aldol products for the creation of all-carbon quaternary stereocentres

inferredcites →https://doi.org/10.1038/ncomms4470openalex-snapshot

A general ligand design for gold catalysis allowing ligand-directed anti-nucleophilic attack of alkynes

inferredcites →https://doi.org/10.1038/nprot.2013.036openalex-snapshot

Stereodefined trisubstituted enolates as a unique entry to all-carbon quaternary stereogenic centers in acyclic systems

inferredcites →https://doi.org/10.1038/s41467-019-11245-2openalex-snapshot

Stereoselective synthesis of medium lactams enabled by metal-free hydroalkoxylation/stereospecific [1,3]-rearrangement

inferredcites →https://doi.org/10.1038/s41557-021-00778-zopenalex-snapshot

Asymmetric dearomatization catalysed by chiral Brønsted acids via activation of ynamides

inferredcites →https://doi.org/10.1038/s41570-021-00266-5openalex-snapshot

Bifunctional reagents in organic synthesis

inferredcites →https://doi.org/10.1039/b211277aopenalex-snapshot

Regiocontrolled Ru-catalyzed addition of carboxylic acids to alkynes: practical protocols for the synthesis of vinyl estersWe thank Prof. Dr. M. T. Reetz for generous support and constant encouragement, and gratefully acknowledge the DFG, the FCI, and the BMBF for financial support.

inferredcites →https://doi.org/10.1039/c0cc03723kopenalex-snapshot

Acetoxypalladation of unactivated alkynes and capture with alkenes to give 1-acetoxy-1,3-dienes taking dioxygen as terminal oxidant

inferredcites →https://doi.org/10.1039/c1cc13595copenalex-snapshot

Palladium-catalyzed hydroacyloxylation of ynamides

inferredcites →https://doi.org/10.1039/c3cc00273jopenalex-snapshot

Gold-catalysed cascade rearrangements of ynamide propargyl esters

inferredcites →https://doi.org/10.1039/c4cc04391jopenalex-snapshot

Stereodefined acyclic trisubstituted metal enolates towards the asymmetric formation of quaternary carbon stereocentres

inferredcites →https://doi.org/10.1039/c4cs00451eopenalex-snapshot

A unified survey of Si–H and H–H bond activation catalysed by electron-deficient boranes

inferredcites →https://doi.org/10.1039/c4gc01328jopenalex-snapshot

Metal-free hydroacyloxylation and hydration reactions of ynamides: synthesis of α-acyloxyenamides and N-acylsulfonamides

inferredcites →https://doi.org/10.1039/c5sc03282bopenalex-snapshot

Advanced 1,1-carboboration reactions with pentafluorophenylboranes

inferredcites →https://doi.org/10.1039/c6cc01565dopenalex-snapshot

Regioselective synthesis of 3,4-disubstituted isocoumarins through the Pd-catalyzed annulation of 2-iodoaromatic acids with ynamides

inferredcites →https://doi.org/10.1039/c6dt04725dopenalex-snapshot

Borane-catalyzed indole synthesis through intramolecular hydroamination

inferredcites →https://doi.org/10.1039/c6sc03036jopenalex-snapshot

Enantioselective allylic alkylation of stereodefined polysubstituted copper enolates as an entry to acyclic quaternary carbon stereocentres

inferredcites →https://doi.org/10.1039/c8cc07328gopenalex-snapshot

1,4-Conjugate addition/esterification of ortho -quinone methides in a multicomponent reaction

inferredcites →https://doi.org/10.1039/c9cc08654dopenalex-snapshot

Frustrated Lewis pair-catalyzed double hydroarylation of alkynes with N -substituted pyrroles

inferredcites →https://doi.org/10.1039/c9cs00769eopenalex-snapshot

Halogenated triarylboranes: synthesis, properties and applications in catalysis

inferredcites →https://doi.org/10.1039/c9sc00334gopenalex-snapshot

Synthesis of sterically hindered 4,5-diarylphenanthrenes via acid-catalyzed bisannulation of benzenediacetaldehydes with alkynes

inferredcites →https://doi.org/10.1039/c9sc01726gopenalex-snapshot

Palladium-catalyzed enantioselective decarboxylative allylic alkylation of fully substituted N -acyl indole-derived enol carbonates

inferredcites →https://doi.org/10.1039/d0cc01424aopenalex-snapshot

Copper-catalyzed tandem cis -carbometallation/cyclization of imine-ynamides with arylboronic acids

inferredcites →https://doi.org/10.1039/d0cs00283fopenalex-snapshot

Reactivity of ynamides in catalytic intermolecular annulations

inferredcites →https://doi.org/10.1039/d0cs00380hopenalex-snapshot

Electron-deficient boron-based catalysts for C–H bond functionalisation

inferredcites →https://doi.org/10.1039/d0cs00474jopenalex-snapshot

Brønsted acid-mediated reactions of ynamides

inferredcites →https://doi.org/10.1039/d0cs00531bopenalex-snapshot

Electron deficient borane-mediated hydride abstraction in amines: stoichiometric and catalytic processes

inferredcites →https://doi.org/10.1039/d0cs00700eopenalex-snapshot

The interplay of carbophilic activation and Au( i )/Au( iii ) catalysis: an emerging technique for 1,2-difunctionalization of C–C multiple bonds

inferredcites →https://doi.org/10.1039/d0cs00769bopenalex-snapshot

Asymmetric synthesis with ynamides: unique reaction control, chemical diversity and applications

inferredcites →https://doi.org/10.1039/d0cy01339kopenalex-snapshot

Triarylborane catalysed N -alkylation of amines with aryl esters

inferredcites →https://doi.org/10.1039/d0ob02478copenalex-snapshot

Tris(pentafluorophenyl)borane catalyzed C–C and C–heteroatom bond formation

inferredcites →https://doi.org/10.1039/d0qo01097aopenalex-snapshot

Ni-Catalyzed stereoselective difunctionalization of alkynes

inferredcites →https://doi.org/10.1039/d0sc03712eopenalex-snapshot

Defunctionalisation catalysed by boron Lewis acids

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